Anomalous Kinetics of Diffusion-Controlled Defect Annealing in Irradiated Ionic Solids Article Swipe

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E. A. Kotomin , V. N. Kuzovkov , Anatoli I. Popov , Joachim Maier , R. Vila ·

YOU? · · 2017 · Open Access · · DOI: https://doi.org/10.1021/acs.jpca.7b10141

The annealing kinetics of the primary electronic F-type color centers (oxygen vacancies with trapped one or two electrons) is analyzed for three ionic materials (Al₂O₃, MgO, and MgF₂) exposed to intensive irradiation by electrons, neutrons, and heavy swift ions. Phenomenological theory of diffusion-controlled recombination of the F-type centers with much more mobile interstitial ions (complementary hole centers) allows us to extract from experimental data the migration energy of interstitials and pre-exponential factor of diffusion. The obtained migration energies are compared with available first-principles calculations. It is demonstrated that with the increase of radiation fluence both the migration energy and pre-exponent are decreasing in all three materials, irrespective of the type of irradiation. Their correlation satisfies the Meyer-Neldel rule observed earlier in glasses, liquids, and disordered materials.The origin of this effect is discussed. This study demonstrates that in the quantitative analysis of the radiation damage of real materials the dependence of the defect migration parameters on the radiation fluence plays an important role and cannot be neglected.

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Crystallographic Defect

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Irradiation Annealing (glass) Fluence Materials science Ion Ionic bonding Electron Diffusion Radiation damage Kinetics Chemical physics Radiation Crystallographic defect Atomic physics Molecular physics Thermodynamics Crystallography Chemistry Nuclear physics Physics Composite material Organic chemistry Quantum mechanics

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Type: article
Language: en
Landing Page: https://doi.org/10.1021/acs.jpca.7b10141
OA Status: green
Cited By: 53
References: 52
Related Works: 10
OpenAlex ID: https://openalex.org/W2771901917

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DOI: https://doi.org/10.1021/acs.jpca.7b10141

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Title: Anomalous Kinetics of Diffusion-Controlled Defect Annealing in Irradiated Ionic Solids

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Language: en

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Publication year: 2017

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Publication date: 2017-12-12

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Authors: E. A. Kotomin, V. N. Kuzovkov, Anatoli I. Popov, Joachim Maier, R. Vila

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Landing page: https://doi.org/10.1021/acs.jpca.7b10141

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Concepts: Irradiation, Annealing (glass), Fluence, Materials science, Ion, Ionic bonding, Electron, Diffusion, Radiation damage, Kinetics, Chemical physics, Radiation, Crystallographic defect, Atomic physics, Molecular physics, Thermodynamics, Crystallography, Chemistry, Nuclear physics, Physics, Composite material, Organic chemistry, Quantum mechanics

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Cited by: 53

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