Charge carrier dynamics and self-trapping on Sb2S3(100) Article Swipe
Lisa Grad
,
Fabian O. von Rohr
,
Matthias Hengsberger
,
Jürg Osterwalder
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.5281/zenodo.6840656
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.5281/zenodo.6840656
Full data set for publication: Published Manuscript: Lisa Grad, Fabian O. von Rohr, Matthias Hengsberger, Jürg Osterwalder Charge carrier dynamics and self-trapping on Sb2S3(100) Physical Review Materials 5, 075401 (2021) DOI: 10.1103/PhysRevMaterials.5.075401 *** Data format *** Photoemission data: Time-resolved photoemission Data were acquired using home-built Labview-based software package as function of emission angle and time delay. The detector images were saved in the Specs GmbH proprietary SpecsLab data format which was loaded, scaled and saved as text file using the software Wavemetrics Igor Pro (version 7) and Igor Pro macro packages provided by Specs GmbH. No further processing like intensity scaling, binning or similar was applied to the data. Static photoemission data were acquired using the SpecsLab Prodigy software provided by Specs GmbH, Berlin, Germany. The data were processed for image distortions by the measurement software and saved as text files (extension .xy) including full header information: two columns Energy, Intensity *** Experimental parameters and reference data *** Specs Phoibos 100 spectrometer and a manipulator with home-built goniometer. The energy settings includes the work function of the electron detector, i.e. the photoelectrons from the Fermi energy appear at a kinetic energy value which equals the photon energy minus the (optional) sample bias voltage. In present measurements (raw data): WF of analyzer: Reference data set from polycrystalline metal using 21.22 eV photons and bias -5 V "Measurement_EF.txt" (text file with header information) Fitting: EF at 26.24 eV Pre-defined analyser WF 4.408 eV Light Sources - He-Ia line (photon energy 21.22 eV, Omicron HIS-13 source, not monochromated, unpolarised) - High-harmonic (HH5) of the second harmonic at 414 nm, wavelength 82 nm, photon energy 15.3 eV - Pump-probe (time-resolved) data taken using the second harmonic (414 nm) of the femtosecond laser as pump and the fourth harmonic (207 nm) as probe pulse. Samples were crystals of Sb2S3, cleaved in ultra-high vacuum Sample temperature was room temperature (290 K) *********************** Fig. 2 Valence Band in normal emission ********************* Static data taken using the HHG light source, i.e. photon energy 15.3 eV 140 deg refers to the manipulator angle setting for normal emission Sample bias -5 V - Fermi energy at 20.3 eV "Spec_Gamma_140deg.txt" full data set, energy from 8.0 eV in steps of 0.05 eV "VBM_Gamma_140deg.txt" zoom on valence band maximum, energy from 13.0 eV in steps of +0.05 eV Raw data as measured with SpecsLab Prodigy: "VB_1.xy" ****** Fig. 3 Time-resolved photoemission spectra including "vertical cuts" above the Fermi energy, i.e. energy distribution curves ********** Photoemission data taken at +0.3 - 3 eV with respect to the Fermi energy of the sample Raw Data set #1855, detector settings: kinetic energy 12.5 eV (center energy) pass energy 15.0 eV sample bias -5 V with respect to ground delays at non equidistant steps between -2 ps and +40 ps with respect to delay zero (coincidence of pump and probe pulses) Raw Data as .ZIP file: "1855 Sb2S3.zip" List of delays: Delays_DataSet1855.txt Raw data: "1855 Sb2S3" Series of detector images for one delay after 80 scans as text files ".tsv" Name is position of delay stage in mm; the temporal coincidence between pump and probe is -7.33 mm ("delay zero") "Info.tsv" contains measured time delays Raw data, preprocessed by cropping and scaling: 3D data cube intensity as function of detector angle (x), energy (y), time delay (z) Data: "Data_1855N80.txt" The different energy, angle, delay settings are given in the following text files: x (196 rows): detector angle (degrees, center=normal emission) "AngleScale_deg_Rows.txt" y (301 columns): energy (eV) "EnergyScale_eV_Cols.txt" z (231 layers): time delays (fs) "TimeDelays_fs_Layers.txt"
Related Topics
Concepts
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://zenodo.org/record/6840656
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- green
- Cited By
- 2
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- 10
- OpenAlex ID
- https://openalex.org/W4285517629
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4285517629Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.5281/zenodo.6840656Digital Object Identifier
- Title
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Charge carrier dynamics and self-trapping on Sb2S3(100)Work title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-07-08Full publication date if available
- Authors
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Lisa Grad, Fabian O. von Rohr, Matthias Hengsberger, Jürg OsterwalderList of authors in order
- Landing page
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https://zenodo.org/record/6840656Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
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https://zenodo.org/record/6840656Direct OA link when available
- Concepts
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Trapping, Charge (physics), Charge carrier, Chemical physics, Dynamics (music), Materials science, Physics, Optoelectronics, Quantum mechanics, Geography, Forestry, AcousticsTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2024: 1, 2021: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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