Dehydrogenation of Cycloalkanes over N-Doped Carbon-Supported Catalysts: The Effects of Active Component and Molecular Structure of the Substrate Article Swipe
Jian Wang
,
He Liu
,
Shiguang Fan
,
Shuai Wang
,
Guanjun Xu
,
Aijun Guo
,
Zongxian Wang
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.3390/nano11112846
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.3390/nano11112846
Efficient dehydrogenation of cycloalkanes under mild conditions is the key to large-scale application of cycloalkanes as a hydrogen storage medium. In this paper, a series of active metals loaded on nitrogen-doped carbon (M/CN, M = Pt, Pd, Ir, Rh, Au, Ru, Ag, Ni, Cu) were prepared to learn the role of active metals in cycloalkane dehydrogenation with cyclohexane as the model reactant. Only Pt/CN, Pd/CN, Rh/CN and Ir/CN can catalyze the dehydrogenation of cyclohexane under the set conditions. Among them, Pt/CN exhibited the best catalytic activity with the TOF value of 269.32 h−1 at 180 °C, followed by Pd/CN, Rh/CN and Ir/CN successively. More importantly, the difference of catalytic activity between these active metals diminishes with the increase in temperature. This implies that there is a thermodynamic effect of cyclohexane dehydrogenation with the synthetic catalysts, which was evidenced by the study on the activation energy. In addition, the effects of molecular structure on cycloalkane dehydrogenation catalyzed by Pt/CN were studied. The results reveal that cycloalkane dehydrogenation activity and hydrogen production rate can be enhanced by optimizing the type, quantity and position of alkyl substituents on cyclohexane.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/nano11112846
- https://www.mdpi.com/2079-4991/11/11/2846/pdf?version=1635234073
- OA Status
- gold
- Cited By
- 6
- References
- 42
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3208362675
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3208362675Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/nano11112846Digital Object Identifier
- Title
-
Dehydrogenation of Cycloalkanes over N-Doped Carbon-Supported Catalysts: The Effects of Active Component and Molecular Structure of the SubstrateWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2021Year of publication
- Publication date
-
2021-10-26Full publication date if available
- Authors
-
Jian Wang, He Liu, Shiguang Fan, Shuai Wang, Guanjun Xu, Aijun Guo, Zongxian WangList of authors in order
- Landing page
-
https://doi.org/10.3390/nano11112846Publisher landing page
- PDF URL
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https://www.mdpi.com/2079-4991/11/11/2846/pdf?version=1635234073Direct link to full text PDF
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://www.mdpi.com/2079-4991/11/11/2846/pdf?version=1635234073Direct OA link when available
- Concepts
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Dehydrogenation, Cycloalkane, Cyclohexane, Catalysis, Alkyl, Chemistry, Substrate (aquarium), Inorganic chemistry, Hydrogen, Materials science, Organic chemistry, Oceanography, GeologyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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6Total citation count in OpenAlex
- Citations by year (recent)
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2024: 2, 2023: 3, 2021: 1Per-year citation counts (last 5 years)
- References (count)
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42Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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