Atomic-Scale Observation of Moiré potential in Twisted Hexagonal Boron Nitride Layers by Electron Microscopy Article Swipe
Ryota Mishima
,
Takuro Nagai
,
Hiroyo Segawa
,
Masahiro Ehara
,
Takashi Uchino
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2024-hbbfj-v2
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2024-hbbfj-v2
Moiré superlattices (MSLs) are an emerging class of two-dimensional functional materials whose electronic states can be tuned by the twist angle between two van der Waals layers and/or the relative placement of the layers. The intriguing prop-erties of MSLs are closely correlated to the moiré potential, which is the electrostatic potential induced by interlayer cou-pling. Intensive efforts have been made to understand the nature and distribution of the moiré potential by using various experimental and theoretical techniques. However, the experimental observation of the moiré potential is still challenging because of the possible presence of the surface and/or interlayer contaminants. In this work, we develop a method to obtain hexagonal boron nitride (hBN) nanolayers (with or without twist) using a specially designed chemical exfoliation tech-nique. The resulting hBN nanolayers are atomically clean and strain free, hence providing ideal MSLs for the investigation of their moiré potential. Aberration-corrected high resolution transmission electron microscopy measurements on the twisted hBN nanolayers allow us to observe moiré diffraction spots in Fourier space. Then, the moiré potential is recon-structed by the inverse fast Fourier transform of the moiré diffraction spots. It has been revealed that the local interlayer atomic overlap plays a decisive role in determining the periodicity and distribution of the moiré potential, as supported by density functional theory calculations. This work not only provides a general strategy to observe the moiré potential in MSLs, but it also expands the application of electron microscopy to the further study of MSLs with atomic resolution.
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- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.26434/chemrxiv-2024-hbbfj-v2
- OA Status
- gold
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- 10
- OpenAlex ID
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https://openalex.org/W4407181952Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.26434/chemrxiv-2024-hbbfj-v2Digital Object Identifier
- Title
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Atomic-Scale Observation of Moiré potential in Twisted Hexagonal Boron Nitride Layers by Electron MicroscopyWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
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2025Year of publication
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2025-02-05Full publication date if available
- Authors
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Ryota Mishima, Takuro Nagai, Hiroyo Segawa, Masahiro Ehara, Takashi UchinoList of authors in order
- Landing page
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https://doi.org/10.26434/chemrxiv-2024-hbbfj-v2Publisher landing page
- Open access
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YesWhether a free full text is available
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-
goldOpen access status per OpenAlex
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https://doi.org/10.26434/chemrxiv-2024-hbbfj-v2Direct OA link when available
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Moiré pattern, Atomic units, Hexagonal boron nitride, Electron microscope, Materials science, Boron nitride, Electron, Boron, Hexagonal crystal system, Condensed matter physics, Nanotechnology, Optics, Crystallography, Chemistry, Physics, Graphene, Quantum mechanics, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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| abstract_inverted_index.have | 57 |
| abstract_inverted_index.high | 146 |
| abstract_inverted_index.made | 59 |
| abstract_inverted_index.only | 218 |
| abstract_inverted_index.role | 197 |
| abstract_inverted_index.that | 188 |
| abstract_inverted_index.this | 100 |
| abstract_inverted_index.with | 245 |
| abstract_inverted_index.work | 216 |
| abstract_inverted_index.(hBN) | 111 |
| abstract_inverted_index.(with | 113 |
| abstract_inverted_index.MSLs, | 229 |
| abstract_inverted_index.Then, | 167 |
| abstract_inverted_index.Waals | 25 |
| abstract_inverted_index.allow | 157 |
| abstract_inverted_index.angle | 20 |
| abstract_inverted_index.boron | 109 |
| abstract_inverted_index.class | 6 |
| abstract_inverted_index.clean | 130 |
| abstract_inverted_index.free, | 133 |
| abstract_inverted_index.hence | 134 |
| abstract_inverted_index.ideal | 136 |
| abstract_inverted_index.local | 190 |
