Biomimetic nacre-like aramid nanofiber-holey MXene composites for lithium-sulfur batteries Article Swipe
Yuying Wang
,
Volkan Çeçen
,
Shoupeng Wang
,
Lei Zhao
,
Li Liu
,
Xiaonan Zhu
,
Yudong Huang
,
Mingqiang Wang
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1016/j.xcrp.2023.101592
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1016/j.xcrp.2023.101592
Polysulfide shuttle and lithium dendrite formation limit practical applications of lithium-sulfur (Li-S) batteries. To address these issues, we propose a nacre-inspired design of MXene/aramid nanofiber (ANF) separator with “brick-and-mortar” microstructure. The combination of shortened ion transfer distance generated by holes on MXene and enlarged interlayer spacing provided by ANFs creates a hierarchical ion path “highway” that modulates the efficiency of ion transportation while synergistically suppressing the polysulfide shuttles. Furthermore, benefitting from the introduction of ANF, the composite membrane has good mechanical properties and impact tolerance. With simultaneous mitigation of dendrite growth and polysulfide poisoning of anodes, the cells with nacre-inspired separator exhibited excellent rate capability to 5 C and had a possible long cycle life of 3,500+ cycles with capacity decay of 0.013% per cycle to 3 C. This work offers a membrane design strategy inspired by the structure of pearl layers, aiming to resolve materials performance challenges of high-performance energy storage. © 2023 The Authors
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.xcrp.2023.101592
- https://ars.els-cdn.com/content/image/1-s2.0-S2666386423004009-fx1_lrg.jpg
- OA Status
- gold
- Cited By
- 10
- References
- 49
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4386969565
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4386969565Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.xcrp.2023.101592Digital Object Identifier
- Title
-
Biomimetic nacre-like aramid nanofiber-holey MXene composites for lithium-sulfur batteriesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-09-22Full publication date if available
- Authors
-
Yuying Wang, Volkan Çeçen, Shoupeng Wang, Lei Zhao, Li Liu, Xiaonan Zhu, Yudong Huang, Mingqiang WangList of authors in order
- Landing page
-
https://doi.org/10.1016/j.xcrp.2023.101592Publisher landing page
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https://ars.els-cdn.com/content/image/1-s2.0-S2666386423004009-fx1_lrg.jpgDirect link to full text PDF
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://ars.els-cdn.com/content/image/1-s2.0-S2666386423004009-fx1_lrg.jpgDirect OA link when available
- Concepts
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Polysulfide, Materials science, Nanofiber, Separator (oil production), Aramid, Composite material, Anode, Microstructure, Composite number, Nanotechnology, Fiber, Electrolyte, Chemistry, Electrode, Thermodynamics, Physics, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
10Total citation count in OpenAlex
- Citations by year (recent)
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2025: 4, 2024: 6Per-year citation counts (last 5 years)
- References (count)
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49Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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