A Step Forward in Understanding the Hydrogen Adsorption and Compression on Activated Carbons Article Swipe

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Pamela Ramírez-Vidal , Rafael Luan Sehn Canevesi , Giuseppe Sdanghi , Sébastien Schaefer , Gaël Maranzana , Alain Celzard , Vanessa Fierro ·

YOU? · · 2021 · Open Access · · DOI: https://doi.org/10.1021/acsami.0c22192

Hydrogen adsorption on activated carbons (ACs) is a promising alternative to compression and liquefaction for storing hydrogen. Herein, we have studied hydrogen adsorption on six commercial ACs (CACs) with surface areas ranging from 996 to 2216 m² g^-1 in a temperature range of 77 to 273 K and pressures up to 15 MPa. Excess hydrogen adsorption capacities of 2.3 to 5.8 wt % were obtained at 77 K and 4 MPa. We demonstrated that, contrary to what is normally done, hydrogen capacity is more accurately predicted by the surface area determined by the nonlocal density functional theory method applied to N₂ and CO₂ adsorption data than by the Brunauer-Emmett-Teller (BET) area. The modified Dubinin-Astakhov (MDA) equation was used to fit the experimental adsorption data, and the relationship between the MDA parameters (n_max, V_a, α, and β) and the textural properties of the CACs was determined for the first time. We concluded that the n_max and V_a parameters are related to the BET area, while the α and β parameters are related to the average micropore size and total pore volume, respectively. α and β were used to evaluate the enthalpy and entropy of adsorption and we show that these parameters can be used to assess the best carbon for hydrogen storage or compression.

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Adsorption Hydrogen storage Activated carbon Materials science Hydrogen Enthalpy Microporous material BET theory Specific surface area Volume (thermodynamics) Thermodynamics Liquefaction Carbon fibers Chemical engineering Composite material Organic chemistry Chemistry Composite number Catalysis Physics Engineering

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Type: article
Language: en
Landing Page: https://doi.org/10.1021/acsami.0c22192
OA Status: green
Cited By: 76
References: 69
Related Works: 10
OpenAlex ID: https://openalex.org/W3135073284

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DOI: https://doi.org/10.1021/acsami.0c22192

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Title: A Step Forward in Understanding the Hydrogen Adsorption and Compression on Activated Carbons

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Language: en

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Publication year: 2021

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Publication date: 2021-03-04

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Authors: Pamela Ramírez-Vidal, Rafael Luan Sehn Canevesi, Giuseppe Sdanghi, Sébastien Schaefer, Gaël Maranzana, Alain Celzard, Vanessa Fierro

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Landing page: https://doi.org/10.1021/acsami.0c22192

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Concepts: Adsorption, Hydrogen storage, Activated carbon, Materials science, Hydrogen, Enthalpy, Microporous material, BET theory, Specific surface area, Volume (thermodynamics), Thermodynamics, Liquefaction, Carbon fibers, Chemical engineering, Composite material, Organic chemistry, Chemistry, Composite number, Catalysis, Physics, Engineering

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Cited by: 76

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