Dilution of the magnetic lattice in the Kitaev candidate $α$-RuCl$_3$ by Rh$^{3+}$ doping Article Swipe
G. Bastien
,
E. Vinokurova
,
M. Lange
,
K. K. Bestha
,
L. T. Corredor
,
G. Kreutzer
,
A. Lubk
,
Thomas Doert
,
B. Buchner
,
A. Isaeva
,
A. U. B. Wolter
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2209.08986
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2209.08986
Magnetic dilution of a well-established Kitaev candidate system is realized in the substitutional Ru$_{1-x}$Rh$_x$Cl$_3$ series ($x = 0.02-0.6$). Optimized syntheses protocols yield uniformly-doped single crystals and polycrystalline powders that are isostructural to the parental $α$-RuCl$_3$ as per X-ray diffraction. The Rh content $x$ is accurately determined by the quantitative energy-dispersive X-ray spectroscopy technique with standards. We determine the magnetic phase diagram of Ru$_{1-x}$Rh$_x$Cl$_3$ for in-plane magnetic fields from magnetization and specific-heat measurements as a function of $x$ and stacking periodicity, and identify the suppression of the magnetic order at $x \approx 0.2$ towards a disordered phase, which does not show any clear signature of freezing into a spin glass. Comparing with previous studies on the substitution series Ru$_{1-x}$Ir$_x$Cl$_3$, we propose that chemical pressure would contribute to the suppression of magnetic order especially in Ru$_{1-x}$Ir$_x$Cl$_3$ and that the zigzag magnetic ground state appears to be relatively robust with respect to the dilution of the Kitaev--$Γ$--Heisenberg magnetic lattice. We also discovered a slight dependence of the magnetic properties on thermal cycling, which would be due to an incomplete structural transition.
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- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2209.08986
- https://arxiv.org/pdf/2209.08986
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4296564918
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https://openalex.org/W4296564918Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2209.08986Digital Object Identifier
- Title
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Dilution of the magnetic lattice in the Kitaev candidate $α$-RuCl$_3$ by Rh$^{3+}$ dopingWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-09-19Full publication date if available
- Authors
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G. Bastien, E. Vinokurova, M. Lange, K. K. Bestha, L. T. Corredor, G. Kreutzer, A. Lubk, Thomas Doert, B. Buchner, A. Isaeva, A. U. B. WolterList of authors in order
- Landing page
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https://arxiv.org/abs/2209.08986Publisher landing page
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https://arxiv.org/pdf/2209.08986Direct link to full text PDF
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://arxiv.org/pdf/2209.08986Direct OA link when available
- Concepts
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Isostructural, Magnetization, Condensed matter physics, Phase diagram, Crystallite, Materials science, Dilution, Spin glass, Crystallography, Crystal structure, Analytical Chemistry (journal), Chemistry, Phase (matter), Physics, Magnetic field, Thermodynamics, Organic chemistry, Chromatography, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.crystals | 24 |
| abstract_inverted_index.cycling, | 168 |
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| abstract_inverted_index.lattice. | 155 |
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| abstract_inverted_index.stacking | 78 |
| abstract_inverted_index.Comparing | 109 |
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| abstract_inverted_index.spectroscopy | 51 |
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| abstract_inverted_index.Ru$_{1-x}$Rh$_x$Cl$_3$ | 13, 62 |
| abstract_inverted_index.Ru$_{1-x}$Ir$_x$Cl$_3$, | 117 |
| abstract_inverted_index.Kitaev--$Γ$--Heisenberg | 153 |
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| sustainable_development_goals[0].display_name | Affordable and clean energy |
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