Defect-enabled fast gas encapsulation into water lattices for innovative energy storage and decarbonization Article Swipe

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Ngoc N. Nguyen , Mirza Galib , Anh V. Nguyen , Zhenyuan Yin ·

YOU? · · 2024 · Open Access · · DOI: https://doi.org/10.26434/chemrxiv-2024-bjv6f

Non-polar gases do not mix well with liquid water, but they can be incorporated massively in solid water lattices and create gas-carrying water structures called gas hydrates. Nature showcases this extraordinary gas/water incorporation through multi-trillion tones of methane solidified in natural hydrates on seafloors. Laboratory experiments successfully produced gas hydrates containing ~5 wt% of hydrogen, 15 wt% of methane, and 30 wt% of CO2. Such water-based gas carriers hold great promise for energy storage and CO2 sequestration, taking the advantages of water as a sustainable feedstock. However, the slow gas encapsulation in water lattices hinders real-world applications. We present a novel defect-engineering concept for tailoring gas uptake in water lattices. We elaborate microscopic views of dopant-induced defects in water lattices, reveal an intrinsic link between the engineered defects and gas encapsulation kinetics, and provide a path-opening concept of defect engineering for efficient gas encapsulation in solid water lattices for energy storage and decarbonization applications.

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Methane Encapsulation (networking) Materials science Natural gas Chemical engineering Nanotechnology Chemistry Computer science Organic chemistry Engineering Computer network

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Type: preprint
Language: en
Landing Page: https://doi.org/10.26434/chemrxiv-2024-bjv6f
OA Status: gold
Related Works: 10
OpenAlex ID: https://openalex.org/W4405323591

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DOI: https://doi.org/10.26434/chemrxiv-2024-bjv6f

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Title: Defect-enabled fast gas encapsulation into water lattices for innovative energy storage and decarbonization

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Type: preprint

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Language: en

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Publication year: 2024

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Publication date: 2024-12-12

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Authors: Ngoc N. Nguyen, Mirza Galib, Anh V. Nguyen, Zhenyuan Yin

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Landing page: https://doi.org/10.26434/chemrxiv-2024-bjv6f

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OA status: gold

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OA URL: https://doi.org/10.26434/chemrxiv-2024-bjv6f

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Concepts: Methane, Encapsulation (networking), Materials science, Natural gas, Chemical engineering, Nanotechnology, Chemistry, Computer science, Organic chemistry, Engineering, Computer network

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Cited by: 0

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