Argon and Other Defects in Amorphous SiO2 Coatings for Gravitational-Wave Detectors Article Swipe
A. Paolone
,
E. Placidi
,
Elena Stellino
,
Maria Grazia Betti
,
E. Majorana
,
Carlo Mariani
,
A. Nucara
,
Oriele Palumbo
,
P. Postorino
,
Marco Sbroscia
,
F. Trequattrini
,
M. Granata
,
D. Hofman
,
C. Michel
,
Laurent Pinard
,
Anaël Lemaı̂tre
,
N. S. Shcheblanov
,
G. Cagnoli
,
F. Ricci
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/coatings12071001
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/coatings12071001
Amorphous SiO2 thin films are one of the two components of the highly reflective mirror coatings of gravitational-wave detectors. For this study, layers of amorphous SiO2 on crystalline Si substrates were produced by ion-beam sputtering (IBS), using accelerated neutralized argon ions as sputtering particles, as is the case for the actual mirror coatings of gravitational-wave detectors. The aim of this study is to investigate the possible presence of various defects in the materials in order to improve the coating quality. We provide evidence that, due to the synthesis method, about 0.2 wt.% of Ar is present in the coatings, and it can be released by means of thermal treatments, starting around 400 °C. The time and temperature to obtain the total release of Ar increases with the coating thickness; for a thickness of 100 nm, all argon is released below 600 °C, while an isotherm of one hour at 900 °C is necessary for a coating 5 μm thick. Besides the Ar atoms left from the synthesis, other defects, such as Si clusters and silicon dangling bonds, are present in the coatings. The concentration of both of them is strongly reduced by thermal treatments either in vacuum or in air. The overall thickness of the coating is slightly increased after thermal treatments, as witnessed by the change of the period of interference fringes.
Related Topics
Concepts
Materials science
Amorphous solid
Sputtering
Coating
Argon
Dangling bond
Silicon
Amorphous silicon
Thin film
Ion
Optics
Analytical Chemistry (journal)
Composite material
Optoelectronics
Crystalline silicon
Nanotechnology
Crystallography
Chemistry
Atomic physics
Physics
Organic chemistry
Chromatography
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/coatings12071001
- https://www.mdpi.com/2079-6412/12/7/1001/pdf?version=1658726426
- OA Status
- gold
- Cited By
- 16
- References
- 41
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4285733226
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4285733226Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3390/coatings12071001Digital Object Identifier
- Title
-
Argon and Other Defects in Amorphous SiO2 Coatings for Gravitational-Wave DetectorsWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-07-15Full publication date if available
- Authors
-
A. Paolone, E. Placidi, Elena Stellino, Maria Grazia Betti, E. Majorana, Carlo Mariani, A. Nucara, Oriele Palumbo, P. Postorino, Marco Sbroscia, F. Trequattrini, M. Granata, D. Hofman, C. Michel, Laurent Pinard, Anaël Lemaı̂tre, N. S. Shcheblanov, G. Cagnoli, F. RicciList of authors in order
- Landing page
-
https://doi.org/10.3390/coatings12071001Publisher landing page
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-
https://www.mdpi.com/2079-6412/12/7/1001/pdf?version=1658726426Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://www.mdpi.com/2079-6412/12/7/1001/pdf?version=1658726426Direct OA link when available
- Concepts
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Materials science, Amorphous solid, Sputtering, Coating, Argon, Dangling bond, Silicon, Amorphous silicon, Thin film, Ion, Optics, Analytical Chemistry (journal), Composite material, Optoelectronics, Crystalline silicon, Nanotechnology, Crystallography, Chemistry, Atomic physics, Physics, Organic chemistry, ChromatographyTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
16Total citation count in OpenAlex
- Citations by year (recent)
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2025: 6, 2024: 4, 2023: 4, 2022: 2Per-year citation counts (last 5 years)
- References (count)
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41Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.coatings. | 181 |
| abstract_inverted_index.increased | 208 |
| abstract_inverted_index.increases | 124 |
| abstract_inverted_index.materials | 72 |
| abstract_inverted_index.necessary | 152 |
| abstract_inverted_index.synthesis | 87 |
| abstract_inverted_index.thickness | 131, 202 |
| abstract_inverted_index.witnessed | 213 |
| abstract_inverted_index.components | 9 |
| abstract_inverted_index.detectors. | 18, 55 |
| abstract_inverted_index.particles, | 43 |
| abstract_inverted_index.reflective | 13 |
| abstract_inverted_index.sputtering | 34, 42 |
| abstract_inverted_index.substrates | 29 |
| abstract_inverted_index.synthesis, | 166 |
| abstract_inverted_index.thickness; | 128 |
| abstract_inverted_index.treatments | 193 |
| abstract_inverted_index.accelerated | 37 |
| abstract_inverted_index.crystalline | 27 |
| abstract_inverted_index.investigate | 63 |
| abstract_inverted_index.neutralized | 38 |
| abstract_inverted_index.temperature | 116 |
| abstract_inverted_index.treatments, | 108, 211 |
| abstract_inverted_index.interference | 221 |
| abstract_inverted_index.concentration | 183 |
| abstract_inverted_index.gravitational-wave | 17, 54 |
| cited_by_percentile_year.max | 99 |
| cited_by_percentile_year.min | 94 |
| corresponding_author_ids | https://openalex.org/A5082279775 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 19 |
| corresponding_institution_ids | https://openalex.org/I160013858, https://openalex.org/I4210149433 |
| citation_normalized_percentile.value | 0.91372205 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |