An Efficient and Stable Lithium‐Oxygen Battery Based on Metal‐Organic Framework Separator Operating at 160 °C Article Swipe
Qianyuan Qiu
,
Jiashu Yuan
,
Gen Li
,
Zheng‐Ze Pan
,
Penghui Yao
,
Yicheng Zhao
,
Cuijuan Zhang
,
Yongdan Li
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/admt.202300743
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/admt.202300743
A lithium oxygen battery (LOB) with molten salt electrolyte operating at elevated temperature has aroused great interest because it enables fast reaction kinetics. However, there is still a lack of open literature on the separator (membrane) of this kind of LOB. Metal‐organic framework (MOF) materials are widely used as components of separators in many kinds of energy storage devices, due to their regular crystalline and well‐defined pore structures. In this work, a MOF material, zirconium (II) 1,4‐benzenedicarboxylate after lithiation (UiO‐66‐SO 3 Li) with a narrow pore size (6 Å), is used as a key component of the separator for LOB operating at elevated temperature. A “rolling dough” method is adopted to prepare the separator, which achieves 100% material utilization. The LOB with this membrane operates at 160 °C and delivers a specific capacity of 5.1 mAh cm −2 with an overpotential as low as 40 mV at 0.1 mA cm −2 and a prolonged cycle life, 180 cycles with a high coulombic efficiency of 99.9% at 0.5 mA cm −2 . This MOF‐based membrane provides efficient Li + transfer and restricts discharge product migration during battery operation, which is promising for the development of LOB in large‐scale practical applications.
Related Topics
Concepts
Separator (oil production)
Overpotential
Faraday efficiency
Electrolyte
Materials science
Zirconium
Chemical engineering
Membrane
Metal-organic framework
Operating temperature
Electrode
Chemistry
Metallurgy
Electrochemistry
Thermodynamics
Organic chemistry
Physical chemistry
Physics
Biochemistry
Adsorption
Engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/admt.202300743
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/admt.202300743
- OA Status
- hybrid
- Cited By
- 4
- References
- 22
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4388575964
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4388575964Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/admt.202300743Digital Object Identifier
- Title
-
An Efficient and Stable Lithium‐Oxygen Battery Based on Metal‐Organic Framework Separator Operating at 160 °CWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-11-10Full publication date if available
- Authors
-
Qianyuan Qiu, Jiashu Yuan, Gen Li, Zheng‐Ze Pan, Penghui Yao, Yicheng Zhao, Cuijuan Zhang, Yongdan LiList of authors in order
- Landing page
-
https://doi.org/10.1002/admt.202300743Publisher landing page
- PDF URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/admt.202300743Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/admt.202300743Direct OA link when available
- Concepts
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Separator (oil production), Overpotential, Faraday efficiency, Electrolyte, Materials science, Zirconium, Chemical engineering, Membrane, Metal-organic framework, Operating temperature, Electrode, Chemistry, Metallurgy, Electrochemistry, Thermodynamics, Organic chemistry, Physical chemistry, Physics, Biochemistry, Adsorption, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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4Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 2, 2024: 2Per-year citation counts (last 5 years)
- References (count)
-
22Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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