Comment on acp-2022-774 Article Swipe
Yiqun Lu
,
Yingge Ma
,
Dan Dan Huang
,
Shengrong Lou
,
Shengao Jing
,
Yaqin Gao
,
Hongli Wang
,
Yanjun Zhang
,
Hui Chen
,
Naiqiang Yan
,
Jianmin Chen
,
C. George
,
Matthieu Riva
,
Cheng Huang
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.5194/acp-2022-774-rc2
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.5194/acp-2022-774-rc2
Abstract. Oxygenated organic molecules (OOMs) are dominated by the N-containing species in polluted urban environment. As N-containing OOMs, especially those with more than one nitrogen atoms, prevailed in the high m/z range (m/z > 350Th), unambiguous identification of N-containing OOMs is highly desirable for understanding of their formation processes, precursors and influencing factors. To achieve this, we applied an ultra-high-resolution chemical ionization-orbitrap (CI-Orbitrap) in a field campaign and found that OOMs contain one (1N-OOMs), two (2N-OOMs) and three (3N-OOMs) nitrogen atoms respectively comprised 50 %, 26 % and 4 % of total OOMs. More interestingly, the fraction of 2N-OOMs increased with the increase of carbon number (nC) and were dominated by the ones derived from aliphatic precursors (2N-OOMAli, 64.2 %), indicating the importance of multistep oxidation. Plausible precursors of 2N-OOMs were aliphatics (2N-OOMAli, 64.2 %), aromatics (2N-OOMAro, 16 %), and monoterpenes (2N-OOMMT, 15.4 %). The 2N-OOMAli was the most abundant 2N-OOMs and its fraction even increased in the polluted day with enhanced proportion of the ones with nC>10. While 2N-OOMAli and 2N-OOMAro were dominated by daytime photochemical production, nighttime NO3-initiated oxidation dominated the formation of 2N-OOMMT. 2N-OOMAro were of highest oxygenation level, followed by 2N-OOMMT and 2N-OOMAli, which were affected by photochemistry and NOx concentrations. These results highlight the significant formation of 2N-OOMs and the influencing factors, on their formation in polluted urban environment, where various VOC precursors and atmospheric oxidants present.
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- Type
- peer-review
- Language
- en
- Landing Page
- https://doi.org/10.5194/acp-2022-774-rc2
- OA Status
- gold
- References
- 44
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
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https://doi.org/10.5194/acp-2022-774-rc2Digital Object Identifier
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Comment on acp-2022-774Work title
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peer-reviewOpenAlex work type
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enPrimary language
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2022Year of publication
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2022-12-12Full publication date if available
- Authors
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Yiqun Lu, Yingge Ma, Dan Dan Huang, Shengrong Lou, Shengao Jing, Yaqin Gao, Hongli Wang, Yanjun Zhang, Hui Chen, Naiqiang Yan, Jianmin Chen, C. George, Matthieu Riva, Cheng HuangList of authors in order
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https://doi.org/10.5194/acp-2022-774-rc2Direct OA link when available
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