Cation controlled rotation in anionic pillar[5]arenes and its application for fluorescence switch Article Swipe
Hao Zheng
,
Lulu Fu
,
Ranran Wang
,
Jianmin Jiao
,
Yingying Song
,
Conghao Shi
,
Yuan Chen
,
Juli Jiang
,
Lin Chen
,
Jing Ma
,
Leyong Wang
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-023-36131-w
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-023-36131-w
Controlling molecular motion is one of hot topics in the field of chemistry. Molecular rotors have wide applications in building nanomachines and functional materials, due to their controllable rotations. Hence, the development of novel rotor systems, controlled by external stimuli, is desirable. Pillar[n]arenes, a class of macrocycles, have a unique planar chirality, in which two stable conformational isomers p R and p S would interconvert by oxygen-through-the-annulus rotations of their hydroquinone rings. We observe the differential kinetic traits of planar chirality transformation in sodium carboxylate pillar[5]arene ( WP5-Na ) and ammonium carboxylate pillar[5]arene ( WP5-NH 4 ), which inspire us to construct a promising rotary platform in anionic pillar[5]arenes ( WP5 ) skeletons. Herein, we demonstrate the non-negligible effect of counter cations on rotational barriers of hydroquinone rings in WP5 , which enables a cation grease/brake rotor system. Applications of this tunable rotor system as fluorescence switch and anti-counterfeiting ink are further explored.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-023-36131-w
- https://www.nature.com/articles/s41467-023-36131-w.pdf
- OA Status
- gold
- Cited By
- 44
- References
- 58
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4319079959
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4319079959Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41467-023-36131-wDigital Object Identifier
- Title
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Cation controlled rotation in anionic pillar[5]arenes and its application for fluorescence switchWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-02-03Full publication date if available
- Authors
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Hao Zheng, Lulu Fu, Ranran Wang, Jianmin Jiao, Yingying Song, Conghao Shi, Yuan Chen, Juli Jiang, Lin Chen, Jing Ma, Leyong WangList of authors in order
- Landing page
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https://doi.org/10.1038/s41467-023-36131-wPublisher landing page
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https://www.nature.com/articles/s41467-023-36131-w.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41467-023-36131-w.pdfDirect OA link when available
- Concepts
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Pillar, Fluorescence, Rotation (mathematics), Nanotechnology, Materials science, Chemistry, Computer science, Physics, Optics, Mechanical engineering, Engineering, Artificial intelligenceTop concepts (fields/topics) attached by OpenAlex
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44Total citation count in OpenAlex
- Citations by year (recent)
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2025: 10, 2024: 22, 2023: 12Per-year citation counts (last 5 years)
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58Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.Controlling | 1 |
| abstract_inverted_index.carboxylate | 85, 92 |
| abstract_inverted_index.demonstrate | 116 |
| abstract_inverted_index.development | 32 |
| abstract_inverted_index.Applications | 139 |
| abstract_inverted_index.applications | 18 |
| abstract_inverted_index.controllable | 28 |
| abstract_inverted_index.differential | 76 |
| abstract_inverted_index.fluorescence | 146 |
| abstract_inverted_index.grease/brake | 136 |
| abstract_inverted_index.hydroquinone | 71, 127 |
| abstract_inverted_index.interconvert | 65 |
| abstract_inverted_index.macrocycles, | 47 |
| abstract_inverted_index.nanomachines | 21 |
| abstract_inverted_index.conformational | 57 |
| abstract_inverted_index.non-negligible | 118 |
| abstract_inverted_index.pillar[5]arene | 86, 93 |
| abstract_inverted_index.transformation | 82 |
| abstract_inverted_index.pillar[5]arenes | 109 |
| abstract_inverted_index.Pillar[n]arenes, | 43 |
| abstract_inverted_index.anti-counterfeiting | 149 |
| abstract_inverted_index.oxygen-through-the-annulus | 67 |
| cited_by_percentile_year.max | 100 |
| cited_by_percentile_year.min | 99 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 11 |
| citation_normalized_percentile.value | 0.98273859 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |