Decamethylferrocene oxidation at interdigitated microband array electrodes in the absence of intentionally added supporting electrolyte: experiment versus finite element model Article Swipe
Tingran Liu
,
Katarzyna Dusiło
,
Marcin Opałło
,
Evaldo B. Carneiro‐Neto
,
Ernesto C. Pereira
,
James E. Taylor
,
Frank Marken
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1007/s44373-025-00032-y
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1007/s44373-025-00032-y
The one-electron oxidation of decamethylferrocene (FeCp* 2 ) in the absence of added supporting electrolyte is investigated as a model redox system in acetonitrile to shed new light onto (i) the effect of added supporting electrolyte and (ii) the impact of using two-electrode versus three-electrode configurations for interdigitated array electrodes. Electrochemical processes at interdigitated microband array electrodes (anode and cathode each 250 platinum bands, 5 μm width, 5 μm gap) are investigated with the aim to explore self-supported processes for electrosynthesis in the absence of added supporting electrolyte. Two types of steady state and the corresponding time to steady state are discussed. When working without added supporting electrolyte, finite element theory predicts current doubling and a marked change in concentration profiles. Implications for electrosynthesis at interdigitated microband electrodes are summarised. Graphical Abstract
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1007/s44373-025-00032-y
- https://link.springer.com/content/pdf/10.1007/s44373-025-00032-y.pdf
- OA Status
- diamond
- References
- 23
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4410497146
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4410497146Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1007/s44373-025-00032-yDigital Object Identifier
- Title
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Decamethylferrocene oxidation at interdigitated microband array electrodes in the absence of intentionally added supporting electrolyte: experiment versus finite element modelWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-05-19Full publication date if available
- Authors
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Tingran Liu, Katarzyna Dusiło, Marcin Opałło, Evaldo B. Carneiro‐Neto, Ernesto C. Pereira, James E. Taylor, Frank MarkenList of authors in order
- Landing page
-
https://doi.org/10.1007/s44373-025-00032-yPublisher landing page
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https://link.springer.com/content/pdf/10.1007/s44373-025-00032-y.pdfDirect link to full text PDF
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YesWhether a free full text is available
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diamondOpen access status per OpenAlex
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https://link.springer.com/content/pdf/10.1007/s44373-025-00032-y.pdfDirect OA link when available
- Concepts
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Electrolyte, Electrode, Finite element method, Materials science, Chemistry, Engineering, Structural engineering, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
- References (count)
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23Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.processes | 52, 79 |
| abstract_inverted_index.profiles. | 121 |
| abstract_inverted_index.discussed. | 102 |
| abstract_inverted_index.electrodes | 57, 128 |
| abstract_inverted_index.supporting | 14, 35, 87, 107 |
| abstract_inverted_index.electrodes. | 50 |
| abstract_inverted_index.electrolyte | 15, 36 |
| abstract_inverted_index.summarised. | 130 |
| abstract_inverted_index.Implications | 122 |
| abstract_inverted_index.acetonitrile | 24 |
| abstract_inverted_index.electrolyte, | 108 |
| abstract_inverted_index.electrolyte. | 88 |
| abstract_inverted_index.investigated | 17, 72 |
| abstract_inverted_index.one-electron | 2 |
| abstract_inverted_index.concentration | 120 |
| abstract_inverted_index.corresponding | 96 |
| abstract_inverted_index.two-electrode | 43 |
| abstract_inverted_index.configurations | 46 |
| abstract_inverted_index.interdigitated | 48, 54, 126 |
| abstract_inverted_index.self-supported | 78 |
| abstract_inverted_index.Electrochemical | 51 |
| abstract_inverted_index.three-electrode | 45 |
| abstract_inverted_index.electrosynthesis | 81, 124 |
| abstract_inverted_index.decamethylferrocene | 5 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 7 |
| citation_normalized_percentile.value | 0.19107593 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |