Bi/CeO2–Decorated CuS Electrocatalysts for CO2-to-Formate Conversion Article Swipe
Qi Wang
,
Tianshuang Bao
,
Xiangchuan Zhao
,
Yue Cao
,
Jun Cao
,
Qiaoling Li
,
Weimeng Si
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/molecules29132948
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/molecules29132948
The electrocatalytic carbon dioxide (CO2) reduction reaction (CO2RR) is extensively regarded as a promising strategy to reach carbon neutralization. Copper sulfide (CuS) has been widely studied for its ability to produce C1 products with high selectivity. However, challenges still remain owing to the poor selectivity of formate. Here, a Bi/CeO2/CuS composite was synthesized using a simple solvothermal method. Bi/CeO2–decorated CuS possessed high formate selectivity, with the Faraday efficiency and current density reaching 88% and 17 mA cm−2, respectively, in an H-cell. The Bi/CeO2/CuS structure significantly reduces the energy barrier formed by OCHO*, resulting in the high activity and selectivity of the CO2 conversion to formate. Ce4+ readily undergoes reduction to Ce3+, allowing the formation of a conductive network of Ce4+/Ce3+. This network facilitates electron transfer, stabilizes the Cu+ species, and enhances the adsorption and activation of CO2. Furthermore, sulfur catalyzes the OCHO* transformation to formate. This work describes a highly efficient catalyst for CO2 to formate, which will aid in catalyst design for CO2RR to target products.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/molecules29132948
- https://www.mdpi.com/1420-3049/29/13/2948/pdf?version=1718951578
- OA Status
- gold
- Cited By
- 7
- References
- 63
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4399906538
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4399906538Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/molecules29132948Digital Object Identifier
- Title
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Bi/CeO2–Decorated CuS Electrocatalysts for CO2-to-Formate ConversionWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-06-21Full publication date if available
- Authors
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Qi Wang, Tianshuang Bao, Xiangchuan Zhao, Yue Cao, Jun Cao, Qiaoling Li, Weimeng SiList of authors in order
- Landing page
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https://doi.org/10.3390/molecules29132948Publisher landing page
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https://www.mdpi.com/1420-3049/29/13/2948/pdf?version=1718951578Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/1420-3049/29/13/2948/pdf?version=1718951578Direct OA link when available
- Concepts
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Formate, Materials science, Nanotechnology, Chemistry, Chemical engineering, Catalysis, Biochemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
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7Total citation count in OpenAlex
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2025: 4, 2024: 3Per-year citation counts (last 5 years)
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63Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| display_name | Bi/CeO2–Decorated CuS Electrocatalysts for CO2-to-Formate Conversion |
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| primary_topic.display_name | CO2 Reduction Techniques and Catalysts |
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