Determining effective diffusion coefficients of chlorohydrocarbons in natural clays: Unique results from highly resolved controlled release field experiments Article Swipe
Beth L. Parker
,
John A. Cherry
,
Philipp Wanner
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.jconhyd.2022.104075
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.jconhyd.2022.104075
This study aims to precisely determine the effective diffusion coefficients of chlorohydrocarbons in low permeable units under in-situ field conditions. To this end, two controlled release field experiments using TCE and PCE as dense non-aqueous phase liquids (DNAPLs) were conducted in two natural clayey deposits. Several months to years after the controlled DNAPL release, highly resolved concentration profiles were determined for the chlorohydrocarbons that had diffused into the clayey deposits. Effective diffusion coefficients for TCE and PCE were then determined by calibrating a 3D numerical and 1D analytical model, respectively, to the measured high-resolution concentration profiles. The simulations revealed that the effective diffusion coefficients vary by as much as a factor of four within the same low permeability unit being consistent with observed small-scale heterogeneities. The determined chlorohydrocarbon effective diffusion coefficients were further used to determine the equivalent thickness of DNAPL that would completely dissolve in an idealized, parallel-plate fracture by diffusion transport into clayey deposits for the time periods of the controlled release field experiments. The equivalent TCE and PCE DNAPL film thicknesses ranged between 36 and 581 μm, respectively, comparable and exceeding fracture apertures measured in naturally fractured clay rich deposits. Hence, films of DNAPL initially contained within fractures in clay-rich deposits can completely dissolve away within a few months to a few years due to diffusion. This stored contaminant mass poses a risk to adjacent aquifers if it is re-released due to diffusion out of the matrix after source depletion or remediation.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.jconhyd.2022.104075
- OA Status
- hybrid
- Cited By
- 7
- References
- 39
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W4295277238Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.jconhyd.2022.104075Digital Object Identifier
- Title
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Determining effective diffusion coefficients of chlorohydrocarbons in natural clays: Unique results from highly resolved controlled release field experimentsWork title
- Type
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articleOpenAlex work type
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enPrimary language
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2022Year of publication
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2022-09-09Full publication date if available
- Authors
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Beth L. Parker, John A. Cherry, Philipp WannerList of authors in order
- Landing page
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https://doi.org/10.1016/j.jconhyd.2022.104075Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1016/j.jconhyd.2022.104075Direct OA link when available
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Diffusion, Environmental remediation, Permeability (electromagnetism), Aquifer, Soil science, Mineralogy, Chemistry, Groundwater, Geology, Materials science, Contamination, Geotechnical engineering, Thermodynamics, Membrane, Physics, Biology, Biochemistry, EcologyTop concepts (fields/topics) attached by OpenAlex
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7Total citation count in OpenAlex
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2025: 2, 2024: 1, 2023: 3, 2022: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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