Creating Reactivity with Unstable Endmembers using Pressure and Temperature: Synthesis of Bulk Cubic Mg0.4Fe0.6N Article Swipe
George Serghiou
,
Gang Ji
,
Nicholas Odling
,
H. J. Reichmann
,
J. P. Morniroli
,
R. Boehler
,
D. J. Frost
,
Jonathan P. Wright
,
Bernd Wunder
·
YOU?
·
· 2015
· Open Access
·
· DOI: https://doi.org/10.1002/anie.201506257
YOU?
·
· 2015
· Open Access
·
· DOI: https://doi.org/10.1002/anie.201506257
Alloy and nitride solid solutions are prominent for structural, energy and information processing applications. There are frequently however barriers to making them. We remove barriers to reactivity here using pressure with a new synthetic approach. We target pressures where the reasons for cubic endmember nitride instability can become the driving force for cubic nitride solid solution stability. Using this approach we form a novel rocksalt Mg 0.4 Fe 0.6 N solid solution at between 15 and 23 GPa and up to 2500 K. This is a system where, neither an alloy nor a nitride solid solution form at ambient conditions and bulk MgN and FeN endmembers do not form, either at ambient or at high pressure. The new nitride is formed, by removing endmember lattice mismatch with pressure, allowing a stabilizing redistribution of valence electrons upon heating. This approach can be employed for a range of normally unreactive systems. Mg, Fe and enhanced nitrogen presence, may also indicate a richer reaction chemistry in our planets interior.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/anie.201506257
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.201506257
- OA Status
- bronze
- Cited By
- 10
- References
- 46
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W1890698080
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W1890698080Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/anie.201506257Digital Object Identifier
- Title
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Creating Reactivity with Unstable Endmembers using Pressure and Temperature: Synthesis of Bulk Cubic Mg0.4Fe0.6NWork title
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articleOpenAlex work type
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enPrimary language
- Publication year
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2015Year of publication
- Publication date
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2015-10-28Full publication date if available
- Authors
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George Serghiou, Gang Ji, Nicholas Odling, H. J. Reichmann, J. P. Morniroli, R. Boehler, D. J. Frost, Jonathan P. Wright, Bernd WunderList of authors in order
- Landing page
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https://doi.org/10.1002/anie.201506257Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.201506257Direct link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.201506257Direct OA link when available
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Reactivity (psychology), Materials science, Mineralogy, Chemistry, Pathology, Medicine, Alternative medicineTop concepts (fields/topics) attached by OpenAlex
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10Total citation count in OpenAlex
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2025: 3, 2024: 1, 2023: 1, 2021: 4, 2016: 1Per-year citation counts (last 5 years)
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46Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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