CNT/PVDF Composite Coating Layer on Cu with a Synergy of Uniform Current Distribution and Stress Releasing for Improving Reversible Li Plating/Stripping Article Swipe
Qiang Guo
,
Yanan Yu
,
Shengjie Xia
,
Cai Shen
,
Di Hu
,
Wei Deng
,
Daojie Dong
,
Xufeng Zhou
,
George Z. Chen
,
Zhaoping Liu
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acsami.2c13193
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acsami.2c13193
The uncontrollable formation of polymorphous Li deposits, e.g., whiskers, mosses, or dendrites resulting from nonuniform interfacial current distribution and internal stress release in the upward direction on the conventional current collector (e.g., Cu foil) of Li metal rechargeable batteries with a lithium-metal-free negatrode (LMFRBs), leads to rapid performance degradation or serious safety problems. The 3D carbon nanotubes (CNTs) skeleton has been proven to effectively reduce the current density and eliminate the internal accumulated stress. However, remarkable electrolyte decomposition, inherent Li source consumption due to repeated SEI formation, and Li+ intercalation in CNTs limit the application of 3D CNTs skeleton. Thus, it is necessary to avoid the side effects of the 3D CNTs skeleton and retain uniform interfacial current distribution and stress mitigation. In this work, we integrate the CNTs network with a soft functional polymer polyvinylidene fluoride (PVDF) to form a relatively dense coating layer on Cu foil, which can shield the contact between the internal surface of the 3D CNTs framework and the electrolyte. Simultaneously, the Li-F-rich SEI resulting from the partial reduction of PVDF with deposited Li and the soft nature of the coating layer release the accumulation of internal stress in the horizontal direction, resulting in mosses/whisker-free Li deposition. Thus, improved Li deposition/dissolution and stable cycling performance of the LMFRBs can be achieved.
Related Topics
Concepts
Materials science
Polyvinylidene fluoride
Current collector
Composite material
Electrolyte
Coating
Carbon nanotube
Whiskers
Plating (geology)
FOIL method
Dissolution
Whisker
Layer (electronics)
Electroplating
Polypyrrole
Polymer
Chemical engineering
Electrode
Engineering
Geophysics
Chemistry
Geology
Polymerization
Physical chemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acsami.2c13193
- OA Status
- green
- Cited By
- 9
- References
- 58
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4297990200
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4297990200Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1021/acsami.2c13193Digital Object Identifier
- Title
-
CNT/PVDF Composite Coating Layer on Cu with a Synergy of Uniform Current Distribution and Stress Releasing for Improving Reversible Li Plating/StrippingWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-09-29Full publication date if available
- Authors
-
Qiang Guo, Yanan Yu, Shengjie Xia, Cai Shen, Di Hu, Wei Deng, Daojie Dong, Xufeng Zhou, George Z. Chen, Zhaoping LiuList of authors in order
- Landing page
-
https://doi.org/10.1021/acsami.2c13193Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://nottingham-repository.worktribe.com/output/11755959Direct OA link when available
- Concepts
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Materials science, Polyvinylidene fluoride, Current collector, Composite material, Electrolyte, Coating, Carbon nanotube, Whiskers, Plating (geology), FOIL method, Dissolution, Whisker, Layer (electronics), Electroplating, Polypyrrole, Polymer, Chemical engineering, Electrode, Engineering, Geophysics, Chemistry, Geology, Polymerization, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
9Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 2, 2024: 2, 2023: 5Per-year citation counts (last 5 years)
- References (count)
-
58Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.a | 40, 131, 140 |
| abstract_inverted_index.3D | 54, 96, 110, 159 |
| abstract_inverted_index.Cu | 32, 146 |
| abstract_inverted_index.In | 122 |
| abstract_inverted_index.Li | 5, 35, 79, 178, 200, 204 |
| abstract_inverted_index.be | 214 |
| abstract_inverted_index.in | 22, 90, 193, 198 |
| abstract_inverted_index.is | 101 |
| abstract_inverted_index.it | 100 |
| abstract_inverted_index.of | 3, 34, 95, 108, 157, 174, 183, 190, 210 |
| abstract_inverted_index.on | 26, 145 |
| abstract_inverted_index.or | 10, 49 |
| abstract_inverted_index.to | 45, 62, 83, 103, 138 |
| abstract_inverted_index.we | 125 |
| abstract_inverted_index.SEI | 85, 168 |
| abstract_inverted_index.The | 0, 53 |
| abstract_inverted_index.and | 18, 68, 87, 113, 119, 162, 179, 206 |
| abstract_inverted_index.can | 149, 213 |
| abstract_inverted_index.due | 82 |
| abstract_inverted_index.has | 59 |
| abstract_inverted_index.the | 23, 27, 65, 70, 93, 105, 109, 127, 151, 154, 158, 163, 166, 171, 180, 184, 188, 194, 211 |
| abstract_inverted_index.CNTs | 91, 97, 111, 128, 160 |
| abstract_inverted_index.PVDF | 175 |
| abstract_inverted_index.been | 60 |
| abstract_inverted_index.form | 139 |
| abstract_inverted_index.from | 13, 170 |
| abstract_inverted_index.side | 106 |
