Catalytic effect of a novel MgC0.5Co3 compound on the dehydrogenation of MgH2 Article Swipe
Yaokun Fu
,
Zhenmin Ding
,
Lu Zhang
,
Hongming Zhang
,
Wenfeng Wang
,
Yuan Li
,
Shumin Han
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1016/j.pnsc.2021.01.009
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1016/j.pnsc.2021.01.009
The application of magnesium hydride (MgH2) is limited due to the high reaction temperature and slow kinetics during dehydrogenation. In order to ameliorate the dehydrogenation property of MgH2, MgC0.5Co3 compound with induction and catalytic effects was introduced into the Mg/MgH2 system via ball-milling and hydriding combustion methods in present study. Compared to the pure MgH2, the initial hydrogen desorption temperature of MgH2–MgC0.5Co3 composite lowered to 237 °C, decreasing by 141 °C. At 325 °C the MgH2–MgC0.5Co3 composite could release 4.38 wt% H2 within 60 min, which is 4.5 times the capacity of hydrogen released by as milled-MgH2. Besides, the hydrogen desorption activation energy of the MgH2–MgC0.5Co3 composite was dramatically reduced to 126.7 ± 1.4 kJ/mol. It was observed that MgC0.5Co3 was chemically stable and no chemical transformation occurred after cycling, which not only inhibited the nucleation and growth of composite particles, but also had a positive effect on the hydrogen desorption reaction of MgH2 due to its catalytic effect. This study may provide references for designing and synthesizing Mg–C–Co alloy compound for the Mg-based hydrogen storage area.
Related Topics
Concepts
Dehydrogenation
Magnesium hydride
Hydrogen storage
Catalysis
Composite number
Desorption
Nucleation
Hydrogen
Materials science
Activation energy
Chemical engineering
Magnesium
Inorganic chemistry
Chemistry
Alloy
Metallurgy
Physical chemistry
Composite material
Organic chemistry
Adsorption
Engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.pnsc.2021.01.009
- OA Status
- hybrid
- Cited By
- 18
- References
- 46
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3134082821
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W3134082821Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.pnsc.2021.01.009Digital Object Identifier
- Title
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Catalytic effect of a novel MgC0.5Co3 compound on the dehydrogenation of MgH2Work title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-03-09Full publication date if available
- Authors
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Yaokun Fu, Zhenmin Ding, Lu Zhang, Hongming Zhang, Wenfeng Wang, Yuan Li, Shumin HanList of authors in order
- Landing page
-
https://doi.org/10.1016/j.pnsc.2021.01.009Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://doi.org/10.1016/j.pnsc.2021.01.009Direct OA link when available
- Concepts
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Dehydrogenation, Magnesium hydride, Hydrogen storage, Catalysis, Composite number, Desorption, Nucleation, Hydrogen, Materials science, Activation energy, Chemical engineering, Magnesium, Inorganic chemistry, Chemistry, Alloy, Metallurgy, Physical chemistry, Composite material, Organic chemistry, Adsorption, EngineeringTop concepts (fields/topics) attached by OpenAlex
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18Total citation count in OpenAlex
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2024: 2, 2023: 4, 2022: 6, 2021: 6Per-year citation counts (last 5 years)
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46Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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