Effect of A-site element on the performance of three-dimensionally ordered macroporous manganese-based perovskite catalyst Article Swipe
Xin Liu
,
Yongqiang Wang
,
Meng Zang
,
Lin Shi
,
Huiying Zhang
,
Chaocheng Zhao
·
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1016/j.jscs.2020.03.005
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1016/j.jscs.2020.03.005
Three-dimensionally ordered macroporous manganese-based perovskite catalyst (3DOM AMnO3, A = Ce, La, Ni) were synthesized by PMMA hard-templating and impregnation method. Physicochemical properties of the samples were characterized by means of various techniques including XRD, BET, SEM, TEM, XPS and H2-TPR, and their catalytic activities were evaluated by toluene combustion. It was found that the 3DOM AMnO3 in each of the samples was perovskite in crystal structure, and only the samples possessed a good quality 3DOM architecture with a surface area of 48.8 m2/g. Due to the highest adsorbed oxygen species concentration (Oads/Olatt = 2.330), the best low-temperature reducibility (The low-temperature reduction peaks of 3DOM CeMnO3 catalysts occur at 425 °C) and the strong interaction between CeO2 and MnOx formed during calcination. The 3DOM CeMnO3 sample showed lower apparent activation energy (34.51 kJ·mol−1, SV = 15,000 h−1) and the best catalytic activity for toluene combustion, with the reaction temperatures (T50%, and T90%) required for achieving toluene conversions of 50%, and 90% being 100 °C, 172 °C at SV = 15,000 h−1, respectively. Keywords: 3DOM, Manganese-based, Perovskite catalyst, A-site element, Catalytic combustion
Related Topics
Concepts
Calcination
Catalysis
Toluene
Manganese
Perovskite (structure)
X-ray photoelectron spectroscopy
Adsorption
Materials science
Specific surface area
Activation energy
Combustion
Catalytic combustion
Chemistry
Chemical engineering
Inorganic chemistry
Nuclear chemistry
Physical chemistry
Crystallography
Organic chemistry
Metallurgy
Engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.jscs.2020.03.005
- OA Status
- hybrid
- Cited By
- 18
- References
- 42
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3013986271
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3013986271Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.jscs.2020.03.005Digital Object Identifier
- Title
-
Effect of A-site element on the performance of three-dimensionally ordered macroporous manganese-based perovskite catalystWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2020Year of publication
- Publication date
-
2020-03-26Full publication date if available
- Authors
-
Xin Liu, Yongqiang Wang, Meng Zang, Lin Shi, Huiying Zhang, Chaocheng ZhaoList of authors in order
- Landing page
-
https://doi.org/10.1016/j.jscs.2020.03.005Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1016/j.jscs.2020.03.005Direct OA link when available
- Concepts
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Calcination, Catalysis, Toluene, Manganese, Perovskite (structure), X-ray photoelectron spectroscopy, Adsorption, Materials science, Specific surface area, Activation energy, Combustion, Catalytic combustion, Chemistry, Chemical engineering, Inorganic chemistry, Nuclear chemistry, Physical chemistry, Crystallography, Organic chemistry, Metallurgy, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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18Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 6, 2023: 3, 2022: 5, 2021: 1Per-year citation counts (last 5 years)
- References (count)
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42Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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