AIEgen configuration transition and aggregation enable dual prompt emission for single‐component nondoped white OLEDs Article Swipe
Jiasen Zhang
,
Qiang Wei
,
Wei Li
,
Hao Chen
,
Xiangyu Zhu
,
Yongqi Bai
,
Nannan Fei
,
Liang Cao
,
Zujin Zhao
,
Anjun Qin
,
Ben Zhong Tang
,
Ziyi Ge
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/agt2.410
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/agt2.410
The dual emission (DE) feature in materials holds great potential to revolutionize the development of one‐component system white organic light‐emitting diodes (WOLEDs). However, the reported DE materials remain scarce owing to the formidable challenge of breaking Kasha's rule and managing the intricate energy/charge transfer processes. Herein, we have introduced a groundbreaking DE AIEgen, 2CzAn‐TPE , which possesses a simple structure and undergoes Z ‐to‐ E isomerization and exhibits yellow and red fluorescence powders for pre ‐ and post ‐sublimation, respectively. With relatively lower potential energy, Z ‐conformation (( Z )‐1,2‐diphenyl‐1,2‐bis(4‐(10‐(9‐phenyl‐9 H ‐carbazol‐3‐yl)anthracen‐9‐yl)phenyl)ethene) of 2CzAn‐TPE can be readily transformed into E ‐conformation (( E )‐1,2‐diphenyl‐1,2‐bis(4‐(10‐(9‐phenyl‐9 H ‐carbazol‐3‐yl)anthracen‐9‐yl)phenyl)ethene) via vacuum sublimation. The utilization of X‐ray diffraction and grazing‐incidence‐wide‐angle X‐ray scattering techniques confirms the structural transformation, while the crystallographic analysis reveals the establishment of numerous intermolecular CH···π interactions between the tetraphenylethene (TPE) moiety and both the anthracene and carbazole units. This allows a densely packed molecular arrangement, thereby offering propitious conditions for excimer generation in the E ‐conformation aggregated state. By utilizing the sublimated 2CzAn‐TPE as an emitter, a nondoped one‐component WOLED was prepared, exhibiting an exceptionally high external quantum efficiency (EQE) of 5.0%, which represents one of the highest performances among all one‐component WOLEDs. This research introduces a novel, simple, and efficient approach to realize highly efficient one‐molecule WOLEDs.
Related Topics
Concepts
OLED
Sublimation (psychology)
Intermolecular force
Quantum efficiency
Aggregation-induced emission
Chemistry
Carbazole
Materials science
Anthracene
Perylene
Crystallography
Photochemistry
Fluorescence
Molecule
Nanotechnology
Optoelectronics
Organic chemistry
Psychology
Quantum mechanics
Layer (electronics)
Psychotherapist
Physics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/agt2.410
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/agt2.410
- OA Status
- gold
- Cited By
- 24
- References
- 37
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4386222068
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4386222068Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/agt2.410Digital Object Identifier
- Title
-
AIEgen configuration transition and aggregation enable dual prompt emission for single‐component nondoped white OLEDsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-08-27Full publication date if available
- Authors
-
Jiasen Zhang, Qiang Wei, Wei Li, Hao Chen, Xiangyu Zhu, Yongqi Bai, Nannan Fei, Liang Cao, Zujin Zhao, Anjun Qin, Ben Zhong Tang, Ziyi GeList of authors in order
- Landing page
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https://doi.org/10.1002/agt2.410Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/agt2.410Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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-
goldOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/agt2.410Direct OA link when available
- Concepts
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OLED, Sublimation (psychology), Intermolecular force, Quantum efficiency, Aggregation-induced emission, Chemistry, Carbazole, Materials science, Anthracene, Perylene, Crystallography, Photochemistry, Fluorescence, Molecule, Nanotechnology, Optoelectronics, Organic chemistry, Psychology, Quantum mechanics, Layer (electronics), Psychotherapist, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
24Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 12, 2024: 10, 2023: 2Per-year citation counts (last 5 years)
- References (count)
-
37Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W2883766801, https://openalex.org/W4322767138, https://openalex.org/W3166344869, https://openalex.org/W3137613351, https://openalex.org/W3093783880, https://openalex.org/W3175991504, https://openalex.org/W2751375647, https://openalex.org/W2911023242, https://openalex.org/W2742925301, https://openalex.org/W3035855873, https://openalex.org/W3048553348, https://openalex.org/W2742628461, https://openalex.org/W2559806631, https://openalex.org/W3088852499, https://openalex.org/W2887309051, https://openalex.org/W2803218699, https://openalex.org/W3117927311, https://openalex.org/W2987505784, https://openalex.org/W2004461657, https://openalex.org/W4297025052, https://openalex.org/W3200492585, https://openalex.org/W4313812500, https://openalex.org/W4283822917, https://openalex.org/W3002119942, https://openalex.org/W3128928209, https://openalex.org/W3134087006, https://openalex.org/W2568638133, https://openalex.org/W2336333337, https://openalex.org/W1963505485, https://openalex.org/W3044415569, https://openalex.org/W3195588649, https://openalex.org/W286333679, https://openalex.org/W4379527490, https://openalex.org/W2252895594, https://openalex.org/W3043044470, https://openalex.org/W2590646638, https://openalex.org/W3127601952 |
| referenced_works_count | 37 |
| abstract_inverted_index., | 55 |
| abstract_inverted_index.E | 65, 100, 103, 164 |
| abstract_inverted_index.H | 91, 105 |
| abstract_inverted_index.Z | 63, 86, 89 |
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| abstract_inverted_index.(WOLEDs). | 22 |
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| abstract_inverted_index.challenge | 34 |
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| abstract_inverted_index.)‐1,2‐diphenyl‐1,2‐bis(4‐(10‐(9‐phenyl‐9 | 90, 104 |
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| corresponding_author_ids | https://openalex.org/A5016131764, https://openalex.org/A5089379373, https://openalex.org/A5072302687, https://openalex.org/A5068310044 |
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| institutions_distinct_count | 12 |
| corresponding_institution_ids | https://openalex.org/I19820366, https://openalex.org/I4210116924, https://openalex.org/I4210165038, https://openalex.org/I4210165339 |
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| sustainable_development_goals[0].display_name | Affordable and clean energy |
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