Bringing weak transitions to light Article Swipe
YOU?
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· 2025
· Open Access
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· DOI: https://doi.org/10.1038/s41467-025-60701-9
Weak transitions between quantum states are of fundamental importance for a broad range of phenomena from analytical biochemistry to precision physics, but generally challenge experimental detection. Due to their small cross sections scaling with the absolute square of their transition matrix elements, spectroscopic measurements often fail in particular in the presence of competing background processes. Here we introduce a general concept to break this scaling law and enhance the transition probability by exploiting a stronger laser-coupled pathway to the same excited state. We demonstrate the concept experimentally by attosecond transient absorption spectroscopy in helium atoms. The quasi-forbidden transitions from the ground state 1 s 2 to the weakly coupled doubly excited 2 p 3 d and s p 2,4− states are boosted by an order of magnitude. Enhancing single-photon-suppressed transitions can find widespread applicability, from spectral diagnostics of complex molecules in life and chemical sciences to precision spectroscopy of weak transitions in metastable atomic nuclei in the search for new physics.
Related Topics
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-025-60701-9
- https://www.nature.com/articles/s41467-025-60701-9.pdf
- OA Status
- gold
- References
- 38
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4411497317
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4411497317Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41467-025-60701-9Digital Object Identifier
- Title
-
Bringing weak transitions to lightWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
-
2025-06-20Full publication date if available
- Authors
-
Yu He, Xiao‐Min Tong, Shuyuan Hu, Gergana D. Borisova, Hao Liang, Maximilian Hartmann, Veit Stooß, Chunhai Lyu, Zoltán Harman, Christoph H. Keitel, Kenneth J. Schäfer, Mette B. Gaarde, Christian Ott, Thomas PfeiferList of authors in order
- Landing page
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https://doi.org/10.1038/s41467-025-60701-9Publisher landing page
- PDF URL
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https://www.nature.com/articles/s41467-025-60701-9.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41467-025-60701-9.pdfDirect OA link when available
- Concepts
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Metastability, Excited state, Spectroscopy, Physics, Scaling, Ground state, Atomic physics, Optical physics, Photon, Attosecond, Laser, Quantum mechanics, Plasma, Ultrashort pulse, Geometry, MathematicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- References (count)
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38Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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