A Highly Stable Yttrium Organic Framework as a Host for Optical Thermometry and D2O Detection Article Swipe
Thomas W. Chamberlain
,
Rafael V. Perrella
,
Tamires M. Oliveira
,
Paulo C. de Sousa Filho
,
Richard I. Walton
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1002/chem.202200410
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1002/chem.202200410
The yttrium organic framework (Y 0.89 Tb 0.10 Eu 0.01 ) 6 (BDC) 7 (OH) 4 (H 2 O) 4 (BDC=benzene‐1,4‐dicarboxylate) is hydrothermally stable up to at least 513 K and thermally stable in air in excess of 673 K. The relative intensities of luminescence of Tb 3+ and Eu 3+ are governed by Tb 3+ ‐to‐Eu 3+ phonon‐assisted energy transfer and Tb 3+ ‐to‐ligand back transfer and are responsible for the differing temperature‐dependent luminescence of the two ions. This provides a ratiometric luminescent thermometer in the 288–573 K temperature range, not previously seen for MOF materials, with a high sensitivity, 1.69±0.04 % K −1 at 523 K. In aqueous conditions, loosely bound H 2 O can be replaced by D 2 O in the same material, which modifies decay lifetimes to yield a quantitative luminescent D 2 O sensor with a useful sensitivity for practical application.
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Metadata
- Type
- article
- Language
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All OpenAlex metadata
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https://doi.org/10.1002/chem.202200410Digital Object Identifier
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A Highly Stable Yttrium Organic Framework as a Host for Optical Thermometry and D2O DetectionWork title
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articleOpenAlex work type
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enPrimary language
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2022Year of publication
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2022-02-14Full publication date if available
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Thomas W. Chamberlain, Rafael V. Perrella, Tamires M. Oliveira, Paulo C. de Sousa Filho, Richard I. WaltonList of authors in order
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https://doi.org/10.1002/chem.202200410Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1002/chem.202200410Direct OA link when available
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Yttrium, Host (biology), Materials science, Environmental science, Biology, Ecology, Metallurgy, OxideTop concepts (fields/topics) attached by OpenAlex
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19Total citation count in OpenAlex
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2025: 4, 2024: 3, 2023: 2, 2022: 10Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| publication_date | 2022-02-14 |
| publication_year | 2022 |
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