Co ₃ O ₄ /C‐NFs Induced 3D Electric Field Enhancement for Dual‐Regulation of Polysulfides and Li ⁺ Transport in Lithium–Sulfur Batteries Article Swipe

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Zhijie Qi , Jun Jiang , Pengcheng Yao , Zhenjie Lu , Shen Ying , Shujun Liu , Sun Jingwen , Pan Xiong , Xin Wang , Xiaoping Ouyang , Junwu Zhu , Yongsheng Fu , Zhijie Qi , Jun Jiang , Pengcheng Yao , Zhenjie Lu , Shen Ying , Shujun Liu , Sun Jingwen , Pan Xiong , Xin Wang , Xiaoping Ouyang , Junwu Zhu , Yongsheng Fu ·

YOU? · · 2025 · Open Access · · DOI: https://doi.org/10.1002/advs.202520167

Lithium–sulfur batteries (LSBs) are promising next‐generation energy storage systems, yet their practical application is hindered by sluggish and uncontrolled mass transport of Li + and lithium polysulfides (LiPSs). Here, a Co 3 O 4 ‐based nano‐framework catalyst (Co 3 O 4 /C‐NFs) is designed featuring a highly symmetric 3D sharp‐edged architecture that induces strong 3D electric field enhancement. This unique structural design promotes the directional migration and enrichment of negatively charged species, thereby accelerating the sulfur reduction reaction (SRR) kinetics, suppressing LiPSs shuttling, and improving Li⁺ transport. Moreover, by monitoring the real‐time conversion of LiPSs during the reaction using integrated in situ techniques, a universal method for quantitatively evaluating LiPSs conversion kinetics is proposed. Both experimental and theoretical results confirm that the 3D electric field enhancement governs mass transfer at multiple scales, achieving efficient ion regulation and interfacial stability. Benefiting from this effect, the assembled double‐layer pouch cell with a high sulfur loading of 6.5 mg cm −2 and a lean electrolyte ratio (E/S = 4 µL mg −1 ) maintains stable cycling for over 100 cycles at 0.1C, delivering a specific capacity of 1200 mAh g −1 . This work introduces a new paradigm of 3D electric field–driven mass transfer modulation for designing high‐performance and practical LSBs.

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Energy Transformation

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Electric field Electrolyte Materials science Mass transfer Catalysis Chemical engineering Lithium (medication) Mass transport Energy storage Kinetics Ion Sulfur Electrode Nanotechnology Work (physics) Degradation (telecommunications) Redox Electrochemistry Current density Field (mathematics) Energy transformation Reduction (mathematics) Energy conversion efficiency Electron transfer

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Type: article
Language: en
Landing Page: https://doi.org/10.1002/advs.202520167
PDF: https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202520167
OA Status: gold
References: 40
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DOI: https://doi.org/10.1002/advs.202520167

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Title: Co ₃ O ₄ /C‐NFs Induced 3D Electric Field Enhancement for Dual‐Regulation of Polysulfides and Li ⁺ Transport in Lithium–Sulfur Batteries

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Publication year: 2025

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Publication date: 2025-11-25

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Authors: Zhijie Qi, Jun Jiang, Pengcheng Yao, Zhenjie Lu, Shen Ying, Shujun Liu, Sun Jingwen, Pan Xiong, Xin Wang, Xiaoping Ouyang, Junwu Zhu, Yongsheng Fu, Zhijie Qi, Jun Jiang, Pengcheng Yao, Zhenjie Lu, Shen Ying, Shujun Liu, Sun Jingwen, Pan Xiong, Xin Wang, Xiaoping Ouyang, Junwu Zhu, Yongsheng Fu

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Landing page: https://doi.org/10.1002/advs.202520167

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Concepts: Electric field, Electrolyte, Materials science, Mass transfer, Catalysis, Chemical engineering, Lithium (medication), Mass transport, Energy storage, Kinetics, Ion, Sulfur, Electrode, Nanotechnology, Work (physics), Degradation (telecommunications), Redox, Electrochemistry, Current density, Field (mathematics), Energy transformation, Reduction (mathematics), Energy conversion efficiency, Electron transfer

