Colossal optical anisotropy from atomic-scale modulations Article Swipe
Hongyan Mei
,
Guodong Ren
,
Boyang Zhao
,
Jad Salman
,
Gwan Yeong Jung
,
Huandong Chen
,
Shantanu Singh
,
Arashdeep Singh Thind
,
John Cavin
,
Jordan A. Hachtel
,
Miaofang Chi
,
Shanyuan Niu
,
Graham Joe
,
Chenghao Wan
,
Nick Settineri
,
Simon J. Teat
,
Bryan C. Chakoumakos
,
Jayakanth Ravichandran
,
Rohan Mishra
,
Mikhail A. Kats
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2303.00041
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2303.00041
In modern optics, materials with large birefringence (Δn, where n is the refractive index) are sought after for polarization control (e.g. in wave plates, polarizing beam splitters, etc.), nonlinear optics and quantum optics (e.g. for phase matching and production of entangled photons), micromanipulation, and as a platform for unconventional light-matter coupling, such as Dyakonov-like surface polaritons and hyperbolic phonon polaritons. Layered "van der Waals" materials, with strong intra-layer bonding and weak inter-layer bonding, can feature some of the largest optical anisotropy; however, their use in most optical systems is limited because their optic axis is out of the plane of the layers and the layers are weakly attached, making the anisotropy hard to access. Here, we demonstrate that a bulk crystal with subtle periodic modulations in its structure -- Sr9/8TiS3 -- is transparent and positive-uniaxial, with extraordinary index n_e = 4.5 and ordinary index n_o = 2.4 in the mid- to far-infrared. The excess Sr, compared to stoichiometric SrTiS3, results in the formation of TiS6 trigonal-prismatic units that break the infinite chains of face-shared TiS6 octahedra in SrTiS3 into periodic blocks of five TiS6 octahedral units. The additional electrons introduced by the excess Sr subsequently occupy the TiS6 octahedral blocks to form highly oriented and polarizable electron clouds, which selectively boost the extraordinary index n_e and result in record birefringence (Δn > 2.1 with low loss). The connection between subtle structural modulations and large changes in refractive index suggests new categories of anisotropic materials and also tunable optical materials with large refractive-index modulation and low optical losses.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2303.00041
- https://arxiv.org/pdf/2303.00041
- OA Status
- green
- Cited By
- 2
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4322825543
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4322825543Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.48550/arxiv.2303.00041Digital Object Identifier
- Title
-
Colossal optical anisotropy from atomic-scale modulationsWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-02-28Full publication date if available
- Authors
-
Hongyan Mei, Guodong Ren, Boyang Zhao, Jad Salman, Gwan Yeong Jung, Huandong Chen, Shantanu Singh, Arashdeep Singh Thind, John Cavin, Jordan A. Hachtel, Miaofang Chi, Shanyuan Niu, Graham Joe, Chenghao Wan, Nick Settineri, Simon J. Teat, Bryan C. Chakoumakos, Jayakanth Ravichandran, Rohan Mishra, Mikhail A. KatsList of authors in order
- Landing page
-
https://arxiv.org/abs/2303.00041Publisher landing page
- PDF URL
-
https://arxiv.org/pdf/2303.00041Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://arxiv.org/pdf/2303.00041Direct OA link when available
- Concepts
-
Birefringence, Anisotropy, Refractive index, Condensed matter physics, Materials science, van der Waals force, Polarizability, Physics, Optics, Polariton, Quantum mechanics, MoleculeTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
2Total citation count in OpenAlex
- Citations by year (recent)
-
2023: 2Per-year citation counts (last 5 years)
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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