Effect of Anode Porosity and Temperature on the Performance and Lithium Plating During Fast‐Charging of Lithium‐Ion Cells Article Swipe
David Robertson
,
LeRoy Flores
,
Alison R. Dunlop
,
Stephen E. Trask
,
Francois L. E. Usseglio‐Viretta
,
Andrew M. Colclasure
,
Zhenzhen Yang
,
Ira Bloom
·
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1002/ente.202000666
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1002/ente.202000666
Twenty‐four single‐layer ≈32 mAh pouch cells are tested to determine the effect of electrode porosity on lithium plating. Twelve cells contain a graphite electrode that is 26% porous, and 47% for the other twelve. The cells are cycled using a 6‐C charge and a C/2 discharge protocol at temperatures in the range of 20‐50 °C. A macro‐homogeneous electrochemical model and microstructure analysis tool set are used to help interpret experimental observations for the effect of anode porosity and ambient temperature on fast‐charging performance. Comparison between the two also highlights gaps in current theoretical understanding that need to be addressed. In post‐test examination, lithium plating is seen in all cells, regardless of porosity. Elevated temperature is shown to reduce the amount of lithium plating and improve initial fast‐charge capacity, but also changes the rate of other, less well‐understood degradation mechanisms. Apparent kinetic rate laws, At + Bt 1/2 , where A and B are constants, can be fit to most of the capacity loss and resistance increase data. The relative magnitudes of A and B change with temperature and porosity. The capacity loss data at 50 °C from the high‐porosity cells are fit by a logistics rate law.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/ente.202000666
- OA Status
- green
- Cited By
- 27
- References
- 39
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3093570699
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3093570699Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/ente.202000666Digital Object Identifier
- Title
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Effect of Anode Porosity and Temperature on the Performance and Lithium Plating During Fast‐Charging of Lithium‐Ion CellsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2020Year of publication
- Publication date
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2020-10-25Full publication date if available
- Authors
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David Robertson, LeRoy Flores, Alison R. Dunlop, Stephen E. Trask, Francois L. E. Usseglio‐Viretta, Andrew M. Colclasure, Zhenzhen Yang, Ira BloomList of authors in order
- Landing page
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https://doi.org/10.1002/ente.202000666Publisher landing page
- Open access
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/1755739Direct OA link when available
- Concepts
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Porosity, Anode, Materials science, Lithium (medication), Electrochemistry, Plating (geology), Electrode, Microstructure, Composite material, Chemical engineering, Analytical Chemistry (journal), Chemistry, Chromatography, Physical chemistry, Engineering, Geophysics, Geology, Medicine, EndocrinologyTop concepts (fields/topics) attached by OpenAlex
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27Total citation count in OpenAlex
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2025: 6, 2024: 3, 2023: 4, 2022: 8, 2021: 6Per-year citation counts (last 5 years)
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39Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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