An intense source for cold cluster ions of a specific composition Article Swipe
Lukas Tiefenthaler
,
João Ameixa
,
Paul Martini
,
Simon Albertini
,
Lorenz Ballauf
,
M. Zankl
,
Marcelo Goulart
,
Felix Laimer
,
K. von Haeften
,
Fábio Zappa
,
P. Scheier
·
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1063/1.5133112
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1063/1.5133112
The demand for nanoscale materials of ultra-high purity and narrow size distribution is addressed. Clusters of Au, C60, H2O, and serine are produced inside helium nanodroplets using a combination of ionization, mass filtering, collisions with atomic or molecular vapor, and electrostatic extraction, in a specific and novel sequence. The helium droplets are produced in an expansion of cold helium gas through a nozzle into vacuum. The droplets are ionized by electron bombardment and subjected to a mass filter. The ionic and mass-selected helium droplets are then guided through a vacuum chamber filled with atomic or molecular vapor where they collide and “pick up” the vapor. The dopants then agglomerate inside the helium droplets around charge centers to singly charged clusters. Evaporation of the helium droplets is induced by collisions in a helium-filled radio frequency (RF)-hexapole, which liberates the cluster ions from the host droplets. The clusters are analyzed with a time-of-flight mass spectrometer. It is demonstrated that using this sequence, the size distribution of the dopant cluster ions is distinctly narrower compared to ionization after pickup. Likewise, the ion cluster beam is more intense. The mass spectra show, as well, that ion clusters of the dopants can be produced with only few helium atoms attached, which will be important for messenger spectroscopy. All these findings are important for the scientific research of clusters and nanoscale materials in general.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1063/1.5133112
- https://aip.scitation.org/doi/pdf/10.1063/1.5133112
- OA Status
- bronze
- Cited By
- 49
- References
- 110
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3012448047
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3012448047Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1063/1.5133112Digital Object Identifier
- Title
-
An intense source for cold cluster ions of a specific compositionWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2020Year of publication
- Publication date
-
2020-03-01Full publication date if available
- Authors
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Lukas Tiefenthaler, João Ameixa, Paul Martini, Simon Albertini, Lorenz Ballauf, M. Zankl, Marcelo Goulart, Felix Laimer, K. von Haeften, Fábio Zappa, P. ScheierList of authors in order
- Landing page
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https://doi.org/10.1063/1.5133112Publisher landing page
- PDF URL
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https://aip.scitation.org/doi/pdf/10.1063/1.5133112Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
bronzeOpen access status per OpenAlex
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https://aip.scitation.org/doi/pdf/10.1063/1.5133112Direct OA link when available
- Concepts
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Helium, Materials science, Atomic physics, Ionization, Ion, Mass spectrum, Mass spectrometry, Electron ionization, Cluster (spacecraft), Dopant, Evaporation, Ion source, Chemistry, Doping, Physics, Optoelectronics, Programming language, Chromatography, Organic chemistry, Computer science, ThermodynamicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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49Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 8, 2023: 7, 2022: 11, 2021: 13Per-year citation counts (last 5 years)
- References (count)
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110Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.frequency | 133 |
| abstract_inverted_index.important | 208, 216 |
| abstract_inverted_index.liberates | 136 |
| abstract_inverted_index.materials | 4, 225 |
| abstract_inverted_index.messenger | 210 |
| abstract_inverted_index.molecular | 37, 95 |
| abstract_inverted_index.nanoscale | 3, 224 |
| abstract_inverted_index.sequence, | 159 |
| abstract_inverted_index.sequence. | 47 |
| abstract_inverted_index.subjected | 73 |
| abstract_inverted_index.addressed. | 13 |
| abstract_inverted_index.collisions | 33, 128 |
| abstract_inverted_index.distinctly | 169 |
| abstract_inverted_index.filtering, | 32 |
| abstract_inverted_index.ionization | 173 |
| abstract_inverted_index.scientific | 219 |
| abstract_inverted_index.ultra-high | 6 |
| abstract_inverted_index.Evaporation | 120 |
| abstract_inverted_index.agglomerate | 108 |
| abstract_inverted_index.bombardment | 71 |
| abstract_inverted_index.combination | 28 |
| abstract_inverted_index.extraction, | 41 |
| abstract_inverted_index.ionization, | 30 |
| abstract_inverted_index.demonstrated | 155 |
| abstract_inverted_index.distribution | 11, 162 |
| abstract_inverted_index.nanodroplets | 25 |
| abstract_inverted_index.electrostatic | 40 |
| abstract_inverted_index.helium-filled | 131 |
| abstract_inverted_index.mass-selected | 81 |
| abstract_inverted_index.spectrometer. | 152 |
| abstract_inverted_index.spectroscopy. | 211 |
| abstract_inverted_index.(RF)-hexapole, | 134 |
| abstract_inverted_index.time-of-flight | 150 |
| cited_by_percentile_year.max | 99 |
| cited_by_percentile_year.min | 90 |
| corresponding_author_ids | https://openalex.org/A5054915258 |
| countries_distinct_count | 3 |
| institutions_distinct_count | 11 |
| corresponding_institution_ids | https://openalex.org/I190249584 |
| citation_normalized_percentile.value | 0.96661687 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |