Development of Scalable Reactive Transport Framework for PFAS Article Swipe
Christian D. Johnson
,
Christopher E. Bagwell
,
Rebecka Bence
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.2172/2204500
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.2172/2204500
Research on PFAS chemicals is extensive and covers all aspects, including analytical quantification, determination of properties, toxicology, ex situ treatment, and in situ remediation. PFAS chemicals are very stable and thus persistent/recalcitrant in the environment. Although there are many unknowns about PFAS chemicals, degradation pathways, reaction rates, etc., many different sorption, oxidation, reduction, biological, and innovative treatment approaches are being developed. Sorption with activated carbon is currently the only fully available in situ treatment technology for PFAS-impacted groundwater. Given the wide array of PFAS chemicals and transformation products, remediation may need multi-step treatment trains to fully address the PFAS contamination. The work here provides kinetic reaction modules that represent an initial cut at functionality representing PFAS migration and reaction in groundwater aquifer flow and transport models. One reaction kinetics module provides a method to model kinetically limited adsorption using a mass transfer model. The second reaction module represents biological transformation of 8:2 FTOH and daughter species, illustrating how a complex reaction pathway network can be represented. Both reaction modules allow for spatially variable parameter values so that a variety of remediation approaches (e.g., a PRB or volumetric treatment or variations in geochemical conditions) can be simulated. The intent with these PFAS reaction modules is to provide tools for practitioners to aid in the selection, design, and assessment of potential in situ PFAS remediation strategies. It is anticipated that, as PFAS remediation technologies and scientific understanding advances, these modules would be refined or replaced to match new knowledge.
Related Topics
Concepts
Metadata
- Type
- report
- Language
- en
- Landing Page
- https://doi.org/10.2172/2204500
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4388381340
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4388381340Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.2172/2204500Digital Object Identifier
- Title
-
Development of Scalable Reactive Transport Framework for PFASWork title
- Type
-
reportOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-10-01Full publication date if available
- Authors
-
Christian D. Johnson, Christopher E. Bagwell, Rebecka BenceList of authors in order
- Landing page
-
https://doi.org/10.2172/2204500Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://www.osti.gov/biblio/2204500Direct OA link when available
- Concepts
-
Computer science, Scalability, DatabaseTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
0Total citation count in OpenAlex
- Related works (count)
-
10Other works algorithmically related by OpenAlex
Full payload
| id | https://openalex.org/W4388381340 |
|---|---|
| doi | https://doi.org/10.2172/2204500 |
| ids.doi | https://doi.org/10.2172/2204500 |
| ids.openalex | https://openalex.org/W4388381340 |
| fwci | |
| type | report |
| title | Development of Scalable Reactive Transport Framework for PFAS |
| biblio.issue | |
| biblio.volume | |
| biblio.last_page | |
| biblio.first_page | |
| topics[0].id | https://openalex.org/T11362 |
| topics[0].field.id | https://openalex.org/fields/22 |
| topics[0].field.display_name | Engineering |
| topics[0].score | 0.9096999764442444 |
| topics[0].domain.id | https://openalex.org/domains/3 |
| topics[0].domain.display_name | Physical Sciences |
| topics[0].subfield.id | https://openalex.org/subfields/2210 |
| topics[0].subfield.display_name | Mechanical Engineering |
| topics[0].display_name | Membrane Separation and Gas Transport |
| is_xpac | False |
| apc_list | |
| apc_paid | |
| concepts[0].id | https://openalex.org/C41008148 |
| concepts[0].level | 0 |
| concepts[0].score | 0.4773699939250946 |
| concepts[0].wikidata | https://www.wikidata.org/wiki/Q21198 |
| concepts[0].display_name | Computer science |
| concepts[1].id | https://openalex.org/C48044578 |
| concepts[1].level | 2 |
| concepts[1].score | 0.46214187145233154 |
| concepts[1].wikidata | https://www.wikidata.org/wiki/Q727490 |
| concepts[1].display_name | Scalability |
| concepts[2].id | https://openalex.org/C77088390 |
| concepts[2].level | 1 |
| concepts[2].score | 0.12295159697532654 |
| concepts[2].wikidata | https://www.wikidata.org/wiki/Q8513 |
| concepts[2].display_name | Database |
| keywords[0].id | https://openalex.org/keywords/computer-science |
| keywords[0].score | 0.4773699939250946 |
| keywords[0].display_name | Computer science |
| keywords[1].id | https://openalex.org/keywords/scalability |
| keywords[1].score | 0.46214187145233154 |
| keywords[1].display_name | Scalability |
| keywords[2].id | https://openalex.org/keywords/database |
| keywords[2].score | 0.12295159697532654 |
| keywords[2].display_name | Database |
| language | en |
| locations[0].id | doi:10.2172/2204500 |
| locations[0].is_oa | False |
| locations[0].source | |
| locations[0].license | |
| locations[0].pdf_url | |
| locations[0].version | publishedVersion |
| locations[0].raw_type | report |
| locations[0].license_id | |
| locations[0].is_accepted | True |
| locations[0].is_published | True |
| locations[0].raw_source_name | |
| locations[0].landing_page_url | https://doi.org/10.2172/2204500 |
| locations[1].id | pmh:oai:osti.gov:2204500 |
| locations[1].is_oa | True |
| locations[1].source.id | https://openalex.org/S4306402487 |
| locations[1].source.issn | |
| locations[1].source.type | repository |
| locations[1].source.is_oa | False |
| locations[1].source.issn_l | |
| locations[1].source.is_core | False |
| locations[1].source.is_in_doaj | False |
| locations[1].source.display_name | OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) |
| locations[1].source.host_organization | https://openalex.org/I139351228 |
| locations[1].source.host_organization_name | Office of Scientific and Technical Information |
| locations[1].source.host_organization_lineage | https://openalex.org/I139351228 |
| locations[1].license | |
| locations[1].pdf_url | |
| locations[1].version | submittedVersion |
| locations[1].raw_type | |
| locations[1].license_id | |
| locations[1].is_accepted | False |
| locations[1].is_published | False |
| locations[1].raw_source_name | |
| locations[1].landing_page_url | https://www.osti.gov/biblio/2204500 |
| indexed_in | crossref |
| authorships[0].author.id | https://openalex.org/A5064320736 |
| authorships[0].author.orcid | https://orcid.org/0000-0002-3616-0378 |
| authorships[0].author.display_name | Christian D. Johnson |
| authorships[0].countries | US |
| authorships[0].affiliations[0].institution_ids | https://openalex.org/I142606810 |
| authorships[0].affiliations[0].raw_affiliation_string | Pacific Northwest National Laboratory (PNNL), Richland, WA (United States) |
| authorships[0].institutions[0].id | https://openalex.org/I142606810 |
| authorships[0].institutions[0].ror | https://ror.org/05h992307 |
| authorships[0].institutions[0].type | facility |
| authorships[0].institutions[0].lineage | https://openalex.org/I1325736334, https://openalex.org/I1330989302, https://openalex.org/I142606810, https://openalex.org/I39565521 |
| authorships[0].institutions[0].country_code | US |
| authorships[0].institutions[0].display_name | Pacific Northwest National Laboratory |
| authorships[0].author_position | first |
| authorships[0].raw_author_name | Christian Johnson |
| authorships[0].is_corresponding | False |
| authorships[0].raw_affiliation_strings | Pacific Northwest National Laboratory (PNNL), Richland, WA (United States) |
| authorships[1].author.id | https://openalex.org/A5020312707 |
| authorships[1].author.orcid | https://orcid.org/0000-0001-6140-4015 |
| authorships[1].author.display_name | Christopher E. Bagwell |
| authorships[1].countries | US |
| authorships[1].affiliations[0].institution_ids | https://openalex.org/I2799909505 |
| authorships[1].affiliations[0].raw_affiliation_string | Savannah River Site (SRS), Aiken, SC (United States) |
| authorships[1].institutions[0].id | https://openalex.org/I2799909505 |
| authorships[1].institutions[0].ror | https://ror.org/05vc7qy59 |
| authorships[1].institutions[0].type | facility |
| authorships[1].institutions[0].lineage | https://openalex.org/I1330989302, https://openalex.org/I2799909505, https://openalex.org/I4210093701 |
| authorships[1].institutions[0].country_code | US |
| authorships[1].institutions[0].display_name | Savannah River National Laboratory |
| authorships[1].author_position | middle |
| authorships[1].raw_author_name | Christopher Bagwell |
| authorships[1].is_corresponding | False |
| authorships[1].raw_affiliation_strings | Savannah River Site (SRS), Aiken, SC (United States) |
| authorships[2].author.id | https://openalex.org/A5093199414 |
| authorships[2].author.orcid | |
| authorships[2].author.display_name | Rebecka Bence |
| authorships[2].countries | US |
| authorships[2].affiliations[0].institution_ids | https://openalex.org/I142606810 |
| authorships[2].affiliations[0].raw_affiliation_string | Pacific Northwest National Laboratory (PNNL), Richland, WA (United States) |
| authorships[2].institutions[0].id | https://openalex.org/I142606810 |
| authorships[2].institutions[0].ror | https://ror.org/05h992307 |
| authorships[2].institutions[0].type | facility |
| authorships[2].institutions[0].lineage | https://openalex.org/I1325736334, https://openalex.org/I1330989302, https://openalex.org/I142606810, https://openalex.org/I39565521 |
| authorships[2].institutions[0].country_code | US |
| authorships[2].institutions[0].display_name | Pacific Northwest National Laboratory |
| authorships[2].author_position | last |
| authorships[2].raw_author_name | Rebecka Bence |
| authorships[2].is_corresponding | False |
| authorships[2].raw_affiliation_strings | Pacific Northwest National Laboratory (PNNL), Richland, WA (United States) |
| has_content.pdf | False |
| has_content.grobid_xml | False |
| is_paratext | False |
| open_access.is_oa | True |
| open_access.oa_url | https://www.osti.gov/biblio/2204500 |
| open_access.oa_status | green |
| open_access.any_repository_has_fulltext | False |
| created_date | 2025-10-10T00:00:00 |
| display_name | Development of Scalable Reactive Transport Framework for PFAS |
| has_fulltext | False |
| is_retracted | False |
| updated_date | 2025-11-06T03:46:38.306776 |
| primary_topic.id | https://openalex.org/T11362 |
| primary_topic.field.id | https://openalex.org/fields/22 |
| primary_topic.field.display_name | Engineering |
| primary_topic.score | 0.9096999764442444 |
| primary_topic.domain.id | https://openalex.org/domains/3 |
| primary_topic.domain.display_name | Physical Sciences |
| primary_topic.subfield.id | https://openalex.org/subfields/2210 |
| primary_topic.subfield.display_name | Mechanical Engineering |
| primary_topic.display_name | Membrane Separation and Gas Transport |
| related_works | https://openalex.org/W2748952813, https://openalex.org/W2390279801, https://openalex.org/W2358668433, https://openalex.org/W2376932109, https://openalex.org/W2001405890, https://openalex.org/W2389214306, https://openalex.org/W2382290278, https://openalex.org/W2350741829, https://openalex.org/W2130043461, https://openalex.org/W2530322880 |
| cited_by_count | 0 |
| locations_count | 2 |
| best_oa_location.id | pmh:oai:osti.gov:2204500 |
| best_oa_location.is_oa | True |
| best_oa_location.source.id | https://openalex.org/S4306402487 |
| best_oa_location.source.issn | |
| best_oa_location.source.type | repository |
| best_oa_location.source.is_oa | False |
| best_oa_location.source.issn_l | |
| best_oa_location.source.is_core | False |
| best_oa_location.source.is_in_doaj | False |
| best_oa_location.source.display_name | OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) |
| best_oa_location.source.host_organization | https://openalex.org/I139351228 |
| best_oa_location.source.host_organization_name | Office of Scientific and Technical Information |
| best_oa_location.source.host_organization_lineage | https://openalex.org/I139351228 |
| best_oa_location.license | |
| best_oa_location.pdf_url | |
| best_oa_location.version | submittedVersion |
| best_oa_location.raw_type | |
| best_oa_location.license_id | |
| best_oa_location.is_accepted | False |
| best_oa_location.is_published | False |
| best_oa_location.raw_source_name | |
| best_oa_location.landing_page_url | https://www.osti.gov/biblio/2204500 |
| primary_location.id | doi:10.2172/2204500 |
| primary_location.is_oa | False |
| primary_location.source | |
| primary_location.license | |
| primary_location.pdf_url | |
| primary_location.version | publishedVersion |
| primary_location.raw_type | report |
| primary_location.license_id | |
| primary_location.is_accepted | True |
| primary_location.is_published | True |
| primary_location.raw_source_name | |
| primary_location.landing_page_url | https://doi.org/10.2172/2204500 |
| publication_date | 2023-10-01 |
| publication_year | 2023 |
| referenced_works_count | 0 |
| abstract_inverted_index.a | 131, 139, 158, 177, 183 |
| abstract_inverted_index.It | 224 |
| abstract_inverted_index.an | 109 |
| abstract_inverted_index.as | 228 |
| abstract_inverted_index.at | 112 |
| abstract_inverted_index.be | 164, 194, 239 |
| abstract_inverted_index.ex | 17 |
| abstract_inverted_index.in | 21, 32, 71, 119, 190, 211, 219 |
| abstract_inverted_index.is | 4, 65, 203, 225 |
| abstract_inverted_index.of | 14, 82, 150, 179, 217 |
| abstract_inverted_index.on | 1 |
| abstract_inverted_index.or | 185, 188, 241 |
| abstract_inverted_index.so | 175 |
| abstract_inverted_index.to | 94, 133, 204, 209, 243 |
| abstract_inverted_index.8:2 | 151 |
| abstract_inverted_index.One | 126 |
| abstract_inverted_index.PRB | 184 |
| abstract_inverted_index.The | 100, 143, 196 |
| abstract_inverted_index.aid | 210 |
| abstract_inverted_index.all | 8 |
| abstract_inverted_index.and | 6, 20, 29, 54, 85, 117, 123, 153, 215, 232 |
| abstract_inverted_index.are | 26, 37, 58 |
| abstract_inverted_index.can | 163, 193 |
| abstract_inverted_index.cut | 111 |
| abstract_inverted_index.for | 75, 170, 207 |
| abstract_inverted_index.how | 157 |
| abstract_inverted_index.may | 89 |
| abstract_inverted_index.new | 245 |
| abstract_inverted_index.the | 33, 67, 79, 97, 212 |
| abstract_inverted_index.Both | 166 |
| abstract_inverted_index.FTOH | 152 |
| abstract_inverted_index.PFAS | 2, 24, 41, 83, 98, 115, 200, 221, 229 |
| abstract_inverted_index.flow | 122 |
| abstract_inverted_index.here | 102 |
| abstract_inverted_index.many | 38, 48 |
| abstract_inverted_index.mass | 140 |
| abstract_inverted_index.need | 90 |
| abstract_inverted_index.only | 68 |
| abstract_inverted_index.situ | 18, 22, 72, 220 |
| abstract_inverted_index.that | 107, 176 |
| abstract_inverted_index.thus | 30 |
| abstract_inverted_index.very | 27 |
| abstract_inverted_index.wide | 80 |
| abstract_inverted_index.with | 62, 198 |
| abstract_inverted_index.work | 101 |
| abstract_inverted_index.Given | 78 |
| abstract_inverted_index.about | 40 |
| abstract_inverted_index.allow | 169 |
| abstract_inverted_index.array | 81 |
| abstract_inverted_index.being | 59 |
| abstract_inverted_index.etc., | 47 |
| abstract_inverted_index.fully | 69, 95 |
| abstract_inverted_index.match | 244 |
| abstract_inverted_index.model | 134 |
| abstract_inverted_index.that, | 227 |
| abstract_inverted_index.there | 36 |
| abstract_inverted_index.these | 199, 236 |
| abstract_inverted_index.tools | 206 |
| abstract_inverted_index.using | 138 |
| abstract_inverted_index.would | 238 |
| abstract_inverted_index.(e.g., | 182 |
| abstract_inverted_index.carbon | 64 |
| abstract_inverted_index.covers | 7 |
| abstract_inverted_index.intent | 197 |
| abstract_inverted_index.method | 132 |
| abstract_inverted_index.model. | 142 |
| abstract_inverted_index.module | 129, 146 |
| abstract_inverted_index.rates, | 46 |
| abstract_inverted_index.second | 144 |
| abstract_inverted_index.stable | 28 |
| abstract_inverted_index.trains | 93 |
| abstract_inverted_index.values | 174 |
| abstract_inverted_index.address | 96 |
| abstract_inverted_index.aquifer | 121 |
| abstract_inverted_index.complex | 159 |
| abstract_inverted_index.design, | 214 |
| abstract_inverted_index.initial | 110 |
| abstract_inverted_index.kinetic | 104 |
| abstract_inverted_index.limited | 136 |
| abstract_inverted_index.models. | 125 |
| abstract_inverted_index.modules | 106, 168, 202, 237 |
| abstract_inverted_index.network | 162 |
| abstract_inverted_index.pathway | 161 |
| abstract_inverted_index.provide | 205 |
| abstract_inverted_index.refined | 240 |
| abstract_inverted_index.variety | 178 |
| abstract_inverted_index.Although | 35 |
| abstract_inverted_index.Research | 0 |
| abstract_inverted_index.Sorption | 61 |
| abstract_inverted_index.aspects, | 9 |
| abstract_inverted_index.daughter | 154 |
| abstract_inverted_index.kinetics | 128 |
| abstract_inverted_index.provides | 103, 130 |
| abstract_inverted_index.reaction | 45, 105, 118, 127, 145, 160, 167, 201 |
| abstract_inverted_index.replaced | 242 |
| abstract_inverted_index.species, | 155 |
| abstract_inverted_index.transfer | 141 |
| abstract_inverted_index.unknowns | 39 |
| abstract_inverted_index.variable | 172 |
| abstract_inverted_index.activated | 63 |
| abstract_inverted_index.advances, | 235 |
| abstract_inverted_index.available | 70 |
| abstract_inverted_index.chemicals | 3, 25, 84 |
| abstract_inverted_index.currently | 66 |
| abstract_inverted_index.different | 49 |
| abstract_inverted_index.extensive | 5 |
| abstract_inverted_index.including | 10 |
| abstract_inverted_index.migration | 116 |
| abstract_inverted_index.parameter | 173 |
| abstract_inverted_index.pathways, | 44 |
| abstract_inverted_index.potential | 218 |
| abstract_inverted_index.products, | 87 |
| abstract_inverted_index.represent | 108 |
| abstract_inverted_index.sorption, | 50 |
| abstract_inverted_index.spatially | 171 |
| abstract_inverted_index.transport | 124 |
| abstract_inverted_index.treatment | 56, 73, 92, 187 |
| abstract_inverted_index.adsorption | 137 |
| abstract_inverted_index.analytical | 11 |
| abstract_inverted_index.approaches | 57, 181 |
| abstract_inverted_index.assessment | 216 |
| abstract_inverted_index.biological | 148 |
| abstract_inverted_index.chemicals, | 42 |
| abstract_inverted_index.developed. | 60 |
| abstract_inverted_index.innovative | 55 |
| abstract_inverted_index.knowledge. | 246 |
| abstract_inverted_index.multi-step | 91 |
| abstract_inverted_index.oxidation, | 51 |
| abstract_inverted_index.reduction, | 52 |
| abstract_inverted_index.represents | 147 |
| abstract_inverted_index.scientific | 233 |
| abstract_inverted_index.selection, | 213 |
| abstract_inverted_index.simulated. | 195 |
| abstract_inverted_index.technology | 74 |
| abstract_inverted_index.treatment, | 19 |
| abstract_inverted_index.variations | 189 |
| abstract_inverted_index.volumetric | 186 |
| abstract_inverted_index.anticipated | 226 |
| abstract_inverted_index.biological, | 53 |
| abstract_inverted_index.conditions) | 192 |
| abstract_inverted_index.degradation | 43 |
| abstract_inverted_index.geochemical | 191 |
| abstract_inverted_index.groundwater | 120 |
| abstract_inverted_index.kinetically | 135 |
| abstract_inverted_index.properties, | 15 |
| abstract_inverted_index.remediation | 88, 180, 222, 230 |
| abstract_inverted_index.strategies. | 223 |
| abstract_inverted_index.toxicology, | 16 |
| abstract_inverted_index.environment. | 34 |
| abstract_inverted_index.groundwater. | 77 |
| abstract_inverted_index.illustrating | 156 |
| abstract_inverted_index.remediation. | 23 |
| abstract_inverted_index.represented. | 165 |
| abstract_inverted_index.representing | 114 |
| abstract_inverted_index.technologies | 231 |
| abstract_inverted_index.PFAS-impacted | 76 |
| abstract_inverted_index.determination | 13 |
| abstract_inverted_index.functionality | 113 |
| abstract_inverted_index.practitioners | 208 |
| abstract_inverted_index.understanding | 234 |
| abstract_inverted_index.contamination. | 99 |
| abstract_inverted_index.transformation | 86, 149 |
| abstract_inverted_index.quantification, | 12 |
| abstract_inverted_index.persistent/recalcitrant | 31 |
| cited_by_percentile_year | |
| countries_distinct_count | 1 |
| institutions_distinct_count | 3 |
| citation_normalized_percentile |