Delamination-assisted ultrafast wrinkle formation in a freestanding film Article Swipe
Yifan Su
,
Alfred Zong
,
Anshul Kogar
,
Di Lu
,
Seung Sae Hong
,
Byron Freelon
,
Timm Rohwer
,
Harold Y. Hwang
,
Nuh Gedik
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2212.12082
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2212.12082
The ability to synthesize and control two-dimensional (2D) crystals creates numerous opportunities for studying emergent states of matter and their novel functionalities. Freestanding films provide a particularly versatile platform for materials engineering in 2D thanks to additional structural motifs not found in films adhered to a flat substrate. A ubiquitous example is wrinkles, yet little is known about how they can develop over as fast as a few picoseconds due to a lack of experimental probes to visualize their dynamics in real time at the nanoscopic scale. Here, we use ultrafast electron diffraction to directly observe light-activated wrinkling formation in a freestanding La$_{2/3}$Ca$_{1/3}$MnO$_3$ film. Via a ``lock-in'' analysis of a single mode of oscillation in the diffraction peak position, intensity, and width, we are able to quantitatively reconstruct how wrinkles develop at the picosecond timescale. Contrary to the common assumption of a fixed boundary condition for freestanding films, we found that wrinkle development is associated with ultrafast delamination at the contact point between the film boundary and the underlying substrate, avoiding a strain build-up in the film. Not only does our work provide a generic protocol to quantify wrinkling dynamics in freestanding films, it also highlights the importance of film-substrate interaction for determining the properties of freestanding structures.
Related Topics
Concepts
Picosecond
Materials science
Delamination (geology)
Ultrashort pulse
Nanoscopic scale
Substrate (aquarium)
Wrinkle
Diffraction
Bridging (networking)
Nanotechnology
Oscillation (cell signaling)
Optoelectronics
Composite material
Optics
Computer science
Laser
Physics
Chemistry
Computer network
Geology
Biology
Oceanography
Paleontology
Subduction
Biochemistry
Tectonics
Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2212.12082
- https://arxiv.org/pdf/2212.12082
- OA Status
- green
- References
- 46
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4312206074
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4312206074Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.48550/arxiv.2212.12082Digital Object Identifier
- Title
-
Delamination-assisted ultrafast wrinkle formation in a freestanding filmWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
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2022Year of publication
- Publication date
-
2022-12-22Full publication date if available
- Authors
-
Yifan Su, Alfred Zong, Anshul Kogar, Di Lu, Seung Sae Hong, Byron Freelon, Timm Rohwer, Harold Y. Hwang, Nuh GedikList of authors in order
- Landing page
-
https://arxiv.org/abs/2212.12082Publisher landing page
- PDF URL
-
https://arxiv.org/pdf/2212.12082Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://arxiv.org/pdf/2212.12082Direct OA link when available
- Concepts
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Picosecond, Materials science, Delamination (geology), Ultrashort pulse, Nanoscopic scale, Substrate (aquarium), Wrinkle, Diffraction, Bridging (networking), Nanotechnology, Oscillation (cell signaling), Optoelectronics, Composite material, Optics, Computer science, Laser, Physics, Chemistry, Computer network, Geology, Biology, Oceanography, Paleontology, Subduction, Biochemistry, TectonicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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46Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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