Desorption electrospray ionization mass spectrometry imaging of latent fingerprints revealed by Oil Red O Article Swipe
Mariska Banidol
,
Sophia Kouider
,
Isaure Sergent
,
Hélène Pizzala
,
Laurence Charles
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/rcm.9724
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/rcm.9724
Mass spectrometry imaging (MSI) is increasingly used to produce chemical images of latent fingerprints. Yet, the actual benefits of MSI for real case studies have to be assessed for fingerprints previously processed by forensic techniques. Here, we have evaluated the compatibility of desorption electrospray ionization (DESI) with the fingerprint enhancement technique involving Oil Red O (ORO). Methods To optimize the ionization step independently from surface extraction, the ORO reagent and its mixture with model compounds (triolein and linoleic acid) were first studied in solution using high‐resolution electrospray ionization tandem mass spectrometry (ESI‐MS/MS). Then, DESI‐MSI experiments were performed in both polarity modes for ORO‐processed fingermarks deposited on pieces of paper used as porous substrates. Results ESI‐MS of ORO reveals a complex mixture of azo dyes. Two main impurities detected beside the targeted species were characterized using MS/MS and then were usefully employed to produce DESI‐MS images of fingermarks, decreasing the scanning rate to get sufficient ion abundance from natural fingerprints. ORO did not prevent chemical profiling, and one major added value of this pink dye was to produce MS images with contrast that cannot be obtained optically for some colored substrates. Conclusions DESI‐MS has demonstrated imaging compatibility with the application of ORO used to enhance latent fingerprints on paper and could also enable chemical profiling in natural fingermarks. In addition, MS images of ORO impurities were of higher quality than optical ones for fingerprints revealed on colored paper.
Related Topics
Concepts
Desorption electrospray ionization
Chemistry
Mass spectrometry
Electrospray ionization
Chromatography
Direct electron ionization liquid chromatography–mass spectrometry interface
Analytical Chemistry (journal)
Extractive electrospray ionization
Electrospray
Ambient ionization
Ionization
Chemical ionization
Sample preparation in mass spectrometry
Ion
Organic chemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/rcm.9724
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/rcm.9724
- OA Status
- hybrid
- Cited By
- 4
- References
- 29
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4392286781
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4392286781Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/rcm.9724Digital Object Identifier
- Title
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Desorption electrospray ionization mass spectrometry imaging of latent fingerprints revealed by Oil Red OWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-02-29Full publication date if available
- Authors
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Mariska Banidol, Sophia Kouider, Isaure Sergent, Hélène Pizzala, Laurence CharlesList of authors in order
- Landing page
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https://doi.org/10.1002/rcm.9724Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/rcm.9724Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/rcm.9724Direct OA link when available
- Concepts
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Desorption electrospray ionization, Chemistry, Mass spectrometry, Electrospray ionization, Chromatography, Direct electron ionization liquid chromatography–mass spectrometry interface, Analytical Chemistry (journal), Extractive electrospray ionization, Electrospray, Ambient ionization, Ionization, Chemical ionization, Sample preparation in mass spectrometry, Ion, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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4Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2, 2024: 2Per-year citation counts (last 5 years)
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29Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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