Comment on acp-2021-1010 Article Swipe
Jingnan Shi
,
Juan Hong
,
Nan Ma
,
Qingwei Luo
,
Yao He
,
Hanbing Xu
,
Haobo Tan
,
Qiaoqiao Wang
,
Jiangchuan Tao
,
Yaqing Zhou
,
Shuang Han
,
Long Peng
,
Linhong Xie
,
Guangsheng Zhou
,
Wanyun Xu
,
Yele Sun
,
Yafang Cheng
,
Hang Su
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.5194/acp-2021-1010-rc2
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.5194/acp-2021-1010-rc2
Abstract. Atmospheric processes, including both primary emissions and secondary formation, may exert complex effects on aerosol hygroscopicity, which is of significant importance in understanding and quantifying the effect of aerosols on climate and human health. In order to explore the influence of local emissions and secondary formation processes on aerosol hygroscopicity, we investigated the hygroscopic properties of submicron aerosol particles at a rural site in the North China Plain (NCP) in winter 2018. This was conducted by simultaneous measurements of aerosol hygroscopicity and chemical composition, using a custom-built hygroscopic tandem differential mobility analyzer (HTDMA) and a capture-vaporizer time-of-flight aerosol chemical speciation monitor (CV-ToF-ACSM). The hygroscopicity results showed that the particles during the entire campaign were mainly externally mixed, with a more hygroscopic (MH) mode and a less hygroscopic (LH) mode. The mean hygroscopicity parameter (κmean) values derived from hygroscopicity measurements for particles at 60, 100, 150, and 200 nm were 0.16, 0.18, 0.16, and 0.15, respectively. During this study, we classified two distinct episodes with different relative humidity (RH) and temperature (T) conditions, indicative of different primary emissions and secondary formation processes. It was observed that aerosols at all measured sizes were more hygroscopic under the high-RH (HRH) episode than those under the low-RH (LRH) episode. During the LRH, κ decreased with increasing particle size, which may be explained by the enhanced domestic heating at low temperature, causing large emissions of non-hygroscopic or less hygroscopic primary aerosols. This is particularly obvious for 200 nm particles, with a dominant number fraction (>50 %) of LH mode particles. Using O:C-dependent hygroscopic parameters of secondary organic compounds (κSOA), closure analysis between the HTDMA-measured κ and the ACSM-derived κ was carried out. The results showed that κSOA under the LRH episode was less sensitive to the changes in organic oxidation level, while κSOA under HRH had a relatively stronger dependency on the organic O:C ratio. This feature suggests that the different sources and aerosol evolution processes, partly resulting from the variation in atmospheric RH and T conditions, may lead to significant changes in aerosol chemical composition, which will further influence their corresponding physical properties.
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Metadata
- Type
- peer-review
- Language
- en
- Landing Page
- https://doi.org/10.5194/acp-2021-1010-rc2
- https://acp.copernicus.org/articles/22/4599/2022/acp-22-4599-2022.pdf
- OA Status
- gold
- References
- 64
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4210896343
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4210896343Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.5194/acp-2021-1010-rc2Digital Object Identifier
- Title
-
Comment on acp-2021-1010Work title
- Type
-
peer-reviewOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-02-07Full publication date if available
- Authors
-
Jingnan Shi, Juan Hong, Nan Ma, Qingwei Luo, Yao He, Hanbing Xu, Haobo Tan, Qiaoqiao Wang, Jiangchuan Tao, Yaqing Zhou, Shuang Han, Long Peng, Linhong Xie, Guangsheng Zhou, Wanyun Xu, Yele Sun, Yafang Cheng, Hang SuList of authors in order
- Landing page
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https://doi.org/10.5194/acp-2021-1010-rc2Publisher landing page
- PDF URL
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https://acp.copernicus.org/articles/22/4599/2022/acp-22-4599-2022.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
- OA URL
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https://acp.copernicus.org/articles/22/4599/2022/acp-22-4599-2022.pdfDirect OA link when available
- Concepts
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Aerosol, Relative humidity, Differential mobility analyzer, Chemistry, Particle (ecology), Atmospheric sciences, Analytical Chemistry (journal), Environmental chemistry, Environmental science, Meteorology, Organic chemistry, Geography, Physics, Oceanography, GeologyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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64Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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