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abstract_inverted_index.situ	102
abstract_inverted_index.that	52, 121
abstract_inverted_index.this	142
abstract_inverted_index.with	149
abstract_inverted_index.work	191
abstract_inverted_index.−1	169, 188
abstract_inverted_index.−2	158
abstract_inverted_index.(SRR)	79
abstract_inverted_index.0.1C,	179
abstract_inverted_index.Here,	29
abstract_inverted_index.LSBs.	208
abstract_inverted_index.LiPSs	82, 95, 110
abstract_inverted_index.Li⁺	86
abstract_inverted_index.field	57, 125
abstract_inverted_index.pouch	147
abstract_inverted_index.ratio	163
abstract_inverted_index.their	11
abstract_inverted_index.using	99
abstract_inverted_index.(LSBs)	3
abstract_inverted_index.cycles	177
abstract_inverted_index.design	62
abstract_inverted_index.during	96
abstract_inverted_index.energy	7
abstract_inverted_index.highly	47
abstract_inverted_index.method	106
abstract_inverted_index.stable	172
abstract_inverted_index.strong	54
abstract_inverted_index.sulfur	76, 152
abstract_inverted_index.unique	60
abstract_inverted_index.charged	71
abstract_inverted_index.confirm	120
abstract_inverted_index.cycling	173
abstract_inverted_index.effect,	143
abstract_inverted_index.governs	127
abstract_inverted_index.induces	53
abstract_inverted_index.lithium	26
abstract_inverted_index.loading	153
abstract_inverted_index.results	119
abstract_inverted_index.scales,	132
abstract_inverted_index.storage	8
abstract_inverted_index.thereby	73
abstract_inverted_index.(LiPSs).	28
abstract_inverted_index.Abstract	0
abstract_inverted_index.capacity	183
abstract_inverted_index.catalyst	37
abstract_inverted_index.designed	44
abstract_inverted_index.electric	56, 124, 198
abstract_inverted_index.hindered	15
abstract_inverted_index.kinetics	112
abstract_inverted_index.multiple	131
abstract_inverted_index.paradigm	195
abstract_inverted_index.promotes	63
abstract_inverted_index.reaction	78, 98
abstract_inverted_index.sluggish	17
abstract_inverted_index.species,	72
abstract_inverted_index.specific	182
abstract_inverted_index.systems,	9
abstract_inverted_index.transfer	129, 201
abstract_inverted_index.‐based	35
abstract_inverted_index./C‐NFs)	42
abstract_inverted_index.Moreover,	88
abstract_inverted_index.achieving	133
abstract_inverted_index.assembled	145
abstract_inverted_index.batteries	2
abstract_inverted_index.designing	204
abstract_inverted_index.efficient	134
abstract_inverted_index.featuring	45
abstract_inverted_index.improving	85
abstract_inverted_index.kinetics,	80
abstract_inverted_index.maintains	171
abstract_inverted_index.migration	66
abstract_inverted_index.practical	12, 207
abstract_inverted_index.promising	5
abstract_inverted_index.proposed.	114
abstract_inverted_index.reduction	77
abstract_inverted_index.symmetric	48
abstract_inverted_index.transport	21
abstract_inverted_index.universal	105
abstract_inverted_index.Benefiting	140
abstract_inverted_index.conversion	93, 111
abstract_inverted_index.delivering	180
abstract_inverted_index.enrichment	68
abstract_inverted_index.evaluating	109
abstract_inverted_index.integrated	100
abstract_inverted_index.introduces	192
abstract_inverted_index.modulation	202
abstract_inverted_index.monitoring	90
abstract_inverted_index.negatively	70
abstract_inverted_index.regulation	136
abstract_inverted_index.shuttling,	83
abstract_inverted_index.stability.	139
abstract_inverted_index.structural	61
abstract_inverted_index.transport.	87
abstract_inverted_index.application	13
abstract_inverted_index.directional	65
abstract_inverted_index.electrolyte	162
abstract_inverted_index.enhancement	126
abstract_inverted_index.interfacial	138
abstract_inverted_index.real‐time	92
abstract_inverted_index.suppressing	81
abstract_inverted_index.techniques,	103
abstract_inverted_index.theoretical	118
abstract_inverted_index.accelerating	74
abstract_inverted_index.architecture	51
abstract_inverted_index.enhancement.	58
abstract_inverted_index.experimental	116
abstract_inverted_index.polysulfides	27
abstract_inverted_index.uncontrolled	19
abstract_inverted_index.sharp‐edged	50
abstract_inverted_index.double‐layer	146
abstract_inverted_index.field–driven	199
abstract_inverted_index.quantitatively	108
abstract_inverted_index.Lithium–sulfur	1
abstract_inverted_index.nano‐framework	36
abstract_inverted_index.next‐generation	6
abstract_inverted_index.high‐performance	205
cited_by_percentile_year
countries_distinct_count	2
institutions_distinct_count	24
citation_normalized_percentile

Co 3 O 4 /C‐NFs Induced 3D Electric Field Enhancement for Dual‐Regulation of Polysulfides and Li + Transport in Lithium–Sulfur Batteries Article Swipe

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Co ₃ O ₄ /C‐NFs Induced 3D Electric Field Enhancement for Dual‐Regulation of Polysulfides and Li ⁺ Transport in Lithium–Sulfur Batteries Article Swipe