Basic magnesium sulfate@TiO2 composite for efficient adsorption and photocatalytic degradation of 4-dodecylmorpholine in brine Article Swipe
Zhongmei Song
,
Huifang Zhang
,
Liang Ma
,
Miao Lu
,
Chengyou Wu
,
Qingqing Liu
,
Xue‐Feng Yu
,
Haining Liu
,
Xiushen Ye
,
Zhen Ma
,
Zhijian Wu
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41598-024-59921-8
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41598-024-59921-8
More than 70% of the potash fertilizer globally is produced by the froth flotation process, in which 4-dodecylmorpholine (DMP) serves as a reverse flotation agent. As the potash fertilizer production rapidly rises, the increased DMP levels in discharged brine pose a threat to the production of high-value chemicals. In this paper, composite particles of basic magnesium sulfate@TiO 2 (BMS@TiO 2 ) were prepared using a simple and mild loading method. These particles were utilized for the adsorption and photocatalytic degradation of DMP in brine. Compared with normal powdered materials, the granular BMS@TiO 2 in this study can be easily separated from liquid, and the degradation intermediates will not enter the brine without causing secondary pollution. BMS@TiO 2 consists of 5·1·7 phase (5Mg(OH) 2 ·MgSO 4 ·7H 2 O) whisker clusters embedding 2.3% TiO 2 . The adsorption equilibrium of DMP on BMS@TiO 2 particles was achieved through hydrogen bonding and pore interception with the adsorption capacity of approximately 5 mg g −1 after 6 h. The photodegradation efficiency of DMP adsorbed on BMS@TiO 2 reached about 92% within 16 h, which is compared with that of pure TiO 2 nanoparticles. Additionally, excellent stability and recyclability of BMS@TiO 2 were also observed in five cycle tests of adsorption and photocatalytic degradation of DMP, and the possible photocatalytic degradation pathways and mechanism of DMP are proposed following molecular electrostatic potential analysis. This work provides a sustainable and environmentally friendly approach for eliminating organic micropollutants from water environments.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41598-024-59921-8
- https://www.nature.com/articles/s41598-024-59921-8.pdf
- OA Status
- gold
- Cited By
- 7
- References
- 73
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4395038818
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4395038818Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41598-024-59921-8Digital Object Identifier
- Title
-
Basic magnesium sulfate@TiO2 composite for efficient adsorption and photocatalytic degradation of 4-dodecylmorpholine in brineWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-04-23Full publication date if available
- Authors
-
Zhongmei Song, Huifang Zhang, Liang Ma, Miao Lu, Chengyou Wu, Qingqing Liu, Xue‐Feng Yu, Haining Liu, Xiushen Ye, Zhen Ma, Zhijian WuList of authors in order
- Landing page
-
https://doi.org/10.1038/s41598-024-59921-8Publisher landing page
- PDF URL
-
https://www.nature.com/articles/s41598-024-59921-8.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://www.nature.com/articles/s41598-024-59921-8.pdfDirect OA link when available
- Concepts
-
Photocatalysis, Adsorption, Brine, Chemical engineering, Magnesium, Potash, Materials science, Chemistry, Fertilizer, Inorganic chemistry, Nuclear chemistry, Catalysis, Organic chemistry, Metallurgy, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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7Total citation count in OpenAlex
- Citations by year (recent)
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2025: 5, 2024: 2Per-year citation counts (last 5 years)
- References (count)
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73Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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