| abstract_inverted_index.plays | 194 |
| abstract_inverted_index.spots | 163 |
| abstract_inverted_index.still | 86 |
| abstract_inverted_index.study | 242 |
| abstract_inverted_index.their | 142 |
| abstract_inverted_index.tuned | 16 |
| abstract_inverted_index.twist | 19 |
| abstract_inverted_index.using | 71, 117 |
| abstract_inverted_index.which | 46 |
| abstract_inverted_index.whose | 11 |
| abstract_inverted_index.work, | 101 |
| abstract_inverted_index.(MSLs) | 2 |
| abstract_inverted_index.Moiré | 0 |
| abstract_inverted_index.and/or | 27, 96 |
| abstract_inverted_index.atomic | 192, 246 |
| abstract_inverted_index.layers | 26 |
| abstract_inverted_index.method | 105 |
| abstract_inverted_index.moiré | 44, 68, 83, 143, 161, 169, 181, 206, 226 |
| abstract_inverted_index.nature | 63 |
| abstract_inverted_index.obtain | 107 |
| abstract_inverted_index.space. | 166 |
| abstract_inverted_index.spots. | 183 |
| abstract_inverted_index.states | 13 |
| abstract_inverted_index.strain | 132 |
| abstract_inverted_index.theory | 213 |
| abstract_inverted_index.twist) | 116 |
| abstract_inverted_index.Fourier | 165, 177 |
| abstract_inverted_index.because | 88 |
| abstract_inverted_index.between | 21 |
| abstract_inverted_index.closely | 40 |
| abstract_inverted_index.density | 211 |
| abstract_inverted_index.develop | 103 |
| abstract_inverted_index.efforts | 56 |
| abstract_inverted_index.expands | 233 |
| abstract_inverted_index.further | 241 |
| abstract_inverted_index.general | 221 |
| abstract_inverted_index.induced | 51 |
| abstract_inverted_index.inverse | 175 |
| abstract_inverted_index.layers. | 33 |
| abstract_inverted_index.nitride | 110 |
| abstract_inverted_index.observe | 160, 224 |
| abstract_inverted_index.overlap | 193 |
| abstract_inverted_index.surface | 95 |
| abstract_inverted_index.twisted | 154 |
| abstract_inverted_index.various | 72 |
| abstract_inverted_index.without | 115 |
| abstract_inverted_index.However, | 77 |
| abstract_inverted_index.chemical | 121 |
| abstract_inverted_index.decisive | 196 |
| abstract_inverted_index.designed | 120 |
| abstract_inverted_index.electron | 149, 237 |
| abstract_inverted_index.emerging | 5 |
| abstract_inverted_index.possible | 91 |
| abstract_inverted_index.presence | 92 |
| abstract_inverted_index.provides | 219 |
| abstract_inverted_index.relative | 29 |
| abstract_inverted_index.revealed | 187 |
| abstract_inverted_index.strategy | 222 |
| abstract_inverted_index.Intensive | 55 |
| abstract_inverted_index.hexagonal | 108 |
| abstract_inverted_index.materials | 10 |
| abstract_inverted_index.placement | 30 |
| abstract_inverted_index.potential | 50, 69, 84, 170, 227 |
| abstract_inverted_index.providing | 135 |
| abstract_inverted_index.resulting | 125 |
| abstract_inverted_index.specially | 119 |
| abstract_inverted_index.supported | 209 |
| abstract_inverted_index.transform | 178 |
| abstract_inverted_index.atomically | 129 |
| abstract_inverted_index.correlated | 41 |
| abstract_inverted_index.cou-pling. | 54 |
| abstract_inverted_index.electronic | 12 |
| abstract_inverted_index.functional | 9, 212 |
| abstract_inverted_index.interlayer | 53, 97, 191 |
| abstract_inverted_index.intriguing | 35 |
| abstract_inverted_index.microscopy | 150, 238 |
| abstract_inverted_index.nanolayers | 112, 127, 156 |
| abstract_inverted_index.potential, | 45, 207 |
| abstract_inverted_index.potential. | 144 |
| abstract_inverted_index.resolution | 147 |
| abstract_inverted_index.understand | 61 |
| abstract_inverted_index.application | 235 |
| abstract_inverted_index.challenging | 87 |
| abstract_inverted_index.determining | 199 |
| abstract_inverted_index.diffraction | 162, 182 |
| abstract_inverted_index.exfoliation | 122 |
| abstract_inverted_index.observation | 80 |
| abstract_inverted_index.periodicity | 201 |
| abstract_inverted_index.prop-erties | 36 |
| abstract_inverted_index.resolution. | 247 |
| abstract_inverted_index.tech-nique. | 123 |
| abstract_inverted_index.techniques. | 76 |
| abstract_inverted_index.theoretical | 75 |
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| abstract_inverted_index.experimental | 73, 79 |
| abstract_inverted_index.measurements | 151 |
| abstract_inverted_index.transmission | 148 |
| abstract_inverted_index.calculations. | 214 |
| abstract_inverted_index.contaminants. | 98 |
| abstract_inverted_index.electrostatic | 49 |
| abstract_inverted_index.investigation | 140 |
| abstract_inverted_index.superlattices | 1 |
| abstract_inverted_index.recon-structed | 172 |
| abstract_inverted_index.two-dimensional | 8 |
| abstract_inverted_index.Aberration-corrected | 145 |
| cited_by_percentile_year | |
| countries_distinct_count | 1 |
| institutions_distinct_count | 5 |
| citation_normalized_percentile.value | 0.03296835 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |