Diffuson-mediated thermal and ionic transport in superionic conductors Article Swipe
Tim Bernges
,
Riley Hanus
,
Bjöern Wankmiller
,
Kazuki Imasato
,
Siqi Lin
,
Michael Ghidiu
,
Marius Gerlitz
,
Martin Peterlechner
,
Samuel A. Graham
,
Geoffroy Hautier
,
Yanzhong Pei
,
Michael Ryan Hansen
,
Gerhard Wilde
,
G. Jeffrey Snyder
,
Janine George
,
Matthias T. Agne
,
Wolfgang G. Zeier
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2021-3zxh4
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2021-3zxh4
Ultra-low lattice thermal conductivity as often found in superionic compounds is greatly beneficial for thermoelectric performance, however, a high ionic conductivity can lead to device degradation. Conversely, high ionic conductivities are searched for materials in solid-state battery applications. It is commonly thought that ionic transport induces low thermal conductivity and that ion and thermal transport are not completely independent properties of a material. However, no direct comparison or underlying physical relationship has been shown between the two. Here we establish that ionic transport can be varied independent of thermal transport in Ag+ superionic conductors, even though both phenomena arise from atomic vibrations. Thermal conductivity measurements, in conjunction with two-channel lattice dynamics modeling, reveals that the vast majority of Ag+ vibrations have non-propagating diffuson-like character, which provides a rational for how these two transport properties can be independent. Our results provide conceptually novel lattice dynamical insights to ionic transport and confirm that ion transport is not a requirement for ultra-low thermal conductivity. Consequently, this work bridges the fields of solid state ionics and thermal transport, thus providing design strategies for functional ionic conducting materials from a vibrational perspective.
Related Topics
Concepts
Ionic bonding
Ionic conductivity
Thermal conductivity
Chemical physics
Ion
Fast ion conductor
Materials science
Thermal conduction
Thermal
Thermoelectric materials
Lattice (music)
Electrical conductor
Ion transporter
Condensed matter physics
Chemistry
Thermodynamics
Electrolyte
Physics
Physical chemistry
Electrode
Composite material
Organic chemistry
Acoustics
Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.26434/chemrxiv-2021-3zxh4
- https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/615406c0700ea66fa971b86a/original/diffuson-mediated-thermal-and-ionic-transport-in-superionic-conductors.pdf
- OA Status
- gold
- Cited By
- 2
- References
- 39
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4238604553
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4238604553Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.26434/chemrxiv-2021-3zxh4Digital Object Identifier
- Title
-
Diffuson-mediated thermal and ionic transport in superionic conductorsWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2021Year of publication
- Publication date
-
2021-09-29Full publication date if available
- Authors
-
Tim Bernges, Riley Hanus, Bjöern Wankmiller, Kazuki Imasato, Siqi Lin, Michael Ghidiu, Marius Gerlitz, Martin Peterlechner, Samuel A. Graham, Geoffroy Hautier, Yanzhong Pei, Michael Ryan Hansen, Gerhard Wilde, G. Jeffrey Snyder, Janine George, Matthias T. Agne, Wolfgang G. ZeierList of authors in order
- Landing page
-
https://doi.org/10.26434/chemrxiv-2021-3zxh4Publisher landing page
- PDF URL
-
https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/615406c0700ea66fa971b86a/original/diffuson-mediated-thermal-and-ionic-transport-in-superionic-conductors.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/615406c0700ea66fa971b86a/original/diffuson-mediated-thermal-and-ionic-transport-in-superionic-conductors.pdfDirect OA link when available
- Concepts
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Ionic bonding, Ionic conductivity, Thermal conductivity, Chemical physics, Ion, Fast ion conductor, Materials science, Thermal conduction, Thermal, Thermoelectric materials, Lattice (music), Electrical conductor, Ion transporter, Condensed matter physics, Chemistry, Thermodynamics, Electrolyte, Physics, Physical chemistry, Electrode, Composite material, Organic chemistry, AcousticsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
2Total citation count in OpenAlex
- Citations by year (recent)
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2022: 2Per-year citation counts (last 5 years)
- References (count)
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39Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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