Defect-assisted reversible phase transition in mono- and few-layer ReS2 Article Swipe
George Zograf
,
Andrew B. Yankovich
,
Betül Küçüköz
,
Abhay V. Agrawal
,
Alexander Yu. Polyakov
,
Joachim Ciers
,
Fredrik Eriksson
,
Åsa Haglund
,
Paul Erhart
,
Tomasz J. Antosiewicz
,
Eva Olsson
,
Timur Shegai
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41699-025-00524-w
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41699-025-00524-w
2D transition metal dichalcogenide (TMD) materials have attracted interest due to their remarkable excitonic, optical, electrical, and mechanical properties, which are dependent on their crystal structure. Consequently, controlling the crystal structure of these materials is essential for fine-tuning their performance, e.g., linear and nonlinear optical, as well as charge transport properties. While various phase-switching TMD materials are available, their transitions are often irreversible. Here, we investigate the mechanism of a light-induced reversible phase transition in mono- and bilayer rhenium disulfide (ReS 2 ). Our observations, based on transmission electron microscopy, nonlinear spectroscopy, and density functional theory, reveal a transition from the ground $${\rm{T}}^{\prime\prime}$$ (double-distorted T) to the metastable $${\rm{H}}^{\prime}$$ (distorted H) phase under femtosecond laser irradiation or influence of highly-energetic electrons. We show that the formation of sulfur vacancies facilitates this phenomenon. Our findings pave the way toward manipulating the crystal structure of ReS 2 and possibly its heterostructures.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41699-025-00524-w
- https://www.nature.com/articles/s41699-025-00524-w.pdf
- OA Status
- gold
- Cited By
- 1
- References
- 100
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4406319829
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https://openalex.org/W4406319829Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41699-025-00524-wDigital Object Identifier
- Title
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Defect-assisted reversible phase transition in mono- and few-layer ReS2Work title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-01-13Full publication date if available
- Authors
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George Zograf, Andrew B. Yankovich, Betül Küçüköz, Abhay V. Agrawal, Alexander Yu. Polyakov, Joachim Ciers, Fredrik Eriksson, Åsa Haglund, Paul Erhart, Tomasz J. Antosiewicz, Eva Olsson, Timur ShegaiList of authors in order
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https://doi.org/10.1038/s41699-025-00524-wPublisher landing page
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https://www.nature.com/articles/s41699-025-00524-w.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41699-025-00524-w.pdfDirect OA link when available
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Phase transition, Materials science, Phase (matter), Crystal (programming language), Crystallography, Chemistry, Physics, Thermodynamics, Computer science, Organic chemistry, Programming languageTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2025: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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