Die gemeinsamen Zwischenprodukte von Sauerstoffentwicklung und Auflösung während der Wasserelektrolyse an Iridium Article Swipe
Olga Kasian
,
Jan‐Philipp Grote
,
Simon Geiger
,
Serhiy Cherevko
,
Karl J. J. Mayrhofer
·
YOU?
·
· 2017
· Open Access
·
· DOI: https://doi.org/10.1002/ange.201709652
YOU?
·
· 2017
· Open Access
·
· DOI: https://doi.org/10.1002/ange.201709652
Dem Wissen über Reaktionsmechanismen beim Katalysatorabbau während der Sauerstoffentwicklung kommt eine Schlüsselrolle bei der Weiterentwicklung von effizienteren und stabileren Elektrolyseuren zu, da die korrosiven Bedingungen an der Anode selbst für vielversprechende Materialien auf Iridium‐Basis problematisch sind. Der Auflösungsmechanismus ist von komplexer Natur, und Zusammenhänge mit der Sauerstoffentwicklung sind wenig erforscht. Die Kopplung einer Rasterflusszelle mit Massenspektrometrie ermöglicht es, Sauerstoffentwicklungs‐ und Abbauprodukte in situ zu detektieren. Demnach sind bei hohen anodischen Potentialen mehrere Auflösungswege möglich, welche auch die Bildung von gasförmigem IrO 3 beinhalten. Auf der Basis der experimentellen Daten werden mögliche Reaktionswege der, durch Sauerstoffentwicklung bedingten, Auflösung von Iridium aufgezeigt und die Rolle von gemeinsamen Intermediaten dieser Reaktionen diskutiert.
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Die gemeinsamen Zwischenprodukte von Sauerstoffentwicklung und Auflösung während der Wasserelektrolyse an IridiumWork title
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articleOpenAlex work type
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dePrimary language
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2017-12-08Full publication date if available
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Olga Kasian, Jan‐Philipp Grote, Simon Geiger, Serhiy Cherevko, Karl J. J. MayrhoferList of authors in order
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https://doi.org/10.1002/ange.201709652Publisher landing page
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39Total citation count in OpenAlex
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2025: 2, 2024: 1, 2023: 4, 2022: 7, 2021: 5Per-year citation counts (last 5 years)
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| corresponding_author_ids | https://openalex.org/A5073632920, https://openalex.org/A5026988312, https://openalex.org/A5073666601, https://openalex.org/A5053735446, https://openalex.org/A5077398710 |
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