Control of the third dimension in copper-based square-lattice antiferromagnets Article Swipe
Paul Goddard
,
John Singleton
,
Isabel Franke
,
Johannes S. Möller
,
Tom Lancaster
,
Andrew J. Steele
,
Craig V. Topping
,
Stephen J. Blundell
,
F. L. Pratt
,
C. Baines
,
Jesper Bendix
,
R. McDonald
,
Jamie Brambleby
,
M. R. Lees
,
Saul H. Lapidus
,
Peter W. Stephens
,
Brendan Twamley
,
Marianne M. Conner
,
Kylee Funk
,
Jordan F. Corbey
,
Hope E. Tran
,
John A. Schlueter
,
Jamie L. Manson
·
YOU?
·
· 2016
· Open Access
·
· DOI: https://doi.org/10.1103/physrevb.93.094430
YOU?
·
· 2016
· Open Access
·
· DOI: https://doi.org/10.1103/physrevb.93.094430
Using a mixed-ligand synthetic scheme, we create a family of quasi-two-dimensional antiferromagnets, namely, [Cu(HF2)(pyz)2]ClO4 [pyz = pyrazine], [CuL2(pyz)2](ClO4)2 [L = pyO = pyridine-N-oxide and 4-phpy-O = 4-phenylpyridine-N-oxide. These materials are shown to possess equivalent two-dimensional [Cu(pyz)2]2+ nearly square layers, but exhibit interlayer spacings that vary from 6.5713 to 16.777 Å, as dictated by the axial ligands. We present the structural and magnetic properties of this family as determined via x-ray diffraction, electron-spin resonance, pulsed- and quasistatic-field magnetometry and muon-spin rotation, and compare them to those of the prototypical two-dimensional magnetic polymer Cu(pyz)2(ClO4)2. We find that, within the limits of the experimental error, the two-dimensional, intralayer exchange coupling in our family of materials remains largely unaffected by the axial ligand substitution, while the observed magnetic ordering temperature (1.91 K for the material with the HF2 axial ligand, 1.70 K for the pyO and 1.63 K for the 4-phpy-O) decreases slowly with increasing layer separation. Despite the structural motifs common to this family and Cu(pyz)2(ClO4)2, the latter has significantly stronger two-dimensional exchange interactions and hence a higher ordering temperature. Here, we discuss these results, as well as the mechanisms that might drive the long-range order in these materials, in terms of departures from the ideal S = 1/2 two-dimensional square-lattice Heisenberg antiferromagnet. In particular, we find that both spin-exchange anisotropy in the intralayer interaction and interlayer couplings (exchange, dipolar, or both) are needed to account for the observed ordering temperatures, with the intralayer anisotropy becoming more important as the layers are pulled further apart.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1103/physrevb.93.094430
- http://link.aps.org/pdf/10.1103/PhysRevB.93.094430
- OA Status
- bronze
- Cited By
- 19
- References
- 65
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2289918054
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W2289918054Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1103/physrevb.93.094430Digital Object Identifier
- Title
-
Control of the third dimension in copper-based square-lattice antiferromagnetsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2016Year of publication
- Publication date
-
2016-03-25Full publication date if available
- Authors
-
Paul Goddard, John Singleton, Isabel Franke, Johannes S. Möller, Tom Lancaster, Andrew J. Steele, Craig V. Topping, Stephen J. Blundell, F. L. Pratt, C. Baines, Jesper Bendix, R. McDonald, Jamie Brambleby, M. R. Lees, Saul H. Lapidus, Peter W. Stephens, Brendan Twamley, Marianne M. Conner, Kylee Funk, Jordan F. Corbey, Hope E. Tran, John A. Schlueter, Jamie L. MansonList of authors in order
- Landing page
-
https://doi.org/10.1103/physrevb.93.094430Publisher landing page
- PDF URL
-
https://link.aps.org/pdf/10.1103/PhysRevB.93.094430Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
bronzeOpen access status per OpenAlex
- OA URL
-
https://link.aps.org/pdf/10.1103/PhysRevB.93.094430Direct OA link when available
- Concepts
-
Pyrazine, Antiferromagnetism, Chemistry, Crystallography, Condensed matter physics, Lattice (music), Anisotropy, Exchange interaction, Copper, Ferromagnetism, Physics, Stereochemistry, Organic chemistry, Acoustics, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
19Total citation count in OpenAlex
- Citations by year (recent)
-
2023: 3, 2022: 1, 2021: 2, 2020: 5, 2019: 3Per-year citation counts (last 5 years)
- References (count)
-
65Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| institutions_distinct_count | 23 |
| citation_normalized_percentile.value | 0.76028317 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |