Combining ultrahigh index with exceptional nonlinearity in resonant transition metal dichalcogenide nanodisks Article Swipe
George Zograf
,
Alexander Yu. Polyakov
,
Maria Bancerek
,
Tomasz J. Antosiewicz
,
Betül Küçüköz
,
Timur Shegai
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41566-024-01444-9
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41566-024-01444-9
Second-order nonlinearity in solids gives rise to a plethora of unique physical phenomena ranging from piezoelectricity and optical rectification to optical parametric amplification, spontaneous parametric down-conversion and the generation of entangled photon pairs. Monolayer transition metal dichalcogenides, such as MoS 2 , exhibit one of the highest known second-order nonlinear coefficients. However, the monolayer nature of these materials prevents the fabrication of resonant objects exclusively from the material itself, necessitating the use of external structures to achieve the optical enhancement of nonlinear processes. Here we exploit the 3R phase of a molybdenum disulfide multilayer for resonant nonlinear nanophotonics. The lack of inversion symmetry—even in the bulk of the material—provides a combination of massive second-order susceptibility, extremely high and anisotropic refractive index in the near-infrared region ( n > 4.5) and low absorption losses, making 3R-MoS 2 highly attractive for nonlinear nanophotonics. We demonstrate this by fabricating 3R-MoS 2 nanodisks of various radii, which support resonant anapole states, and observing substantial (>100-fold) enhancement of second-harmonic generation in a single resonant nanodisk compared with an unpatterned flake of the same thickness. The enhancement is maximized at the spectral overlap between the anapole state of the disk and the material resonance of the second-order susceptibility. Our approach unveils a powerful tool for enhancing the entire spectrum of optical second-order nonlinear processes in nanostructured van der Waals materials, thereby paving the way for nonlinear and quantum high-index transition metal dichalcogenide nanophotonics.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41566-024-01444-9
- https://www.nature.com/articles/s41566-024-01444-9.pdf
- OA Status
- hybrid
- Cited By
- 42
- References
- 59
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4399814715
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4399814715Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41566-024-01444-9Digital Object Identifier
- Title
-
Combining ultrahigh index with exceptional nonlinearity in resonant transition metal dichalcogenide nanodisksWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-06-13Full publication date if available
- Authors
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George Zograf, Alexander Yu. Polyakov, Maria Bancerek, Tomasz J. Antosiewicz, Betül Küçüköz, Timur ShegaiList of authors in order
- Landing page
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https://doi.org/10.1038/s41566-024-01444-9Publisher landing page
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https://www.nature.com/articles/s41566-024-01444-9.pdfDirect link to full text PDF
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://www.nature.com/articles/s41566-024-01444-9.pdfDirect OA link when available
- Concepts
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Nanophotonics, Nonlinear optics, Materials science, Monolayer, Second-harmonic generation, Optoelectronics, Plasmon, Refractive index, Photonics, Physics, Condensed matter physics, Nanotechnology, Optics, LaserTop concepts (fields/topics) attached by OpenAlex
- Cited by
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42Total citation count in OpenAlex
- Citations by year (recent)
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2025: 34, 2024: 8Per-year citation counts (last 5 years)
- References (count)
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59Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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