Creating a Ferromagnetic Ground State with Tc Above Room Temperature in a Paramagnetic Alloy through Non‐Equilibrium Nanostructuring Article Swipe
Xinglong Ye
,
Nuno M. Fortunato
,
Abhishek Sarkar
,
Holger Geßwein
,
Di Wang
,
Xiang Chen
,
Benedikt Eggert
,
Heiko Wende
,
Richard A. Brand
,
Hongbin Zhang
,
Horst Hahn
,
Robert Kruk
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202108793
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202108793
Materials with strong magnetostructural coupling have complex energy landscapes featuring multiple local ground states, thus making it possible to switch among distinct magnetic‐electronic properties. However, these energy minima are rarely accessible by a mere application of an external stimuli to the system in equilibrium state. A ferromagnetic ground state, with T c above room temperature, can be created in an initially paramagnetic alloy by nonequilibrium nanostructuring. By a dealloying process, bulk chemically disordered FeRh alloys are transformed into a nanoporous structure with the topology of a few nanometer‐sized ligaments and nodes. Magnetometry and Mössbauer spectroscopy reveal the coexistence of two magnetic ground states, a conventional low‐temperature spin‐glass and a hitherto‐unknown robust ferromagnetic phase. The emergence of the ferromagnetic phase is validated by density functional theory calculations showing that local tetragonal distortion induced by surface stress favors ferromagnetic ordering. The study provides a means for reaching conventionally inaccessible magnetic states, resulting in a complete on/off ferromagnetic–paramagnetic switching over a broad temperature range.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202108793
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202108793
- OA Status
- hybrid
- Cited By
- 5
- References
- 59
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3215141239
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3215141239Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202108793Digital Object Identifier
- Title
-
Creating a Ferromagnetic Ground State with Tc Above Room Temperature in a Paramagnetic Alloy through Non‐Equilibrium NanostructuringWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2021Year of publication
- Publication date
-
2021-12-01Full publication date if available
- Authors
-
Xinglong Ye, Nuno M. Fortunato, Abhishek Sarkar, Holger Geßwein, Di Wang, Xiang Chen, Benedikt Eggert, Heiko Wende, Richard A. Brand, Hongbin Zhang, Horst Hahn, Robert KrukList of authors in order
- Landing page
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https://doi.org/10.1002/adma.202108793Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202108793Direct link to full text PDF
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YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202108793Direct OA link when available
- Concepts
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Ferromagnetism, Materials science, Paramagnetism, Condensed matter physics, Ground state, Tetragonal crystal system, Alloy, Magnetometer, Phase (matter), Magnetic field, Physics, Metallurgy, Atomic physics, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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5Total citation count in OpenAlex
- Citations by year (recent)
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2025: 1, 2024: 1, 2023: 2, 2022: 1Per-year citation counts (last 5 years)
- References (count)
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59Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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