Delamination-Assisted Ultrafast Wrinkle Formation in a Freestanding Film Article Swipe
Yifan Su
,
Alfred Zong
,
Anshul Kogar
,
Di Lu
,
Seung Sae Hong
,
Byron Freelon
,
Timm Rohwer
,
Bai Yang Wang
,
Harold Y. Hwang
,
Nuh Gedik
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/acs.nanolett.3c02898
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/acs.nanolett.3c02898
Freestanding films provide a versatile platform for materials engineering thanks to additional structural motifs not found in films with a substrate. A ubiquitous example is wrinkles, yet little is known about how they can develop over as fast as a few picoseconds due to a lack of experimental probes to visualize their dynamics in real time on the nanoscopic scale. Here, we use time-resolved electron diffraction to directly observe light-activated wrinkling formation in freestanding La2/3Ca1/3MnO3 films. Via a "lock-in" analysis of oscillations in the diffraction peak position, intensity, and width, we quantitatively reconstructed how wrinkles develop on the time scale of lattice vibration. Contrary to the common assumption of fixed boundary conditions, we found that wrinkle development is associated with ultrafast delamination at the film boundaries. Our work provides a generic protocol to quantify wrinkling dynamics in freestanding films and highlights the importance of the film-substrate interaction in determining the properties of freestanding structures.
Related Topics
Concepts
Wrinkle
Delamination (geology)
Materials science
Ultrashort pulse
Composite material
Nanotechnology
Optics
Laser
Physics
Subduction
Tectonics
Biology
Paleontology
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.nanolett.3c02898
- OA Status
- green
- Cited By
- 9
- References
- 46
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4388868387
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4388868387Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.nanolett.3c02898Digital Object Identifier
- Title
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Delamination-Assisted Ultrafast Wrinkle Formation in a Freestanding FilmWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-11-21Full publication date if available
- Authors
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Yifan Su, Alfred Zong, Anshul Kogar, Di Lu, Seung Sae Hong, Byron Freelon, Timm Rohwer, Bai Yang Wang, Harold Y. Hwang, Nuh GedikList of authors in order
- Landing page
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https://doi.org/10.1021/acs.nanolett.3c02898Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
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https://www.osti.gov/biblio/2404889Direct OA link when available
- Concepts
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Wrinkle, Delamination (geology), Materials science, Ultrashort pulse, Composite material, Nanotechnology, Optics, Laser, Physics, Subduction, Tectonics, Biology, PaleontologyTop concepts (fields/topics) attached by OpenAlex
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9Total citation count in OpenAlex
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2025: 6, 2024: 2, 2023: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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