| abstract_inverted_index.soft | 132, 181 |
| abstract_inverted_index.this | 123 |
| abstract_inverted_index.with | 39, 130, 176 |
| abstract_inverted_index.Thus, | 99, 202 |
| abstract_inverted_index.avoid | 104 |
| abstract_inverted_index.dense | 142 |
| abstract_inverted_index.e.g., | 7 |
| abstract_inverted_index.foil) | 33 |
| abstract_inverted_index.foil, | 147 |
| abstract_inverted_index.layer | 144, 186 |
| abstract_inverted_index.leads | 44 |
| abstract_inverted_index.limit | 92 |
| abstract_inverted_index.metal | 36 |
| abstract_inverted_index.rapid | 46 |
| abstract_inverted_index.which | 148 |
| abstract_inverted_index.work, | 124 |
| abstract_inverted_index.(CNTs) | 57 |
| abstract_inverted_index.(PVDF) | 137 |
| abstract_inverted_index.(e.g., | 31 |
| abstract_inverted_index.LMFRBs | 212 |
| abstract_inverted_index.carbon | 55 |
| abstract_inverted_index.nature | 182 |
| abstract_inverted_index.proven | 61 |
| abstract_inverted_index.reduce | 64 |
| abstract_inverted_index.retain | 114 |
| abstract_inverted_index.safety | 51 |
| abstract_inverted_index.shield | 150 |
| abstract_inverted_index.source | 80 |
| abstract_inverted_index.stable | 207 |
| abstract_inverted_index.stress | 20, 120, 192 |
| abstract_inverted_index.upward | 24 |
| abstract_inverted_index.between | 153 |
| abstract_inverted_index.coating | 143, 185 |
| abstract_inverted_index.contact | 152 |
| abstract_inverted_index.current | 16, 29, 66, 117 |
| abstract_inverted_index.cycling | 208 |
| abstract_inverted_index.density | 67 |
| abstract_inverted_index.effects | 107 |
| abstract_inverted_index.mosses, | 9 |
| abstract_inverted_index.network | 129 |
| abstract_inverted_index.partial | 172 |
| abstract_inverted_index.polymer | 134 |
| abstract_inverted_index.release | 21, 187 |
| abstract_inverted_index.serious | 50 |
| abstract_inverted_index.stress. | 73 |
| abstract_inverted_index.surface | 156 |
| abstract_inverted_index.uniform | 115 |
| abstract_inverted_index.However, | 74 |
| abstract_inverted_index.fluoride | 136 |
| abstract_inverted_index.improved | 203 |
| abstract_inverted_index.inherent | 78 |
| abstract_inverted_index.internal | 19, 71, 155, 191 |
| abstract_inverted_index.repeated | 84 |
| abstract_inverted_index.skeleton | 58, 112 |
| abstract_inverted_index.(LMFRBs), | 43 |
| abstract_inverted_index.Li-F-rich | 167 |
| abstract_inverted_index.achieved. | 215 |
| abstract_inverted_index.batteries | 38 |
| abstract_inverted_index.collector | 30 |
| abstract_inverted_index.dendrites | 11 |
| abstract_inverted_index.deposited | 177 |
| abstract_inverted_index.deposits, | 6 |
| abstract_inverted_index.direction | 25 |
| abstract_inverted_index.eliminate | 69 |
| abstract_inverted_index.formation | 2 |
| abstract_inverted_index.framework | 161 |
| abstract_inverted_index.integrate | 126 |
| abstract_inverted_index.nanotubes | 56 |
| abstract_inverted_index.necessary | 102 |
| abstract_inverted_index.negatrode | 42 |
| abstract_inverted_index.problems. | 52 |
| abstract_inverted_index.reduction | 173 |
| abstract_inverted_index.resulting | 12, 169, 197 |
| abstract_inverted_index.skeleton. | 98 |
| abstract_inverted_index.whiskers, | 8 |
| abstract_inverted_index.direction, | 196 |
| abstract_inverted_index.formation, | 86 |
| abstract_inverted_index.functional | 133 |
| abstract_inverted_index.horizontal | 195 |
| abstract_inverted_index.nonuniform | 14 |
| abstract_inverted_index.relatively | 141 |
| abstract_inverted_index.remarkable | 75 |
| abstract_inverted_index.accumulated | 72 |
| abstract_inverted_index.application | 94 |
| abstract_inverted_index.consumption | 81 |
| abstract_inverted_index.degradation | 48 |
| abstract_inverted_index.deposition. | 201 |
| abstract_inverted_index.effectively | 63 |
| abstract_inverted_index.electrolyte | 76 |
| abstract_inverted_index.interfacial | 15, 116 |
| abstract_inverted_index.mitigation. | 121 |
| abstract_inverted_index.performance | 47, 209 |
| abstract_inverted_index.accumulation | 189 |
| abstract_inverted_index.conventional | 28 |
| abstract_inverted_index.distribution | 17, 118 |
| abstract_inverted_index.electrolyte. | 164 |
| abstract_inverted_index.polymorphous | 4 |
| abstract_inverted_index.rechargeable | 37 |
| abstract_inverted_index.intercalation | 89 |
| abstract_inverted_index.Li<sup>+</sup> | 88 |
| abstract_inverted_index.decomposition, | 77 |
| abstract_inverted_index.polyvinylidene | 135 |
| abstract_inverted_index.uncontrollable | 1 |
| abstract_inverted_index.Simultaneously, | 165 |
| abstract_inverted_index.lithium-metal-free | 41 |
| abstract_inverted_index.mosses/whisker-free | 199 |
| abstract_inverted_index.deposition/dissolution | 205 |
| cited_by_percentile_year.max | 98 |
| cited_by_percentile_year.min | 94 |
| corresponding_author_ids | https://openalex.org/A5100749714, https://openalex.org/A5109998601, https://openalex.org/A5080423762 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I142263535, https://openalex.org/I19820366, https://openalex.org/I4210165339 |
| citation_normalized_percentile.value | 0.73487062 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |