Constructing Rich Interfacial Structure by Carbon Dots to Improve the Sodium Storage Capacity of Sb/C Composite Article Swipe
Xue Zhong
,
Jiaming Duan
,
Yinger Xiang
,
Xinyu Hu
,
Yujie Huang
,
Yujin Li
,
Wentao Deng
,
Guoqiang Zou
,
Hongshuai Hou
,
Xiaobo Ji
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202306574
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202306574
Designing Sb/carbon composite is an effective strategy to enhance the cycle stability and rate capability of Sb anodes for sodium ion batteries. However, the introduction of carbon often leads to a loss in specific capacity and initial Coulombic efficiency (ICE). In this work, a new perspective is adopted by focusing on improving the “sloping capacity” contribution of carbon (C) in Sb/C composites, rather than solely increasing the platform capacity of Sb as traditionally done. Theoretical predictions indicate that constructing Sb/C composites with high Sb and carbon interfacial areas can provide more Na adsorption sites, thus enhancing the “sloping capacity” of amorphous carbon. Guided by DFT, a rational Sb/C/NSCDs‐2(N) is successfully developed by self‐embedding Sb nanodots into 2D‐amorphous carbon sheets doped with N/S. Sb/C/NSCDs‐2(N) exhibits abundant Sb/carbon interfacial areas and excellent nanoscale effects, demonstrating ideal electrochemical sodium storage performances. Impressively, the Sb/C/NSCDs‐2(N) provides a “sloping capacity” close to 160 mAh g −1 . Significantly, owing to the fact that these interfaces and defects are not in direct contact with the electrolyte, the side reaction of electrolyte is effectively inhibited, leading to no decrease of ICE.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adfm.202306574
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202306574
- OA Status
- bronze
- Cited By
- 38
- References
- 55
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4386806946
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- OpenAlex ID
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https://openalex.org/W4386806946Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/adfm.202306574Digital Object Identifier
- Title
-
Constructing Rich Interfacial Structure by Carbon Dots to Improve the Sodium Storage Capacity of Sb/C CompositeWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-09-15Full publication date if available
- Authors
-
Xue Zhong, Jiaming Duan, Yinger Xiang, Xinyu Hu, Yujie Huang, Yujin Li, Wentao Deng, Guoqiang Zou, Hongshuai Hou, Xiaobo JiList of authors in order
- Landing page
-
https://doi.org/10.1002/adfm.202306574Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202306574Direct link to full text PDF
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YesWhether a free full text is available
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-
bronzeOpen access status per OpenAlex
- OA URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202306574Direct OA link when available
- Concepts
-
Materials science, Composite number, Carbon fibers, Amorphous carbon, Chemical engineering, Faraday efficiency, Amorphous solid, Electrochemistry, Nanotechnology, Adsorption, Electrolyte, Monolayer, Anode, Composite material, Electrode, Organic chemistry, Physical chemistry, Engineering, ChemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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38Total citation count in OpenAlex
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2025: 13, 2024: 24, 2023: 1Per-year citation counts (last 5 years)
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55Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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