Conductive Zeolite Supported Indium–Tin Alloy Nanoclusters for Selective and Scalable Formic Acid Electrosynthesis Article Swipe
Zhen Zhang
,
Minzhe Li
,
Shuwen Yang
,
Qianyi Ma
,
Jianan Dang
,
Renfei Feng
,
Zhengyu Bai
,
Dianhua Liu
,
Ming Feng
,
Zhongwei Chen
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202407266
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202407266
Upgrading excess CO 2 toward the electrosynthesis of formic acid is of significant research and commercial interest. However, simultaneously achieving high selectivity and industrially relevant current densities of CO 2 ‐to‐formate conversion remains a grand challenge for practical implementations. Here, an electrically conductive zeolite support is strategically designed by implanting Sn ions into the skeleton structure of a zeolite Y, which impregnates ultrasmall In 0.2 Sn 0.8 alloy nanoclusters into the supercages of the tailored 12‐ring framework. The prominent electronic and geometric interactions between In 0.2 Sn 0.8 nanoalloy and zeolite support lead to the delocalization of electron density that enhances orbital hybridizations between In active site and *OCHO intermediate. Thus, the energy barrier for the rate‐limiting *OCHO formation step is reduced, facilitating the electrocatalytic hydrogenation of CO 2 to formic acid. Accordingly, the developed zeolite electrocatalyst achieves an industrial‐level partial current density of 322 mA cm −2 and remarkable Faradaic efficiency of 98.2% for formate production and stably maintains Faradaic efficiency above 93% at an industrially relevant current density for over 102 h. This work opens up new opportunities of conductive zeolite‐based electrocatalysts for industrial‐level formic acid electrosynthesis from CO 2 electrolysis and toward practically accessible electrocatalysis and energy conversion.
Related Topics
Concepts
Electrosynthesis
Faraday efficiency
Nanoclusters
Materials science
Zeolite
Electrocatalyst
Formic acid
Electrolysis
Inorganic chemistry
Chemical engineering
Catalysis
Nanotechnology
Electrolyte
Electrode
Chemistry
Electrochemistry
Organic chemistry
Physical chemistry
Engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202407266
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202407266
- OA Status
- bronze
- Cited By
- 16
- References
- 75
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4401184460
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4401184460Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/adma.202407266Digital Object Identifier
- Title
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Conductive Zeolite Supported Indium–Tin Alloy Nanoclusters for Selective and Scalable Formic Acid ElectrosynthesisWork title
- Type
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articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-07-31Full publication date if available
- Authors
-
Zhen Zhang, Minzhe Li, Shuwen Yang, Qianyi Ma, Jianan Dang, Renfei Feng, Zhengyu Bai, Dianhua Liu, Ming Feng, Zhongwei ChenList of authors in order
- Landing page
-
https://doi.org/10.1002/adma.202407266Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202407266Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
bronzeOpen access status per OpenAlex
- OA URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202407266Direct OA link when available
- Concepts
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Electrosynthesis, Faraday efficiency, Nanoclusters, Materials science, Zeolite, Electrocatalyst, Formic acid, Electrolysis, Inorganic chemistry, Chemical engineering, Catalysis, Nanotechnology, Electrolyte, Electrode, Chemistry, Electrochemistry, Organic chemistry, Physical chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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16Total citation count in OpenAlex
- Citations by year (recent)
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2025: 15, 2024: 1Per-year citation counts (last 5 years)
- References (count)
-
75Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.industrially | 24, 167 |
| abstract_inverted_index.interactions | 83 |
| abstract_inverted_index.nanoclusters | 69 |
| abstract_inverted_index.hydrogenation | 126 |
| abstract_inverted_index.intermediate. | 110 |
| abstract_inverted_index.opportunities | 180 |
| abstract_inverted_index.strategically | 47 |
| abstract_inverted_index.delocalization | 96 |
| abstract_inverted_index.hybridizations | 103 |
| abstract_inverted_index.simultaneously | 19 |
| abstract_inverted_index.electrocatalyst | 137 |
| abstract_inverted_index.rate‐limiting | 117 |
| abstract_inverted_index.zeolite‐based | 183 |
| abstract_inverted_index.‐to‐formate | 31 |
| abstract_inverted_index.electrocatalysis | 198 |
| abstract_inverted_index.electrocatalysts | 184 |
| abstract_inverted_index.electrocatalytic | 125 |
| abstract_inverted_index.electrosynthesis | 7, 189 |
| abstract_inverted_index.implementations. | 39 |
| abstract_inverted_index.industrial‐level | 140, 186 |
| cited_by_percentile_year.max | 100 |
| cited_by_percentile_year.min | 90 |
| corresponding_author_ids | https://openalex.org/A5061368050, https://openalex.org/A5100784984, https://openalex.org/A5036892042, https://openalex.org/A5100390167 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I143593769, https://openalex.org/I149240348, https://openalex.org/I151746483, https://openalex.org/I17145004, https://openalex.org/I180585399, https://openalex.org/I19820366, https://openalex.org/I4210156066 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.8500000238418579 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile.value | 0.88532784 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |