Biobased biodegradable chelating agents enhance coupled ex situ and in situ carbon dioxide mineralization via peridotite dissolution and wormholing Article Swipe
Luis Salalá
,
Noriaki Watanabe
,
Jiajie Wang
,
Atsushi Okamoto
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s43247-025-02687-2
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s43247-025-02687-2
Mantle peridotite, which is also present in near-surface environments, reacts readily with CO 2 , and is expected to be suitable for CO 2 mineralization. However, the low permeability and porosity of mantle peridotite, in addition to its volume changes during carbonation remain major obstacles to large-scale CO 2 mineralization. Here we propose a coupled ex-situ and in-situ CO 2 mineralization approach employing biobased and biodegradable chelating agents. This involves the injection of an acidic chelating agent to enhance the permeability and porosity, along with divalent metal ion extraction to achieve ex-situ CO 2 mineralization on the surface (stage 1). Subsequently, an alkaline chelating agent is employed for CO 2 capture, injection, and enhanced in-situ mineralization (stage 2). This study experimentally demonstrated a substantial permeability enhancement and Mg-Fe cation extraction by chelating agents, a crucial process of stage 1. The injection of acidic chelating agents leads to the formation of prominent wormholes, resulting in a 21-fold increase in permeability within ~20 minutes, indicating the potential to enhance the injectivity and CO 2 mineralization capacity of peridotite.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s43247-025-02687-2
- https://www.nature.com/articles/s43247-025-02687-2.pdf
- OA Status
- gold
- References
- 46
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4413375369
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4413375369Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s43247-025-02687-2Digital Object Identifier
- Title
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Biobased biodegradable chelating agents enhance coupled ex situ and in situ carbon dioxide mineralization via peridotite dissolution and wormholingWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-08-21Full publication date if available
- Authors
-
Luis Salalá, Noriaki Watanabe, Jiajie Wang, Atsushi OkamotoList of authors in order
- Landing page
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https://doi.org/10.1038/s43247-025-02687-2Publisher landing page
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https://www.nature.com/articles/s43247-025-02687-2.pdfDirect link to full text PDF
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YesWhether a free full text is available
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-
goldOpen access status per OpenAlex
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https://www.nature.com/articles/s43247-025-02687-2.pdfDirect OA link when available
- Concepts
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In situ, Dissolution, Mineralization (soil science), Carbon dioxide, Peridotite, Chemistry, Environmental chemistry, Chemical engineering, Environmental science, Geology, Geochemistry, Organic chemistry, Mantle (geology), Engineering, NitrogenTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- References (count)
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46Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W4404458360, https://openalex.org/W2104032373, https://openalex.org/W2984659082, https://openalex.org/W3021957865, https://openalex.org/W2079086890, https://openalex.org/W4380985492, https://openalex.org/W3187664582, https://openalex.org/W2102735659, https://openalex.org/W4399617995, https://openalex.org/W2915799898, https://openalex.org/W2931585576, https://openalex.org/W1979590077, https://openalex.org/W2090157006, https://openalex.org/W3208704500, https://openalex.org/W2797696457, https://openalex.org/W2585847218, https://openalex.org/W3122723814, https://openalex.org/W4307721373, https://openalex.org/W4390492030, https://openalex.org/W2557032280, https://openalex.org/W3156071636, https://openalex.org/W2615393618, https://openalex.org/W4389720646, https://openalex.org/W3201798539, https://openalex.org/W4313654801, https://openalex.org/W4307124411, https://openalex.org/W4391915944, https://openalex.org/W1985574842, https://openalex.org/W2895951831, https://openalex.org/W4404400094, https://openalex.org/W4392095103, https://openalex.org/W3177798130, https://openalex.org/W755437216, https://openalex.org/W2176493563, https://openalex.org/W4407780515, https://openalex.org/W2055414831, https://openalex.org/W1996969213, https://openalex.org/W2609382449, https://openalex.org/W1837526995, https://openalex.org/W2510414820, https://openalex.org/W2814459026, https://openalex.org/W2068328429, https://openalex.org/W2975634117, https://openalex.org/W4211056572, https://openalex.org/W2766716302, https://openalex.org/W2080131712 |
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