Constructing Ag/Cu 2 O Interface for Efficient Neutral CO 2 Electroreduction to C 2 H 4 Article Swipe
Zongnan Wei
,
Wenwen Wang
,
Tao Shao
,
Shuaibing Yang
,
Chang Liu
,
Duan‐Hui Si
,
Rong Cao
,
Minna Cao
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202417066
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202417066
Neutral CO 2 electroreduction to multi‐carbons (C 2+ ) offers a promising pathway to reduce the CO 2 and energy losses originating from the carbonate formation. However, the sluggish kinetics of C−C coupling brings a significant challenge of achieving high selectivity of a single product (such as ethylene), especially at industrial‐relevant current densities (>300 mA cm −2 ). Here, we reported an optimized Ag‐Cu 2 O interfacial catalyst that exhibited C 2+ Faradaic efficiency (FE) of 73.6 % at 650 mA cm −2 in a flow cell. Remarkably, it obtained FE C2H4 of 66.0 % with a partial current density of 429.1 mA cm −2 , making it stand out among the reported Cu‐based electrocatalysts. In situ Raman spectra uncovered that the Ag/Cu 2 O interfaces enabled a high coverage of *CO around the partially reduced Cu + /Cu 0 active sites. Furthermore, theoretical calculations demonstrated the enhanced CO formation and C−C coupling at the Ag/Cu 2 O interface. This work reported an unprecedented neutral CO 2 electroreduction to C 2 H 4 performance and provided an in‐depth comprehension of the role of the bimetallic interface.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/ange.202417066
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/ange.202417066
- OA Status
- bronze
- Cited By
- 4
- References
- 61
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4403870560
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- OpenAlex ID
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https://openalex.org/W4403870560Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/ange.202417066Digital Object Identifier
- Title
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Constructing Ag/Cu 2 O Interface for Efficient Neutral CO 2 Electroreduction to C 2 H 4Work title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-10-29Full publication date if available
- Authors
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Zongnan Wei, Wenwen Wang, Tao Shao, Shuaibing Yang, Chang Liu, Duan‐Hui Si, Rong Cao, Minna CaoList of authors in order
- Landing page
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https://doi.org/10.1002/ange.202417066Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/ange.202417066Direct link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/ange.202417066Direct OA link when available
- Concepts
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Interface (matter), Chemistry, Electrochemistry, Materials science, Inorganic chemistry, Nanotechnology, Combinatorial chemistry, Electrode, Molecule, Physical chemistry, Organic chemistry, Gibbs isothermTop concepts (fields/topics) attached by OpenAlex
- Cited by
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4Total citation count in OpenAlex
- Citations by year (recent)
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2025: 4Per-year citation counts (last 5 years)
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61Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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