Dichography: Two-frame Ultrafast Imaging from a Single Diffraction Pattern Article Swipe
YOU?
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· 2025
· Open Access
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· DOI: https://doi.org/10.48550/arxiv.2508.20153
X-ray free-electron lasers can nowadays deliver pairs of ultrabright, ultrashort light pulses with controllable delays at different photon energies. When combined with diffraction experiments, the interaction of these pulses with a sample at different times can produce two snapshots of an evolving system, enabling spatial and temporal resolution of ultrafast dynamics in nanomatter at and beyond the terahertz time scale. However, light detectors are orders of magnitude slower. The diffraction signals from the two pulses overlap in the recorded data and cannot be separated using currently available analysis methods. Here, we address this challenge by introducing Dichography, a diffraction imaging technique that restores the two unique views of the sample from superimposed scattering signals. We apply Dichography to experimental diffraction patterns of isolated xenon-doped superfluid helium nanodroplets, imaged using time-delayed, two-color X-ray pulses at intensities near the detection limit. The reconstructed images provide evidence of the survival of the xenon structures up to 750 fs after the interaction with the first shot. The capabilities of Dichography are further explored by applying the method to data from a second experiment, in which we retrieve the images of two distinct silver nanoparticles intercepted by the same light pulse. Dichography enables a new class of experiments for spatially and temporally resolving ultrafast phenomena, making a significant step toward the original promise of X-ray free-electron lasers to capture ultrafast movies of nanomatter.
Related Topics
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2508.20153
- https://arxiv.org/pdf/2508.20153
- OA Status
- green
- OpenAlex ID
- https://openalex.org/W4416681809
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4416681809Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2508.20153Digital Object Identifier
- Title
-
Dichography: Two-frame Ultrafast Imaging from a Single Diffraction PatternWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2025Year of publication
- Publication date
-
2025-08-27Full publication date if available
- Authors
-
Linos Hecht, André Al Haddad, Björn Bastian, T. Baumann, Johan Bielecki, Christoph Bostedt, Subhendu De, Simon Dold, Fanny Goy, Christina Gräf, Gregor Knopp, Katharina Kolatzki, Sivarama Krishnan, Björn Kruse, Asbjørn Ø. Lægdsmand, Bruno Langbehn, S. Mandal, Tommaso Mazza, Michael Meyer, Christian Peltz, Thomas Pfeifer, Safi Rafie-Zinedine, Antoine Sarracini, Mario Sauppe, Florian Schenk, Björn Senfftleben, F. Stienkemeier, Zhibin Sun, Rico Mayro P. Tanyag, Paul Tümmler, Sergey Usenko, Carl Frederic Ussling, Vanessa Wood, Alessandro ColomboList of authors in order
- Landing page
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https://arxiv.org/abs/2508.20153Publisher landing page
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https://arxiv.org/pdf/2508.20153Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
-
https://arxiv.org/pdf/2508.20153Direct OA link when available
- Cited by
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0Total citation count in OpenAlex
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| abstract_inverted_index.scale. | 59 |
| abstract_inverted_index.second | 177 |
| abstract_inverted_index.silver | 188 |
| abstract_inverted_index.toward | 214 |
| abstract_inverted_index.unique | 105 |
| abstract_inverted_index.address | 91 |
| abstract_inverted_index.capture | 223 |
| abstract_inverted_index.deliver | 5 |
| abstract_inverted_index.enables | 197 |
| abstract_inverted_index.further | 167 |
| abstract_inverted_index.imaging | 99 |
| abstract_inverted_index.overlap | 75 |
| abstract_inverted_index.produce | 36 |
| abstract_inverted_index.promise | 217 |
| abstract_inverted_index.provide | 142 |
| abstract_inverted_index.signals | 70 |
| abstract_inverted_index.slower. | 67 |
| abstract_inverted_index.spatial | 44 |
| abstract_inverted_index.system, | 42 |
| abstract_inverted_index.However, | 60 |
| abstract_inverted_index.analysis | 87 |
| abstract_inverted_index.applying | 170 |
| abstract_inverted_index.combined | 20 |
| abstract_inverted_index.distinct | 187 |
| abstract_inverted_index.dynamics | 50 |
| abstract_inverted_index.enabling | 43 |
| abstract_inverted_index.evidence | 143 |
| abstract_inverted_index.evolving | 41 |
| abstract_inverted_index.explored | 168 |
| abstract_inverted_index.isolated | 122 |
| abstract_inverted_index.methods. | 88 |
| abstract_inverted_index.nowadays | 4 |
| abstract_inverted_index.original | 216 |
| abstract_inverted_index.patterns | 120 |
| abstract_inverted_index.recorded | 78 |
| abstract_inverted_index.restores | 102 |
| abstract_inverted_index.retrieve | 182 |
| abstract_inverted_index.signals. | 113 |
| abstract_inverted_index.survival | 146 |
| abstract_inverted_index.temporal | 46 |
| abstract_inverted_index.available | 86 |
| abstract_inverted_index.challenge | 93 |
| abstract_inverted_index.currently | 85 |
| abstract_inverted_index.detection | 137 |
| abstract_inverted_index.detectors | 62 |
| abstract_inverted_index.different | 16, 33 |
| abstract_inverted_index.energies. | 18 |
| abstract_inverted_index.magnitude | 66 |
| abstract_inverted_index.resolving | 207 |
| abstract_inverted_index.separated | 83 |
| abstract_inverted_index.snapshots | 38 |
| abstract_inverted_index.spatially | 204 |
| abstract_inverted_index.technique | 100 |
| abstract_inverted_index.terahertz | 57 |
| abstract_inverted_index.two-color | 130 |
| abstract_inverted_index.ultrafast | 49, 208, 224 |
| abstract_inverted_index.nanomatter | 52 |
| abstract_inverted_index.phenomena, | 209 |
| abstract_inverted_index.resolution | 47 |
| abstract_inverted_index.scattering | 112 |
| abstract_inverted_index.structures | 150 |
| abstract_inverted_index.superfluid | 124 |
| abstract_inverted_index.temporally | 206 |
| abstract_inverted_index.ultrashort | 9 |
| abstract_inverted_index.Dichography | 116, 165, 196 |
| abstract_inverted_index.diffraction | 22, 69, 98, 119 |
| abstract_inverted_index.experiment, | 178 |
| abstract_inverted_index.experiments | 202 |
| abstract_inverted_index.intensities | 134 |
| abstract_inverted_index.interaction | 25, 157 |
| abstract_inverted_index.intercepted | 190 |
| abstract_inverted_index.introducing | 95 |
| abstract_inverted_index.nanomatter. | 227 |
| abstract_inverted_index.significant | 212 |
| abstract_inverted_index.xenon-doped | 123 |
| abstract_inverted_index.Dichography, | 96 |
| abstract_inverted_index.capabilities | 163 |
| abstract_inverted_index.controllable | 13 |
| abstract_inverted_index.experimental | 118 |
| abstract_inverted_index.experiments, | 23 |
| abstract_inverted_index.superimposed | 111 |
| abstract_inverted_index.ultrabright, | 8 |
| abstract_inverted_index.free-electron | 1, 220 |
| abstract_inverted_index.nanodroplets, | 126 |
| abstract_inverted_index.nanoparticles | 189 |
| abstract_inverted_index.reconstructed | 140 |
| abstract_inverted_index.time-delayed, | 129 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 34 |
| citation_normalized_percentile |