A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system Article Swipe
Tianle Pan
,
Andrew T. Lambe
,
Weiwei Hu
,
Yicong He
,
Minghao Hu
,
Huaishan Zhou
,
Xinming Wang
,
Qingqing Hu
,
Hui Chen
,
Yue Zhao
,
Yuanlong Huang
,
Doug R. Worsnop
,
Zhe Peng
,
Melissa A. Morris
,
Douglas A. Day
,
Pedro Campuzano‐Jost
,
J. L. Jiménez
,
Shantanu H. Jathar
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.5194/amt-17-4915-2024
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.5194/amt-17-4915-2024
Oxidation flow reactors (OFRs) have been extensively utilized to examine the formation of secondary organic aerosol (SOA). However, the UV lamps typically employed to initiate the photochemistry in OFRs can result in an elevated reactor temperature when their implications are not thoroughly evaluated. In this study, we conducted a comprehensive investigation into the temperature distribution within an Aerodyne potential aerosol mass OFR (PAM-OFR) and then examined the subsequent effects on flow and chemistry due to lamp heating. A lamp-induced temperature increase was observed, which was a function of lamp-driving voltage, number of lamps, lamp types, OFR residence time, and positions within the PAM-OFR. Under typical PAM-OFR operational conditions (e.g., < 5 d of equivalent atmospheric OH exposure under low-NOx conditions), the temperature increase typically ranged from 1–5 °C. Under extreme (but less frequently encountered) conditions, the heating could reach up to 15 °C. The influences of the increased temperature over ambient conditions on the flow distribution, gas, and condensed-phase chemistry within PAM-OFR were evaluated. Our findings indicate that the increase in temperature altered the flow field, resulting in a diminished tail on the residence time distribution and corresponding oxidant exposure due to faster recirculation. According to simulation results from a radical chemistry box model, the variation in absolute oxidant concentration within PAM-OFR due to temperature increase was minimal (< 5 %). The temperature influences on seed organic aerosol (OA) and newly formed secondary OA were also investigated, suggesting that an increase in temperature can impact the yield, size, and oxidation levels of representative biogenic and anthropogenic SOA types. Recommendations for temperature-dependent SOA yield corrections and PAM-OFR operating protocols that mitigate lamp-induced temperature enhancement and fluctuations are presented. We recommend blowing air around the reactor's exterior with fans during PAM-OFR experiments to minimize the temperature increase within PAM-OFR. Temperature increases are substantially lower for OFRs utilizing less powerful lamps compared to the Aerodyne version.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.5194/amt-17-4915-2024
- OA Status
- gold
- Cited By
- 2
- References
- 150
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4401918917
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4401918917Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.5194/amt-17-4915-2024Digital Object Identifier
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A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) systemWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-08-27Full publication date if available
- Authors
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Tianle Pan, Andrew T. Lambe, Weiwei Hu, Yicong He, Minghao Hu, Huaishan Zhou, Xinming Wang, Qingqing Hu, Hui Chen, Yue Zhao, Yuanlong Huang, Doug R. Worsnop, Zhe Peng, Melissa A. Morris, Douglas A. Day, Pedro Campuzano‐Jost, J. L. Jiménez, Shantanu H. JatharList of authors in order
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https://doi.org/10.5194/amt-17-4915-2024Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.5194/amt-17-4915-2024Direct OA link when available
- Concepts
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Aerosol, Chemistry, Flow (mathematics), Environmental chemistry, Mechanics, Organic chemistry, PhysicsTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2025: 2Per-year citation counts (last 5 years)
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150Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| primary_location.raw_source_name | Atmospheric Measurement Techniques |
| primary_location.landing_page_url | https://doi.org/10.5194/amt-17-4915-2024 |
| publication_date | 2024-08-27 |
| publication_year | 2024 |
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