Concurrent multi-peak Bragg coherent x-ray diffraction imaging of 3D nanocrystal lattice displacement via global optimization Article Swipe
YOU?
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· 2023
· Open Access
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· DOI: https://doi.org/10.1038/s41524-023-01022-7
In this paper we demonstrated a method to reconstruct vector-valued lattice distortion fields within nanoscale crystals by optimization of a forward model of multi-reflection Bragg coherent diffraction imaging (MR-BCDI) data. The method flexibly accounts for geometric factors that arise when making BCDI measurements, is amenable to efficient inversion with modern optimization toolkits, and allows for globally constraining a single image reconstruction to multiple Bragg peak measurements. This is enabled by a forward model that emulates the multiple Bragg peaks of a MR-BCDI experiment from a single estimate of the 3D crystal sample. We present this forward model, we implement it within the stochastic gradient descent optimization framework, and we demonstrate it with simulated and experimental data of nanocrystals with inhomogeneous internal lattice displacement. We find that utilizing a global optimization approach to MR-BCDI affords a reliable path to convergence of data which is otherwise challenging to reconstruct.
Related Topics
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41524-023-01022-7
- https://www.nature.com/articles/s41524-023-01022-7.pdf
- OA Status
- gold
- Cited By
- 7
- References
- 41
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4378086191
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4378086191Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41524-023-01022-7Digital Object Identifier
- Title
-
Concurrent multi-peak Bragg coherent x-ray diffraction imaging of 3D nanocrystal lattice displacement via global optimizationWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-05-23Full publication date if available
- Authors
-
Siddharth Maddali, Travis D. Frazer, Nazar Delegan, Katherine Harmon, Sean E. Sullivan, Marc Allain, Wonsuk Cha, Alan Dibos, Ishwor Poudyal, Saugat Kandel, Youssef S. G. Nashed, F. Joseph Heremans, Hoydoo You, Yue Cao, S. O. HruszkewyczList of authors in order
- Landing page
-
https://doi.org/10.1038/s41524-023-01022-7Publisher landing page
- PDF URL
-
https://www.nature.com/articles/s41524-023-01022-7.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://www.nature.com/articles/s41524-023-01022-7.pdfDirect OA link when available
- Concepts
-
Bragg's law, Global optimization, Optics, Diffraction, Lattice (music), Gradient descent, Algorithm, Bragg peak, Displacement (psychology), Computer science, Physics, Artificial intelligence, Acoustics, Artificial neural network, Psychology, Beam (structure), PsychotherapistTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
7Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 3, 2024: 4Per-year citation counts (last 5 years)
- References (count)
-
41Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.forward | 21, 72, 96 |
| abstract_inverted_index.imaging | 28 |
| abstract_inverted_index.lattice | 11, 122 |
| abstract_inverted_index.present | 94 |
| abstract_inverted_index.sample. | 92 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.accounts | 34 |
| abstract_inverted_index.amenable | 45 |
| abstract_inverted_index.approach | 131 |
| abstract_inverted_index.coherent | 26 |
| abstract_inverted_index.crystals | 16 |
| abstract_inverted_index.emulates | 75 |
| abstract_inverted_index.estimate | 87 |
| abstract_inverted_index.flexibly | 33 |
| abstract_inverted_index.globally | 56 |
| abstract_inverted_index.gradient | 104 |
| abstract_inverted_index.internal | 121 |
| abstract_inverted_index.multiple | 63, 77 |
| abstract_inverted_index.reliable | 136 |
| abstract_inverted_index.(MR-BCDI) | 29 |
| abstract_inverted_index.efficient | 47 |
| abstract_inverted_index.geometric | 36 |
| abstract_inverted_index.implement | 99 |
| abstract_inverted_index.inversion | 48 |
| abstract_inverted_index.nanoscale | 15 |
| abstract_inverted_index.otherwise | 144 |
| abstract_inverted_index.simulated | 113 |
| abstract_inverted_index.toolkits, | 52 |
| abstract_inverted_index.utilizing | 127 |
| abstract_inverted_index.distortion | 12 |
| abstract_inverted_index.experiment | 83 |
| abstract_inverted_index.framework, | 107 |
| abstract_inverted_index.stochastic | 103 |
| abstract_inverted_index.challenging | 145 |
| abstract_inverted_index.convergence | 139 |
| abstract_inverted_index.demonstrate | 110 |
| abstract_inverted_index.diffraction | 27 |
| abstract_inverted_index.reconstruct | 9 |
| abstract_inverted_index.constraining | 57 |
| abstract_inverted_index.demonstrated | 5 |
| abstract_inverted_index.experimental | 115 |
| abstract_inverted_index.nanocrystals | 118 |
| abstract_inverted_index.optimization | 18, 51, 106, 130 |
| abstract_inverted_index.reconstruct. | 147 |
| abstract_inverted_index.displacement. | 123 |
| abstract_inverted_index.inhomogeneous | 120 |
| abstract_inverted_index.measurements, | 43 |
| abstract_inverted_index.measurements. | 66 |
| abstract_inverted_index.vector-valued | 10 |
| abstract_inverted_index.reconstruction | 61 |
| abstract_inverted_index.multi-reflection | 24 |
| cited_by_percentile_year.max | 98 |
| cited_by_percentile_year.min | 97 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 15 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/11 |
| sustainable_development_goals[0].score | 0.4399999976158142 |
| sustainable_development_goals[0].display_name | Sustainable cities and communities |
| citation_normalized_percentile.value | 0.90456709 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |