Dynamically Stable and Amplified Circularly Polarized Excimer Emission (CPEE) of Achiral Pyrene-Based Dye Regulated by Solvation of Chiral Co-assembly Process Article Swipe
Yuxia Zhang
,
Hang Li
,
Zhongxing Geng
,
Wen‐Hua Zheng
,
Yiwu Quan
,
Yixiang Cheng
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-1720043/v1
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-1720043/v1
Chiral supramolecular assembly has been assigned to be one of the most favorable strategies for the development of excellent circularly polarized luminescent (CPL)-active materials. Herein, we report our study of an achiral boron-containing pyrene (Py)-based chromophore (PyBO) as a circularly polarized excimer emission (CPEE) dye induced by chiral co-assemblies containing chiral binaphthyl-based enantiomers (R/S-M). Chiral co-assembly R/S-M-(PyBO)4 fresh film spin-coated from toluene solution can exhibit orderly nanofibers and strong green CPEE (λem = 512 nm, gem = ± 0.45, ΦFL = 51.2 %) resulting from an achiral PyBO excimer. In contrast, only a very weak blue CPL was observed (λem = 461 nm, gem = ± 0.0125, ΦFL = 19.0 %) after 187 h due to PyBO monomer emission as spherulite growth. Interestingly, this kind of chiral co-assembly R-M-(PyBO)4-T film from tetrahydrofuran (THF) solution retains uniform morphology and affords the most stable and strongest CPEE performance (λem = 512 nm, gem = + 0.62, ΦFL = 53.3 %) after 10 days.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-1720043/v1
- https://www.researchsquare.com/article/rs-1720043/latest.pdf
- OA Status
- green
- References
- 38
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4282918847
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Raw OpenAlex JSON
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https://openalex.org/W4282918847Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.21203/rs.3.rs-1720043/v1Digital Object Identifier
- Title
-
Dynamically Stable and Amplified Circularly Polarized Excimer Emission (CPEE) of Achiral Pyrene-Based Dye Regulated by Solvation of Chiral Co-assembly ProcessWork title
- Type
-
preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-06-14Full publication date if available
- Authors
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Yuxia Zhang, Hang Li, Zhongxing Geng, Wen‐Hua Zheng, Yiwu Quan, Yixiang ChengList of authors in order
- Landing page
-
https://doi.org/10.21203/rs.3.rs-1720043/v1Publisher landing page
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https://www.researchsquare.com/article/rs-1720043/latest.pdfDirect link to full text PDF
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.researchsquare.com/article/rs-1720043/latest.pdfDirect OA link when available
- Concepts
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Excimer, Pyrene, Tetrahydrofuran, Materials science, Chromophore, Photochemistry, Enantiomer, Luminescence, Crystallography, Fluorescence, Chemistry, Stereochemistry, Optoelectronics, Optics, Organic chemistry, Physics, SolventTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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38Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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