Atoms to fibers: Identifying novel processing methods in the synthesis of pitch-based carbon fibers Article Swipe
Asmita Jana
,
Taishan Zhu
,
Yanming Wang
,
Jeramie J. Adams
,
Logan T. Kearney
,
Amit K. Naskar
,
Jeffrey C. Grossman
,
Nicola Ferralis
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1126/sciadv.abn1905
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1126/sciadv.abn1905
Understanding and optimizing the key mechanisms used in the synthesis of pitch-based carbon fibers (CFs) are challenging, because unlike polyacrylonitrile-based CFs, the feedstock for pitch-based CFs is chemically heterogeneous, resulting in complex fabrication leading to inconsistency in the final properties. In this work, we use molecular dynamics simulations to explore the processing and chemical phase space through a framework of CF models to identify their effects on elastic performance. The results are in excellent agreement with experiments. We find that density, followed by alignment, and functionality of the molecular constituents dictate the CF mechanical properties more strongly than their size and shape. Last, we propose a previously unexplored fabrication route for high-modulus CFs. Unlike graphitization, this results in increased sp 3 fraction, achieved via generating high-density CFs. In addition, the high sp 3 fraction leads to the fabrication of CFs with isometric compressive and tensile moduli, enabling their potential applications for compressive loading.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1126/sciadv.abn1905
- OA Status
- gold
- Cited By
- 26
- References
- 54
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4220811386
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4220811386Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1126/sciadv.abn1905Digital Object Identifier
- Title
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Atoms to fibers: Identifying novel processing methods in the synthesis of pitch-based carbon fibersWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-03-18Full publication date if available
- Authors
-
Asmita Jana, Taishan Zhu, Yanming Wang, Jeramie J. Adams, Logan T. Kearney, Amit K. Naskar, Jeffrey C. Grossman, Nicola FerralisList of authors in order
- Landing page
-
https://doi.org/10.1126/sciadv.abn1905Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1126/sciadv.abn1905Direct OA link when available
- Concepts
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Carbon fibers, Computer science, Materials science, Nanotechnology, Composite material, Composite numberTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
26Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 9, 2024: 5, 2023: 10, 2022: 2Per-year citation counts (last 5 years)
- References (count)
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54Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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