Comment on egusphere-2023-2328 Article Swipe
Ryan Farley
,
James E. Lee
,
Laura-Hélà ̈na Rivellini
,
Alex K. Y. Lee
,
Rachael Dal Porto
,
Christopher D. Cappa
,
Kyle Gorkowski
,
Abu Sayeed Shawon
,
Katherine Benedict
,
A. C. Aiken
,
Manvendra K. Dubey
,
Qi Zhang
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.5194/egusphere-2023-2328-rc1
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.5194/egusphere-2023-2328-rc1
Abstract. A high-resolution soot particle aerosol mass spectrometer (SP-AMS) was used to selectively measure refractory black carbon (rBC) and its associated coating material using both the ensemble size-resolved mass spectral mode and the event trigger single particle (ETSP) mode in Houston, Texas in summer 2022. This study was conducted as part of the Department of Energy Atmospheric Radiation Measurement (ARM) program’s Tracking Aerosol Convection Interactions Experiment (TRACER) field campaign. The study revealed an average (± 1s) rBC concentration of 103 ± 176 ng m-3. Additionally, the coatings on the BC particles were primarily composed of organics (59 %; 219 ± 260 ng m-3) and sulfate (26 %; 94 ± 55 ng m-3). Positive matrix factorization (PMF) analysis of the ensemble mass spectra of BC-containing particles resolved four distinct types of soot aerosol, including an oxidized organic aerosol (OOABC,PMF) factor associated with processed primary organic aerosol, an inorganic sulfate factor (SO4,BC,PMF), an oxidized rBC factor (O-BCPMF), and a mixed mineral dust/biomass burning aerosol factor with significant contribution from potassium (K-BBBC,PMF). Additionally, K-Means clustering analysis of the single particle mass spectra identified eight different clusters, including soot particles enriched in hydrocarbon like organic aerosol (HOABC,ETSP), sulfate (SO4,BC,ETSP), two types of rBC, OOA (OOABC,ETSP), chloride (ClBC,ETSP) and nitrate (NO3,BC,ETSP). The single particle measurements demonstrate substantial variation in BC coating thickness with coating-to-rBC mass ratios ranging from 0.1 to 100. The mixing state index (χ), which denotes the degree of homogeneity of the soot aerosol, varied from 4 to 94 % with a median of 40 %, indicating that the aerosol population lies in between internal and external mixing but has large temporal and source type variability. In addition, a significant fraction of BC-containing particles, a majority enriched with oxidized organics and sulfate, exhibit sufficiently high κ values and diameters conducive to activation as cloud nuclei under atmospherically relevant supersaturation conditions. This finding bears significance in comprehending the activation of rBC-containing particles as cloud droplets and the origins of CCN in urban areas. Our analysis highlights the complex nature of soot aerosol and underscore the need to comprehend its variability across different environments for accurate assessment of climate change.
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Metadata
- Type
- peer-review
- Language
- en
- Landing Page
- https://doi.org/10.5194/egusphere-2023-2328-rc1
- OA Status
- gold
- References
- 82
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4389476431
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4389476431Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.5194/egusphere-2023-2328-rc1Digital Object Identifier
- Title
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Comment on egusphere-2023-2328Work title
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peer-reviewOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-12-08Full publication date if available
- Authors
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Ryan Farley, James E. Lee, Laura-Hélà ̈na Rivellini, Alex K. Y. Lee, Rachael Dal Porto, Christopher D. Cappa, Kyle Gorkowski, Abu Sayeed Shawon, Katherine Benedict, A. C. Aiken, Manvendra K. Dubey, Qi ZhangList of authors in order
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https://doi.org/10.5194/egusphere-2023-2328-rc1Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.5194/egusphere-2023-2328-rc1Direct OA link when available
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Aerosol, Soot, Analytical Chemistry (journal), Chemistry, Sulfate, Particle (ecology), Mineralogy, Environmental chemistry, Combustion, Physical chemistry, Organic chemistry, Geology, OceanographyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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82Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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