Acidity drives selectivity: tuning reaction pathways under hydrodeoxygenation conditions Article Swipe
Guilherme B. Strapasson
,
Gabriel B. Báfero
,
Davi S. Leite
,
D Santos
,
Ângela Albuquerque
,
Ingrid D. Barcelos
,
Liane M. Rossi
,
Cristiane B. Rodella
,
Daniela Zanchet
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2024-vx59v
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2024-vx59v
The design and tuning of active sites (e.g., metallic, acid, and redox sites) are crucial for developing active, selective, and stable catalysts. Metal-support interactions (MSI) and the creation of interfacial sites can tailor the catalytic performance of metal/oxide catalysts for various reactions, directly impacting C-O, C-C, and C-H bond activation and H2 spillover. By modulating the acidity of the support (i.e., Brønsted-rich or Lewis-rich), we elucidate the role of acid sites over the acetone hydrodeoxygenation reaction pathways. Brønsted-rich catalysts favor the formation of selective C-O bond cleavage products, whereas Lewis-rich catalysts favor C-C coupling + C-O bond cleavage cascade products. We demonstrate that tailoring active sites from the support and constructing active metal-oxide interfacial sites can tune the catalytic performance toward targeted reaction pathways with enhanced stability. Our findings provide insights into C-O, C-C, and C-H bond activation, cleavage, and coupling that can be expanded to multiple catalytic reactions, contributing to the development of new functional materials with enhanced performance.
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Metadata
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- preprint
- Language
- en
- Landing Page
- https://doi.org/10.26434/chemrxiv-2024-vx59v
- https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/6734b1297be152b1d0f46796/original/acidity-drives-selectivity-tuning-reaction-pathways-under-hydrodeoxygenation-conditions.pdf
- OA Status
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All OpenAlex metadata
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https://doi.org/10.26434/chemrxiv-2024-vx59vDigital Object Identifier
- Title
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Acidity drives selectivity: tuning reaction pathways under hydrodeoxygenation conditionsWork title
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-11-19Full publication date if available
- Authors
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Guilherme B. Strapasson, Gabriel B. Báfero, Davi S. Leite, D Santos, Ângela Albuquerque, Ingrid D. Barcelos, Liane M. Rossi, Cristiane B. Rodella, Daniela ZanchetList of authors in order
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https://doi.org/10.26434/chemrxiv-2024-vx59vPublisher landing page
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https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/6734b1297be152b1d0f46796/original/acidity-drives-selectivity-tuning-reaction-pathways-under-hydrodeoxygenation-conditions.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/6734b1297be152b1d0f46796/original/acidity-drives-selectivity-tuning-reaction-pathways-under-hydrodeoxygenation-conditions.pdfDirect OA link when available
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Hydrodeoxygenation, Selectivity, Chemistry, Catalysis, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.(i.e., | 60 |
| abstract_inverted_index.active | 5, 104, 111 |
| abstract_inverted_index.design | 1 |
| abstract_inverted_index.sites) | 12 |
| abstract_inverted_index.stable | 20 |
| abstract_inverted_index.tailor | 32 |
| abstract_inverted_index.toward | 120 |
| abstract_inverted_index.tuning | 3 |
| abstract_inverted_index.acetone | 73 |
| abstract_inverted_index.acidity | 56 |
| abstract_inverted_index.active, | 17 |
| abstract_inverted_index.cascade | 98 |
| abstract_inverted_index.crucial | 14 |
| abstract_inverted_index.provide | 129 |
| abstract_inverted_index.support | 59, 108 |
| abstract_inverted_index.various | 40 |
| abstract_inverted_index.whereas | 88 |
| abstract_inverted_index.cleavage | 86, 97 |
| abstract_inverted_index.coupling | 93, 140 |
| abstract_inverted_index.creation | 27 |
| abstract_inverted_index.directly | 42 |
| abstract_inverted_index.enhanced | 125, 158 |
| abstract_inverted_index.expanded | 144 |
| abstract_inverted_index.findings | 128 |
| abstract_inverted_index.insights | 130 |
| abstract_inverted_index.multiple | 146 |
| abstract_inverted_index.pathways | 123 |
| abstract_inverted_index.reaction | 75, 122 |
| abstract_inverted_index.targeted | 121 |
| abstract_inverted_index.catalysts | 38, 78, 90 |
| abstract_inverted_index.catalytic | 34, 118, 147 |
| abstract_inverted_index.cleavage, | 138 |
| abstract_inverted_index.elucidate | 65 |
| abstract_inverted_index.formation | 81 |
| abstract_inverted_index.impacting | 43 |
| abstract_inverted_index.materials | 156 |
| abstract_inverted_index.metallic, | 8 |
| abstract_inverted_index.pathways. | 76 |
| abstract_inverted_index.products, | 87 |
| abstract_inverted_index.products. | 99 |
| abstract_inverted_index.selective | 83 |
| abstract_inverted_index.tailoring | 103 |
| abstract_inverted_index.Lewis-rich | 89 |
| abstract_inverted_index.activation | 49 |
| abstract_inverted_index.catalysts. | 21 |
| abstract_inverted_index.developing | 16 |
| abstract_inverted_index.functional | 155 |
| abstract_inverted_index.modulating | 54 |
| abstract_inverted_index.reactions, | 41, 148 |
| abstract_inverted_index.selective, | 18 |
| abstract_inverted_index.spillover. | 52 |
| abstract_inverted_index.stability. | 126 |
| abstract_inverted_index.activation, | 137 |
| abstract_inverted_index.demonstrate | 101 |
| abstract_inverted_index.development | 152 |
| abstract_inverted_index.interfacial | 29, 113 |
| abstract_inverted_index.metal-oxide | 112 |
| abstract_inverted_index.metal/oxide | 37 |
| abstract_inverted_index.performance | 35, 119 |
| abstract_inverted_index.Lewis-rich), | 63 |
| abstract_inverted_index.constructing | 110 |
| abstract_inverted_index.contributing | 149 |
| abstract_inverted_index.interactions | 23 |
| abstract_inverted_index.performance. | 159 |
| abstract_inverted_index.Metal-support | 22 |
| abstract_inverted_index.Brønsted-rich | 61, 77 |
| abstract_inverted_index.hydrodeoxygenation | 74 |
| cited_by_percentile_year | |
| countries_distinct_count | 1 |
| institutions_distinct_count | 9 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/9 |
| sustainable_development_goals[0].score | 0.5299999713897705 |
| sustainable_development_goals[0].display_name | Industry, innovation and infrastructure |
| citation_normalized_percentile.value | 0.27554761 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |