Controlled quantum well formation on DNA-wrapped carbon nanotubes via peroxide-mediated aryl diazonium reduction Article Swipe
Stanislav Piletsky
,
Erin Keblish
,
Daniel A. Heller
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2024-8f3jf-v3
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2024-8f3jf-v3
Quantum well defect-modified single walled carbon nanotubes are environmentally sensitive nanomaterials with wide-ranging applications in biosensing, imaging, light harvesting, quantum computing, energy storage and catalysis. The most common method for covalent functionalization of nanotubes for biosensing applications involves reactions with aryl diazonium salts to generate sp3 aryl defect sites, commonly followed by wrapping with single stranded DNA. We describe herein a rapid aryl diazonium functionalization reaction directly compatible with DNA-wrapped nanotubes. The reaction uses mild aqueous conditions at physiological pH and can be easily monitored in real-time via fluorescence analysis to control the degree of functionalization. Overall, this reaction greatly simplifies the production of covalently functionalized DNA-wrapped carbon nanotubes, expanding their potential for industrial and biomedical applications.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.26434/chemrxiv-2024-8f3jf-v3
- OA Status
- gold
- Cited By
- 1
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W4402814734Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.26434/chemrxiv-2024-8f3jf-v3Digital Object Identifier
- Title
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Controlled quantum well formation on DNA-wrapped carbon nanotubes via peroxide-mediated aryl diazonium reductionWork title
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-09-25Full publication date if available
- Authors
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Stanislav Piletsky, Erin Keblish, Daniel A. HellerList of authors in order
- Landing page
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https://doi.org/10.26434/chemrxiv-2024-8f3jf-v3Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://doi.org/10.26434/chemrxiv-2024-8f3jf-v3Direct OA link when available
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Aryl, Peroxide, Carbon nanotube, Reduction (mathematics), Chemistry, DNA, Photochemistry, Materials science, Nanotechnology, Polymer chemistry, Organic chemistry, Biochemistry, Alkyl, Geometry, MathematicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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1Total citation count in OpenAlex
- Citations by year (recent)
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2025: 1Per-year citation counts (last 5 years)
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.their | 110 |
| abstract_inverted_index.carbon | 5, 107 |
| abstract_inverted_index.common | 27 |
| abstract_inverted_index.defect | 47 |
| abstract_inverted_index.degree | 93 |
| abstract_inverted_index.easily | 83 |
| abstract_inverted_index.energy | 21 |
| abstract_inverted_index.herein | 59 |
| abstract_inverted_index.method | 28 |
| abstract_inverted_index.single | 3, 54 |
| abstract_inverted_index.sites, | 48 |
| abstract_inverted_index.walled | 4 |
| abstract_inverted_index.Quantum | 0 |
| abstract_inverted_index.aqueous | 75 |
| abstract_inverted_index.control | 91 |
| abstract_inverted_index.greatly | 99 |
| abstract_inverted_index.quantum | 19 |
| abstract_inverted_index.storage | 22 |
| abstract_inverted_index.Overall, | 96 |
| abstract_inverted_index.analysis | 89 |
| abstract_inverted_index.commonly | 49 |
| abstract_inverted_index.covalent | 30 |
| abstract_inverted_index.describe | 58 |
| abstract_inverted_index.directly | 66 |
| abstract_inverted_index.followed | 50 |
| abstract_inverted_index.generate | 44 |
| abstract_inverted_index.imaging, | 16 |
| abstract_inverted_index.involves | 37 |
| abstract_inverted_index.reaction | 65, 72, 98 |
| abstract_inverted_index.stranded | 55 |
| abstract_inverted_index.wrapping | 52 |
| abstract_inverted_index.diazonium | 41, 63 |
| abstract_inverted_index.expanding | 109 |
| abstract_inverted_index.monitored | 84 |
| abstract_inverted_index.nanotubes | 6, 33 |
| abstract_inverted_index.potential | 111 |
| abstract_inverted_index.reactions | 38 |
| abstract_inverted_index.real-time | 86 |
| abstract_inverted_index.sensitive | 9 |
| abstract_inverted_index.biomedical | 115 |
| abstract_inverted_index.biosensing | 35 |
| abstract_inverted_index.catalysis. | 24 |
| abstract_inverted_index.compatible | 67 |
| abstract_inverted_index.computing, | 20 |
| abstract_inverted_index.conditions | 76 |
| abstract_inverted_index.covalently | 104 |
| abstract_inverted_index.industrial | 113 |
| abstract_inverted_index.nanotubes, | 108 |
| abstract_inverted_index.nanotubes. | 70 |
| abstract_inverted_index.production | 102 |
| abstract_inverted_index.simplifies | 100 |
| abstract_inverted_index.DNA-wrapped | 69, 106 |
| abstract_inverted_index.biosensing, | 15 |
| abstract_inverted_index.harvesting, | 18 |
| abstract_inverted_index.applications | 13, 36 |
| abstract_inverted_index.fluorescence | 88 |
| abstract_inverted_index.wide-ranging | 12 |
| abstract_inverted_index.applications. | 116 |
| abstract_inverted_index.nanomaterials | 10 |
| abstract_inverted_index.physiological | 78 |
| abstract_inverted_index.functionalized | 105 |
| abstract_inverted_index.defect-modified | 2 |
| abstract_inverted_index.environmentally | 8 |
| abstract_inverted_index.functionalization | 31, 64 |
| abstract_inverted_index.functionalization. | 95 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 91 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 3 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/12 |
| sustainable_development_goals[0].score | 0.46000000834465027 |
| sustainable_development_goals[0].display_name | Responsible consumption and production |
| citation_normalized_percentile.value | 0.59076346 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |